scholarly journals Effects of Using Two Different Biogenic Emission Models on Ozone and Particles in Europe

Author(s):  
Jianhui Jiang ◽  
Sebnem Aksoyoglu ◽  
Giancarlo Ciarelli ◽  
Emmanouil Oikonomakis ◽  
André S. H. Prévôt
2012 ◽  
Vol 12 (16) ◽  
pp. 7399-7412 ◽  
Author(s):  
A. Zare ◽  
J. H. Christensen ◽  
P. Irannejad ◽  
J. Brandt

Abstract. Knowledge about isoprene emissions and concentration distribution is important for chemistry transport models (CTMs), because isoprene acts as a precursor for tropospheric ozone and subsequently affects the atmospheric concentrations of many other atmospheric compounds. Isoprene has a short lifetime, and hence it is very difficult to evaluate its emission estimates against measurements. For this reason, we coupled two isoprene emission models with the Danish Eulerian Hemispheric Model (DEHM), and evaluated the simulated background ozone concentrations based on different models for isoprene emissions. In this research, results of using the two global biogenic emission models; GEIA (Global Emissions Inventory Activity) and MEGAN (the global Model of Emissions of Gases and Aerosols from Nature) are compared and evaluated. The total annual emissions of isoprene for the year 2006 estimated by using MEGAN is 592 Tg yr−1 for an extended area of the Northern Hemisphere, which is 21% higher than that estimated by using GEIA. The overall feature of the emissions from the two models is quite similar, but differences are found mainly in Africa's savannah and in the southern part of North America. Differences in spatial distribution of emission factors are found to be a key source of these discrepancies. In spite of the short life-time of isoprene, a direct evaluation of isoprene concentrations using the two biogenic emission models in DEHM has been made against available measurements in Europe. Results show an agreement between two models simulations and the measurements in general and that the CTM is able to simulate isoprene concentrations. Additionally, investigation of ozone concentrations resulting from the two biogenic emission models show that isoprene simulated by MEGAN strongly affects the ozone production in the African savannah; the effect is up to 10% more than that obtained using GEIA. In contrast, the impact of using GEIA is higher in the Amazon region with more than 8% higher ozone concentrations compared to that of using MEGAN. Comparing the ozone concentrations obtained by DEHM using the two different isoprene models with measurements from Europe and North America, show an agreement on the hourly, mean daily and daily maximum values. However, the average of ozone daily maximum value simulated by using MEGAN is slightly closer to the measured value for the average of all measuring sites in Europe.


1997 ◽  
Vol 12 (1) ◽  
pp. 71-77
Author(s):  
John A. Brockhaus ◽  
Jayantha Ediriwickrema ◽  
Heather Cheshire ◽  
Siamak Khorram

2018 ◽  
Author(s):  
Jianhui Jiang ◽  
Sebnem Aksoyoglu ◽  
Giancarlo Ciarelli ◽  
Emmanouil Oikonomakis ◽  
Imad El-Haddad ◽  
...  

2012 ◽  
Vol 12 (4) ◽  
pp. 9247-9281 ◽  
Author(s):  
A. Zare ◽  
J. Brandt ◽  
J. H. Christensen ◽  
P. Irannejad

Abstract. Knowledge about isoprene emissions and concentration distribution is important for chemistry transport models (CTMs), because isoprene acts as a precursor for tropospheric ozone and subsequently affects the atmospheric concentrations of many other atmospheric compounds. Isoprene has a short lifetime, and hence it is very difficult to evaluate its emission estimates against measurements. For this reason, we coupled two isoprene emission models with the Danish Eulerian Hemispheric Model (DEHM), and evaluated the simulated background ozone concentrations based on different models for isoprene emissions. In this research, results of using the two global biogenic emission models; GEIA (Global Emissions Inventory Activity) and MEGAN (the global Model of Emissions of Gases and Aerosols from Nature) are compared and evaluated. The total annual emissions of isoprene for the year 2006 estimated by using MEGAN is 732 Tg yr−1 for an extended area of the Northern Hemisphere, which is 50% higher than that estimated by using GEIA. The overall feature of the emissions from the two models are quite similar, but significant differences are found mainly in Africa's savannah and the rain forests of South America, and in some subtropical regions, such as the Middle East, India and the southern part of North America. Differences in spatial distribution of emission factors are found to be a key source of these discrepancies. In spite of the short life-time of isoprene, a direct evaluation of isoprene concentrations using the two biogenic emission models has been made against available measurements in Europe. Results show that the two models in general represent the measurements well and that the CTM is able to simulate isoprene concentrations. Additionally, investigation of ozone concentrations resulting from the two biogenic emission models show that isoprene simulated by MEGAN strongly affects the ozone production in the African savannah; the effect is up to 20% more than that obtained using GEIA. In contrast, the impact of using GEIA is higher in the Amazon region with more than 15% higher ozone concentrations compared to that of using MEGAN. Comparing the results for ozone concentrations for Europe obtained by using the two different models with measurements, show that the MEGAN emission model improves the model performance significantly in the Mediterranean area.


2019 ◽  
Vol 19 (17) ◽  
pp. 11199-11212 ◽  
Author(s):  
Ana Stojiljkovic ◽  
Mari Kauhaniemi ◽  
Jaakko Kukkonen ◽  
Kaarle Kupiainen ◽  
Ari Karppinen ◽  
...  

Abstract. We have numerically evaluated how effective selected potential measures would be for reducing the impact of road dust on ambient air particulate matter (PM10). The selected measures included a reduction of the use of studded tyres on light-duty vehicles and a reduction of the use of salt or sand for traction control. We have evaluated these measures for a street canyon located in central Helsinki for four years (2007–2009 and 2014). Air quality measurements were conducted in the street canyon for two years, 2009 and 2014. Two road dust emission models, NORTRIP (NOn-exhaust Road TRaffic Induced Particle emissions) and FORE (Forecasting Of Road dust Emissions), were applied in combination with the Operational Street Pollution Model (OSPM), a street canyon dispersion model, to compute the street increments of PM10 (i.e. the fraction of PM10 concentration originating from traffic emissions at the street level) within the street canyon. The predicted concentrations were compared with the air quality measurements. Both road dust emission models reproduced the seasonal variability of the PM10 concentrations fairly well but under-predicted the annual mean values. It was found that the largest reductions of concentrations could potentially be achieved by reducing the fraction of vehicles that use studded tyres. For instance, a 30 % decrease in the number of vehicles using studded tyres would result in an average decrease in the non-exhaust street increment of PM10 from 10 % to 22 %, depending on the model used and the year considered. Modelled contributions of traction sand and salt to the annual mean non-exhaust street increment of PM10 ranged from 4 % to 20 % for the traction sand and from 0.1 % to 4 % for the traction salt. The results presented here can be used to support the development of optimal strategies for reducing high springtime particulate matter concentrations originating from road dust.


2020 ◽  
Vol 501 (1) ◽  
pp. 337-346
Author(s):  
E Mestre ◽  
E de Oña Wilhelmi ◽  
D Khangulyan ◽  
R Zanin ◽  
F Acero ◽  
...  

ABSTRACT Since 2009, several rapid and bright flares have been observed at high energies (>100 MeV) from the direction of the Crab nebula. Several hypotheses have been put forward to explain this phenomenon, but the origin is still unclear. The detection of counterparts at higher energies with the next generation of Cherenkov telescopes will be determinant to constrain the underlying emission mechanisms. We aim at studying the capability of the Cherenkov Telescope Array (CTA) to explore the physics behind the flares, by performing simulations of the Crab nebula spectral energy distribution, both in flaring and steady state, for different parameters related to the physical conditions in the nebula. In particular, we explore the data recorded by Fermi during two particular flares that occurred in 2011 and 2013. The expected GeV and TeV gamma-ray emission is derived using different radiation models. The resulting emission is convoluted with the CTA response and tested for detection, obtaining an exclusion region for the space of parameters that rule the different flare emission models. Our simulations show different scenarios that may be favourable for achieving the detection of the flares in Crab with CTA, in different regimes of energy. In particular, we find that observations with low sub-100 GeV energy threshold telescopes could provide the most model-constraining results.


Author(s):  
Maren Schnieder ◽  
Chris Hinde ◽  
Andrew West

Global concerns about the environmental effects (e.g., pollution, land use, noise) of last-mile deliveries are increasing. Parcel lockers are seen as an option to reduce these external effects of last-mile deliveries. The contributions of this paper are threefold: firstly, the research studies simulating the emissions caused by parcel delivery to lockers are summarized. Secondly, a demand model for parcel deliveries in New York City (NYC) is created for 365 days and delivery trips to lockers and homes are optimized for 20 “real-world” scenarios. Thirdly, using the emission factors included in the HandBook Emission Factors for Road Transport (HBEFA) database, the maximum percentage of customers who could pick up a parcel by car from parcel lockers that would result in fewer total emissions (driving customers + walking customers) than if home deliveries were adopted is calculated for various pollutants and scenario assumptions (i.e., street types, temperature, parking duration, level of service and vehicle drivetrain). This paper highlights how small changes in the calibration can significantly change the results and therefore using average values for emission factors or only considering one pollutant like most studies may not be appropriate.


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