Beating standard quantum limit via two-axis magnetic susceptibility measurement

We report a metrology scheme which measures magnetic susceptibility of an atomic spin ensemble along the x and z direction and produces parameter estimation with precision beating the standard quantum limit. The atomic ensemble is initialized via one-axis spin squeezing with optimized squeezing time and parameter φ to be estimated is assumed as uniformly distributed between 0 and 2π, while fixed in each estimation. One estimation of φ can be produced with every two magnetic susceptibility data measured along the two axis respectively, which has imprecision scaling (1.43 ± 0.02)/N 0.687±0.003 with respect to the number N of atomic spins. The measurement scheme is easy to implement and is robust against measurement fluctuation caused by environment noise and measurement defects.

Spin-Mechanics with Nitrogen-Vacancy Centers and Trapped Particles

Controlling the motion of macroscopic oscillators in the quantum regime has been the subject of intense research in recent decades. In this direction, opto-mechanical systems, where the motion of micro-objects is strongly coupled with laser light radiation pressure, have had tremendous success. In particular, the motion of levitating objects can be manipulated at the quantum level thanks to their very high isolation from the environment under ultra-low vacuum conditions. To enter the quantum regime, schemes using single long-lived atomic spins, such as the electronic spin of nitrogen-vacancy (NV) centers in diamond, coupled with levitating mechanical oscillators have been proposed. At the single spin level, they offer the formidable prospect of transferring the spins’ inherent quantum nature to the oscillators, with foreseeable far-reaching implications in quantum sensing and tests of quantum mechanics. Adding the spin degrees of freedom to the experimentalists’ toolbox would enable access to a very rich playground at the crossroads between condensed matter and atomic physics. We review recent experimental work in the field of spin-mechanics that employ the interaction between trapped particles and electronic spins in the solid state and discuss the challenges ahead. Our focus is on the theoretical background close to the current experiments, as well as on the experimental limits, that, once overcome, will enable these systems to unleash their full potential.

Free coherent evolution of a coupled atomic spin system initialized by electron scattering

Full insight into the dynamics of a coupled quantum system depends on the ability to follow the effect of a local excitation in real-time. Here, we trace the free coherent evolution of a pair of coupled atomic spins by means of scanning tunneling microscopy. Rather than using microwave pulses, we use a direct-current pump-probe scheme to detect the local magnetization after a current-induced excitation performed on one of the spins. By making use of magnetic interaction with the probe tip, we are able to tune the relative precession of the spins. We show that only if their Larmor frequencies match, the two spins can entangle, causing angular momentum to be swapped back and forth. These results provide insight into the locality of electron spin scattering and set the stage for controlled migration of a quantum state through an extended spin lattice.

Readout and control of an endofullerene electronic spin

Atomic spins for quantum technologies need to be individually addressed and positioned with nanoscale precision. C60 fullerene cages offer a robust packaging for atomic spins, while allowing in-situ physical positioning at the nanoscale. However, achieving single-spin level readout and control of endofullerenes has so far remained elusive. In this work, we demonstrate electron paramagnetic resonance on an encapsulated nitrogen spin (14N@C60) within a C60 matrix using a single near-surface nitrogen vacancy (NV) center in diamond at 4.7 K. Exploiting the strong magnetic dipolar interaction between the NV and endofullerene electronic spins, we demonstrate radio-frequency pulse controlled Rabi oscillations and measure spin-echos on an encapsulated spin. Modeling the results using second-order perturbation theory reveals an enhanced hyperfine interaction and zero-field splitting, possibly caused by surface adsorption on diamond. These results demonstrate the first step towards controlling single endofullerenes, and possibly building large-scale endofullerene quantum machines, which can be scaled using standard positioning or self-assembly methods.

Coherently forming a single molecule in an optical trap

Ultracold single molecules have wide-ranging potential applications, such as ultracold chemistry, precision measurements, quantum simulation, and quantum computation. However, given the difficulty of achieving full control of a complex atom-molecule system, the coherent formation of single molecules remains a challenge. Here, we report an alternative route to coherently bind two atoms into a weakly bound molecule at megahertz levels by coupling atomic spins to their two-body relative motion in a strongly focused laser with inherent polarization gradients. The coherent nature is demonstrated by long-lived atom-molecule Rabi oscillations. We further manipulate the motional levels of the molecules and measure the binding energy precisely. This work opens the door to full control of all degrees of freedom in atom-molecule systems.

Light-mediated strong coupling between a mechanical oscillator and atomic spins 1 meter apart

Engineering strong interactions between quantum systems is essential for many phenomena of quantum physics and technology. Typically, strong coupling relies on short-range forces or on placing the systems in high-quality electromagnetic resonators, which restricts the range of the coupling to small distances. We used a free-space laser beam to strongly couple a collective atomic spin and a micromechanical membrane over a distance of 1 meter in a room-temperature environment. The coupling is highly tunable and allows the observation of normal-mode splitting, coherent energy exchange oscillations, two-mode thermal noise squeezing, and dissipative coupling. Our approach to engineering coherent long-distance interactions with light makes it possible to couple very different systems in a modular way, opening up a range of opportunities for quantum control and coherent feedback networks.