scholarly journals Studying the Linear and Nonlinear Optical Properties by Using Z-Scan Technique for CdS Thin Films Prepared by CBD Technique

2018 ◽  
Vol 10 (3) ◽  
pp. 7
Author(s):  
Ahmed S. Jabbar ◽  
Sabah I. Abbas ◽  
Muneer H. Al-zubaidy

CdS films prepared by using CBD technique, linear optical properties tests measured by UV-3000 Nano from OPTIMA, nonlinear properties contained the nonlinear refractive index and nonlinear absorption coefficient by using single light beam source green semiconductor developed laser (SZ- 303 LASER) with material Nd:YVO4+KTP or Aluminum Alloy, and Wavelength Range is (532 nm), Beam Dimension 6 Meter distance Output Laser spot 18 mm ± 2.0 mm.

1993 ◽  
Vol 329 ◽  
Author(s):  
Douglas A. Keszler ◽  
Annapoorna Akella ◽  
Kathleen I. Schaffers ◽  
Theodore Alekel

AbstractBy considering selected examples of new structure types, guidelines are set forth for the synthesis of new solid-state inorganic borates that are likely to have desirable properties for nonlinear optical applications. The structures of two new, noncentrosymmetric orthoborate fluorides BaCaBO3F and Ba7(BO3)3F5 demonstrate a feasibility for controlling linear optical properties and for producing noncentrosymmetric borates that melt congruently. The structure of SrLi(B3O5)3 represents an additional example of a noncentrosymmetric borate resulting from chirality of the B3O7 ring. In addition to potential practical value, crystals of the type AMOB2O5 (A = K, Rb, and Cs; M = Nb and Ta) provide a unique means for examining the structural dependent interrelationships of linear and nonlinear optical properties.


2016 ◽  
Vol 7 ◽  
pp. 111-120 ◽  
Author(s):  
Mario Hentschel ◽  
Bernd Metzger ◽  
Bastian Knabe ◽  
Karsten Buse ◽  
Harald Giessen

We study the linear and nonlinear optical properties of hybrid metallic–dielectric plasmonic gap nanoantennas. Using a two-step-aligned electron beam lithography process, we demonstrate the ability to selectively and reproducibly fill the gap region of nanoantennas with dielectric nanoparticles made of lithium niobate (LiNbO3) with high efficiency. The linear optical properties of the antennas are modified due to the large refractive index of the material. This leads to a change in the coupling strength as well as an increase of the effective refractive index of the surrounding. The combination of these two effects causes a red- or blue-shift of the plasmonic modes, respectively. We find that the nonlinear optical properties of the combined system are only modified in the range of one order of magnitude. The observed changes in our experiments in the nonlinear emission can be traced to the changed dielectric environment and thus the modified linear optical properties. The intrinsic nonlinearity of the dielectric used is in fact small when compared to the nonlinearity of the metallic part of the hybrid antennas. Thus, the nonlinear signals generated by the antenna itself are dominant in our experiments. We demonstrate that the well-known nonlinear response of bulk dielectric materials cannot always straightforwardly be used to boost the nonlinear response of nanoscale antenna systems. Our results significantly deepen the understanding of these interesting hybrid systems and offer important guidelines for the design of nanoscale, nonlinear light sources.


1996 ◽  
Vol 438 ◽  
Author(s):  
R. H. Magruder ◽  
R. A. Weeks ◽  
T. S. Anderson ◽  
R. A. Zuhr

AbstractThe linear and nonlinear optical properties of a series of Sb nanometer dimension metal colloids in silica were measured. The colloids were fabricated by the implantation of Sb in silica with nominal doses of 3, 6 and 9x1016 ions/cm2 at 320 keV. The linear optical response was measured from 200 to 900 nm. The nonlinear optical properties were measured using the z-scan technique at wavelengths of 596 and 617 nm. The results are compared to linear and nonlinear properties of a sample implanted with 6x1016 Ag ions/cm 2. Both absorption and the nonlinear index of refraction increase with increasing volume fraction for the Sb implanted samples. The lower linear absorption and comparable nonlinear index of refraction for the Sb colloid-glass composites may be better for devices than composites using metal colloids that have a surface plasmon resonance.


2004 ◽  
Vol 846 ◽  
Author(s):  
Andrew C. Pineda ◽  
Shashi P. Karna

ABSTRACTIn this paper, we present the results of our first-principles quantum mechanical studies of the electronic structure, geometry, and linear and nonlinear optical (NLO) properties of tetrahedral Gam Nm (m=1, 4, 7, 17) atomic clusters. Our calculated results suggest that the linear and NLO properties both exhibit a strong dependence upon cluster size and shape (geometry). However, the size- and the geometry-dependences are more pronounced for the NLO properties than for the linear optical properties. For clusters containing equal numbers of Ga and N atoms, an open-structure with no network-forming ring has a much larger second-order NLO coefficient than a cluster with a closed ring structure.


2009 ◽  
Vol 18 (03) ◽  
pp. 465-470
Author(s):  
XIANGHUA SHEN ◽  
CHENGYOU LIU ◽  
HONG SHEN

Ordered Au nanoparticle arrays were fabricated on fused quartz substrates using nanosphere lithography. Linear and nonlinear optical properties of triangular Au nanoparticle arrays were investigated. Two LSPR peaks due to the surface plasmon resonance of Au particles were observed. The nonlinear optical properties were measured using the Z-scan technique at a wavelength of 532 nm and pulse duration of 10 ns. The nanoparticle arrays exhibit distinct nonlinear absorption saturation behavior, the absorption coefficient was determined to be –3.5 × 103 (cm/GW).


CrystEngComm ◽  
2014 ◽  
Vol 16 (30) ◽  
pp. 6889-6895 ◽  
Author(s):  
Jerald V. Ramaclus ◽  
Tina Thomas ◽  
S. Ramesh ◽  
P. Sagayaraj ◽  
E. A. Michael

The morphology of the DSSS crystal has been modified from bulk parallelepiped to an elongated cuboid shape by changing the supersaturation from high to low. The growth dynamics, defect mechanisms, linear and nonlinear properties are discussed in detail.


2021 ◽  
Vol 129 (5) ◽  
pp. 626
Author(s):  
Hacene Manaa ◽  
Devrim Attila ◽  
Ayse Gul Gurek ◽  
Sughra Mohamed ◽  
Fadheela A. Alawainati ◽  
...  

In this work, the photo-physical properties of seven different phthalocyanine derivatives are studied, with a focus on their transparency spectral range. Two compounds among them are recently synthesised. The investigations include synthesis, photoluminescence, absorptive and refractive nonlinear properties, and optical limiting performances. The compounds are found to be emitting interesting broad fluorescence bands in the visible range. The nonlinear optical properties are investigated with the help of Z-scan technique, with both a continuous laser at 488, 514.5 and 632.8 nm, and with a pulsed laser at 532 nm. The sign and the magnitude of the nonlinear refractive index, third-order susceptibility, and nonlinear absorption coefficient have been evaluated in the seven compounds. The optical limiting performance of each compound was also evaluated in the continuous and pulsed laser excitation regimes. Keywords:


Proceedings ◽  
2018 ◽  
Vol 9 (1) ◽  
pp. 4 ◽  
Author(s):  
Rosa M. F. Batista ◽  
Susana P. G. Costa ◽  
Michael Belsley ◽  
M. Manuela M. Raposo

New push-pull second harmonic generation (SHG) chromophores 2 were synthesized in order to study their linear and nonlinear optical properties. The donor-acceptor π-conjugated systems 2 were prepared in good to excellent yields by a simple aldol-type condensation of the precursor aldehydes 1 with 6-nitro-2-methyl-1,3-benzothiazole in the presence of NaOH. Hyper-Rayleigh scattering in dioxane solutions was used to evaluate their second-order nonlinear optical properties. The experimental results showed that the optical (linear and nonlinear) properties are influenced by the electron-donor strength of the groups of the π-conjugated bridge. The vinyl-benzothiazole derivative 2b, with methoxyl as the donor group, exhibited the largest first hyperpolarizability β (1660 × 10−30 esu, 40 times greater than the standard reference pNA molecule) and the highest decomposition temperature (Td = 360 °C). The good balance between nonlinearity and thermal stability makes this compound a promising candidate as second harmonic generator (SHG) for nonlinear optics.


1990 ◽  
Author(s):  
Tapio T. Rantala ◽  
Mark I. Stockman ◽  
Daniel A. Jelski ◽  
Thomas F. George

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