Iodine release from high-burnup fuel structures: Separate-effect tests and simulated fuel pellets for better understanding of iodine behaviour in nuclear fuels

Iodine release modelling of nuclear fuel pellets has major uncertainties that restrict applications in current fuel performance codes. The uncertainties origin from both the chemical behaviour of iodine in the fuel pellet and the release of different chemical species. The structure of nuclear fuel pellet evolves due to neutron and fission product irradiation, thermo-mechanical loads and fission product chemical interactions. This causes extra challenges for the fuel behaviour modelling. After sufficient amount of irradiation, a new type of structure starts forming at the cylindrical pellet outer edge. The porous structure is called high-burnup structure or rim structure. The effects of high-burnup structure on fuel behaviour become more pronounced with increasing burnup. As the phenomena in the nuclear fuel pellet are diverse, experiments with simulated fuel pellets can help in understanding and limiting the problem at hand. As fission gas or iodine release behaviour from high-burnup structure is not fully understood, the current preliminary study focuses on (i) sintering of porous fuel samples with Cs and I, (ii) measurements of released species during the annealing experiments and (iii) interpretation of the iodine release results with the scope of current fission gas release models. Graphical abstract

Simplified Model of a High Burnup Spent Nuclear Fuel Rod under Lateral Impact Considering a Stress-Based Failure Criterion

The inventory of spent nuclear fuel (SNF) generated in nuclear power plants is continuously increasing, and it is very important to maintain the structural integrity of SNF for economical and efficient management. The cladding surrounding nuclear fuel must be protected from physical and mechanical deterioration, which causes fuel rod breakage. In this study, the material properties of the simplified beam model of a SNF rod were calibrated for a drop accident evaluation by considering the pellet–clad interaction (PCI) of the high burnup fuel rod. In a horizontal drop, which is the most damaging during a drop accident of SNF, the stress in the cladding caused by the inertia action of the pellets has a great effect on the integrity of the fuel rod. The failure criterion for SNF was selected as the membrane plus bending stress through stress linearization in the cross-sections through the thickness of the cladding. Because the stress concentration in the cladding around the vicinity of the pellet–pellet interface cannot be simulated in a simplified beam model, a stress correction factor is derived through a comparison of the simplified model and detailed model. The applicability of the developed simplified model is checked through dynamic impact simulations. The developed model can be used in cask level analyses and is expected to be usefully utilized to evaluate the structural integrity of SNF under transport and in storage conditions.