Ultrafast Relaxation of Localized Excitations in Solids

1988 ◽  
pp. 269-273
Author(s):  
Y. Kayanuma
Keyword(s):  
Ultrafast Relaxation ◽  
Localized Excitations

Double-Excitation Dynamics in m-LPPP probed with sub-20 fs Time Resolution

2003 ◽  
Vol 771 ◽  
Author(s):  
C. Gadermaier ◽  
G. Cerullo ◽  
C. Manzoni ◽  
U. Scherf ◽  
E.J.W. List ◽  
...  
Keyword(s):  
Vibrational Relaxation ◽  
Broad Band ◽  
Generation Efficiency ◽  
Exciton Dissociation ◽  
Charge Generation ◽  
Carrier Generation ◽  
Dissociation Probability ◽  
Ultrafast Relaxation ◽  
First Excited State ◽  
Differential Transmission

AbstractIn a novel modification of transient differential transmission spectroscopy, the first excited state S1 is reexcited via a second laser pulse towards a higher lying state Sn. The dynamics of the relaxation of this state Sn as well as the states created from Sn are revealed by a broad-band probe pulse.We find that the charge carrier generation efficiency from Sn is higher compared to S1. The push and probe durations below 20 fs enable the temporal resolution of the ultrafast relaxation of the Sn state and enables us to identify the two main contributions to enhanced charge generation from Sn, energy migration towards sites of high dissociation probability, and exciton dissociation during vibrational relaxation.

The effect of hydrogen bonds on the ultrafast relaxation dynamics of a BODIPY dimer

2021 ◽  
Vol 154 (8) ◽  
pp. 084201
Author(s):  
Elisa Fresch ◽  
Nicola Peruffo ◽  
Mariachiara Trapani ◽  
Massimiliano Cordaro ◽  
Giovanni Bella ◽  
...  
Keyword(s):  
Hydrogen Bonds ◽  
Relaxation Dynamics ◽  
Ultrafast Relaxation

scholarly journals Vibrational resonant inelastic X-ray scattering in liquid acetic acid: a ruler for molecular chain lengths

2021 ◽  
Vol 11 (1) ◽  
Author(s):  
Viktoriia Savchenko ◽  
Iulia Emilia Brumboiu ◽  
Victor Kimberg ◽  
Michael Odelius ◽  
Pavel Krasnov ◽  
...  
Keyword(s):  
Molecular Structure ◽  
Acetic Acid ◽  
Molecular Chain ◽  
X Ray ◽  
X Ray Scattering ◽  
Localized Excitations ◽  
Vibrational Excitations ◽  
Chain Lengths ◽  
X Ray Absorption ◽  
Ray Scattering

AbstractQuenching of vibrational excitations in resonant inelastic X-ray scattering (RIXS) spectra of liquid acetic acid is observed. At the oxygen core resonance associated with localized excitations at the O–H bond, the spectra lack the typical progression of vibrational excitations observed in RIXS spectra of comparable systems. We interpret this phenomenon as due to strong rehybridization of the unoccupied molecular orbitals as a result of hydrogen bonding, which however cannot be observed in x-ray absorption but only by means of RIXS. This allows us to address the molecular structure of the liquid, and to determine a lower limit for the average molecular chain length.

Virasoro structure and localized excitations of the LKR system

2003 ◽  
Vol 44 (12) ◽  
pp. 5869 ◽  
Author(s):  
S. Y. Lou ◽  
C. Rogers ◽  
W. K. Schief
Keyword(s):  
Localized Excitations

Ultrafast relaxation of the fundamental vibrations of SH- and OH- in potassium halides

1994 ◽  
Vol 58 (1-6) ◽  
pp. 33-36 ◽  
Author(s):  
C.E. Mungan ◽  
U. Happek ◽  
A.J. Sievers
Keyword(s):  
Ultrafast Relaxation ◽  
Potassium Halides
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