Thallium based heavy inorganic scintillators: Recent developments and future perspective

The current development status and future perspective of Tl-based inorganic scintillators are the subjects of this highlights. Thallium (Tl) ion is known to have very efficient luminescence in the widely...

Gamma-ray Spectroscopy Using Inorganic Scintillator Coated with Reduced Graphene Oxide in Fiber-Optic Radiation Sensor

In this study, we developed a remote gamma-ray spectroscopy system based on a fiber-optic radiation sensor (FORS) that is composed of an inorganic scintillator coated with reduced graphene oxide (RGO) and a plastic optical fiber (POF). As a preliminary experiment, we measured the transmitted light intensities using RGO membranes of different thicknesses with different wavelengths of emitted light. To evaluate the FORS performance, we determined the optimal thickness of the RGO membrane and measured the amounts of scintillating light and gamma energy spectra using radioactive isotopes such as 60Co and 137Cs. The amounts of scintillating light from the RGO-coated inorganic scintillators increased, and the energy resolutions of the gamma-ray spectra were enhanced. In addition, the gamma-ray energy spectra were measured using different types of RGO-coated inorganic scintillators depending on the lengths of the POFs for remote gamma-ray spectroscopy. It was expected that inorganic scintillators coated with RGO in FORS can deliver improved performance, such as increments of scintillating light and energy resolution in gamma-ray spectroscopy, and they can be used to identify nuclides remotely in various nuclear facilities.

The Future Role of Inorganic Crystal Scintillators in Dark Matter Investigations

Crystal scintillators and in particular inorganic scintillators play an important role in the investigation of Dark Matter (DM) and other rare processes. The investigation of a DM signature, as the annual modulation, or the directionality technique requires the use of highly radiopure detectors able to explore the very low energy region maintaining a high stability of the running conditions. In this paper, the cases of NaI(Tl), ZnWO4 and SrI2(Eu) crystal scintillators are described in the framework of our activities at the Gran Sasso National Laboratory of the INFN. Their role, the obtained results in DM investigation, as well as their potential and perspectives for the future are reviewed.

Light Extraction Enhancement Techniques for Inorganic Scintillators

Scintillators play a key role in the detection chain of several applications which rely on the use of ionizing radiation, and it is often mandatory to extract and detect the generated scintillation light as efficiently as possible. Typical inorganic scintillators do however feature a high index of refraction, which impacts light extraction efficiency in a negative way. Furthermore, several applications such as preclinical Positron Emission Tomography (PET) rely on pixelated scintillators with small pitch. In this case, applying reflectors on the crystal pixel surface, as done conventionally, can have a dramatic impact of the packing fraction and thus the overall system sensitivity. This paper presents a study on light extraction techniques, as well as combinations thereof, for two of the most used inorganic scintillators (LYSO and BGO). Novel approaches, employing Distributed Bragg Reflectors (DBRs), metal coatings, and a modified Photonic Crystal (PhC) structure, are described in detail and compared with commonly used techniques. The nanostructure of the PhC is surrounded by a hybrid organic/inorganic silica sol-gel buffer layer which ensures robustness while maintaining its performance unchanged. We observed in particular a maximum light gain of about 41% on light extraction and 21% on energy resolution for BGO, a scintillator which has gained interest in the recent past due to its prompt Cherenkov component and lower cost.

Light Extraction Enhancement Techniques for Inorganic Scintillators

Scintillators play a key role in the detection chain of several applications which rely on the use of ionizing radiation, and it is often mandatory to extract and detect the generated scintillation light as efficiently as possible. In positron emission tomography (PET), for example, both energy resolution and coincidence resolving time, two of the key detection parameters, depend strongly on the total amount of light which reaches the photodetector surface as well as its spatial and temporal distribution. Typical inorganic scintillators do however feature a high index of refraction, which impacts light extraction efficiency in a negative way. Furthermore, several applications such as preclinical PET rely on pixelated scintillators with small pitch. In this case, applying reflectors on the crystal pixel surface, as done conventionally, can have a dramatic impact of the packing fraction and thus the overall system sensitivity. This paper presents a study on light extraction techniques, as well as combinations thereof, for two of the most used inorganic scintillators (LYSO and BGO). Novel approaches, employing distributed Bragg reflectors (DBRs), metal coatings, and a modified Photonic Crystal (PhC) structure, are described in detail and compared with commonly used techniques. The nanostructure of the PhC is surrounded by a hybrid organic/inorganic silica sol-gel buffer layer which ensures robustness while maintaining its performance unchanged. We observed in particular a maximum light gain of about 41% on light extraction and 21% on energy resolution for BGO, a scintillator which has gained interest in the recent past due to its prompt Cherenkov component and lower cost.

Scintillation materials based on metal iodates by rare earth doping modifications for use in radioluminescence and X-ray imaging

Scintillators, which can emit visible photons under γ- or X-ray excitation, are widely used in radiation detection. Traditional inorganic scintillators usually bring with some drawbacks, such as hygroscopicity or a...