Evaluation of BRDF Information Retrieved from Time-Series Multiangle Data of the Himawari-8 AHI

Recently, much attention has been given to using geostationary Earth orbit (GEO) meteorological satellite data for retrieving land surface parameters due to their high observation frequencies. However, their bidirectional reflectance distribution function (BRDF) information content with a single viewing angle has not been sufficiently investigated, which lays a foundation for subsequent quantitative estimation. In this study, we aim to comprehensively evaluate BRDF information from time-series observations from the Advanced Himawari Imager (AHI) onboard the GEO satellite Himawari-8. First, ~6.2 km monthly multiangle surface reflectances from POLDER onboard a low-Earth-orbiting (LEO) satellite with good angle distributions over various land types during 2008 were used as reference data, and corresponding 0.05° high-quality MODIS (i.e., onboard LEO satellites) and AHI datasets during four months in 2020 were obtained using cloud and aerosol property products. Then, indicators of angle distribution, BRDF change, and albedos were retrieved by the kernel-driven Ross-Li BRDF model from the three datasets, which were used for comparisons over different time spans. Generally, the quality of sun-viewing geometries varies dramatically for accumulated AHI observations according to the weight-of-determination, and wide-ranging anisotropic flat indices are obtained. The root-mean-square-errors of white sky albedos between AHI and MODIS half-month data are 0.018 and 0.033 in the red and near-infrared bands, respectively, achieving smaller values of 0.004 and 0.007 between the half-month and daily AHI data, respectively, due to small variances in sun-viewing geometries. The generally wide AHI BRDF variances and good consistency in albedo with MODIS show their potential for retrieving anisotropy information and albedo, while angle accumulation quality of AHI time-series observations must be considered.

Empirically derived parameterizations of the direct aerosol radiative effect based on ORACLES aircraft observations

In this paper, we use observations from the NASA ORACLES (ObseRvations of CLouds above Aerosols and their intEractionS) aircraft campaign to develop a framework by way of two parameterizations that establishes regionally representative relationships between aerosol-cloud properties and their radiative effects. These relationships rely on new spectral aerosol property retrievals of the single scattering albedo (SSA) and asymmetry parameter (ASY). The retrievals capture the natural variability of the study region as sampled, and both were found to be fairly narrowly constrained (SSA: 0.83 ± 0.03 in the mid-visible, 532 nm; ASY: 0.54 ± 0.06 at 532 nm). The spectral retrievals are well suited for calculating the direct aerosol radiative effect (DARE) since SSA and ASY are tied directly to the irradiance measured in the presence of aerosols – one of the inputs to the spectral DARE. The framework allows for entire campaigns to be generalized into a set of parameterizations. For a range of solar zenith angles, it links the broadband DARE to the mid-visible aerosol optical depth (AOD) and the albedo (α) of the underlying scene (either clouds or clear sky) by way of the first parameterization: P(AOD, α). For ORACLES, the majority of the case-to-case variability of the broadband DARE is attributable to the dependence on the two driving parameters of P(AOD, α). A second, extended, parameterization PX(AOD, α, SSA) explains even more of the case-to-case variability by introducing the mid-visible SSA as a third parameter. These parameterizations establish a direct link from two or three mid-visible (narrowband) parameters to the broadband DARE, implicitly accounting for the underlying spectral dependencies of its drivers. They circumvent some of the assumptions when calculating DARE from satellite products or in a modeling context. For example, the DARE dependence on aerosol microphysical properties is not explicit in P or PX because the asymmetry parameter varies too little from case to case to translate into appreciable DARE variability. While these particular DARE parameterizations only represent the ORACLES data, they raise the prospect of generalizing the framework to other regions.

Technical note: Comparison and interconversion of pH based on different standard states for aerosol acidity characterization

Aerosol pH is often calculated based on different standard states thus making it inappropriate to compare aerosol acidity parameters derived thereby. Such comparisons are however routinely performed in the atmospheric science community. This study attempts to address this issue for the first time by providing a theoretical framework to compare and convert between aerosol pH values calculated based on molarity, molality and mole fractions. Using hourly ionic species measurements in Guangzhou, China, it is observed that pHx (mole fraction based) is always 1.74 pH unit higher than pHm (molality based) and follow the same trend, regardless of aerosol property. The difference between pHx and pHc (molarity based), on the other hand, ranges from 1.74 to 1.89 depending on the density of hygroscopic aerosol. It is observed that application of this pH standardization protocol can significantly influence conclusions on aerosol acidity reported by past studies and is thus highly recommended.

SAM-CAAM: A Concept for Acquiring Systematic Aircraft Measurements to Characterize Aerosol Air Masses

A modest operational program of systematic aircraft measurements can resolve key satellite aerosol data record limitations. Satellite observations provide frequent global aerosol amount maps but offer only loose aerosol property constraints needed for climate and air quality applications. We define and illustrate the feasibility of flying an aircraft payload to measure key aerosol optical, microphysical, and chemical properties in situ. The flight program could characterize major aerosol airmass types statistically, at a level of detail unobtainable from space. It would 1) enhance satellite aerosol retrieval products with better climatology assumptions and 2) improve translation between satellite-retrieved optical properties and species-specific aerosol mass and size simulated in climate models to assess aerosol forcing, its anthropogenic components, and other environmental impacts. As such, Systematic Aircraft Measurements to Characterize Aerosol Air Masses (SAM-CAAM) could add value to data records representing several decades of aerosol observations from space; improve aerosol constraints on climate modeling; help interrelate remote sensing, in situ, and modeling aerosol-type definitions; and contribute to future satellite aerosol missions. Fifteen required variables are identified and four payload options of increasing ambition are defined to constrain these quantities. “Option C” could meet all the SAM-CAAM objectives with about 20 instruments, most of which have flown before, but never routinely several times per week, and never as a group. Aircraft integration and approaches to data handling, payload support, and logistical considerations for a long-term, operational mission are discussed. SAM-CAAM is feasible because, for most aerosol sources and specified seasons, particle properties tend to be repeatable, even if aerosol loading varies.