The role of resonance radiation in the propagation of a positive pre-breakdown ionization wave in long discharge tubes

The work is devoted to calculating the flux of resonance photons towards the boundary of a cylindrical discharge tube of a finite size during the propagation of a pre-breakdown ionization wave of positive polarity. A cylindrical discharge tube of finite dimensions with argon at the pressure of p=1 Torr is considered. The propagation mechanisms of metastable and resonance atoms are compared. For the considered discharge conditions, the space-time distributions of metastable and resonance atoms are calculated. The manuscript presents a technique for calculating the flux of resonance photons onto the discharge tube wall with the account of the radiation trapping. It is shown that for the studied conditions the photon flux density towards the longitudinal boundary of the tube ahead of the ionization wave can reach 1013 cm-2s-1. The obtained results allow describing the appearance of seed electrons ahead of the positive ionization wavefront during its propagation due to the electron photoemission from the discharge tube wall.

Influence of radiation transport on discharge characteristics of an atmospheric pressure plasma jet in Argon

In the current work the method of radiation trapping treatment infinite coaxial cylinders using spherical coordinates is introduced. The operator of resonant transition process is obtained explicitly in the matrix form and its response to delta-function is analyzed in both hollow and solid cylinders. The influence of radiation trapping effect is shown on the example of model of miniaturized non-thermal atmospheric pressure plasma jet. The results of the calculations with the developed matrix method are compared to those based on the effective probability approximation. It is shown that the use of matrix method leads to significant spatial redistribution of the excited plasma species due to the non-local effects of radiation transport mechanism.

1.5 μm photoluminescence and upconversion photoluminescence in GeGaAsS:Er chalcogenide glass

The paper reports on ≈1.5 μm Stokes photoluminescence (PL) emission and upconversion photoluminescence (UCPL) emission in the visible and near-infrared spectral region in Er3+-doped Ge25Ga8As2S65 chalcogenide glasses at pumping wavelengths of 980 and 1550 nm. The ≈1.5 μm PL emission spectra are broadened with increasing concentration of Er ions which is discussed in terms of radiation trapping and UCPL dynamics affecting the Er3+: 4I13/2 level lifetime. The UCPL emission was observed at ≈530, ≈550, ≈660, ≈810 and ≈990 nm and its overall intensity as well as red-to-green UCPL emission intensity ratio increases with increasing Er concentration. To explore the UCPL dynamics we measured double logarithmic dependency of green (≈550 nm) and red (≈660 nm) UCPL emission versus pump power at pumping wavelength of 975 nm. Moreover, we measured quadrature frequency resolved spectroscopy (QFRS) on green UCPL emission (≈550 nm) using 975 nm pumping wavelength and various excitation powers. The QFRS spectra on green UCPL were analyzed in term of QFRS transfer function for three-level model from which we deduced energy transfer upconversion rate w11 (s−1) originating from Er3+: 4I11/2, 4I11/2→4F7/2, 4I15/2 transitions.