Modelling the Interaction Between the Atmospheric Boundary Layer and Evaporating Sea Spray Droplets

Abstract The effects of large eddies (LE) on the marine boundary layer (MBL) microphysics and thermodynamics is investigated using a 2D Lagrangian model with spectral bin microphysics including effects of sea spray. The 600 m × 400 m MBL computational area is covered by 3750 adjacent interacting Lagrangian parcels moving in a turbulent-like flow. A turbulent-like velocity field is designed as a sum of a high number of harmonics with random time-dependent amplitudes and different wavelengths including large eddies with scales of several hundred meters. The model explicitly calculates diffusion growth/evaporation, collisions, and sedimentation of droplets forming both as sea spray droplets and background aerosols, as well as aerosol masses within droplets. The turbulent mixing between parcels is explicitly taken into account. Sea spray generation is determined by a source function depending on the background wind speed assumed in the simulations to be equal to 20 m s−1. The results of simulations obtained by taking into account the effects of LE are compared to those obtained under the assumption that the vertical transport of droplets and passive scalars is caused by small-scale turbulent diffusion. Small-scale turbulence diffusion taken alone leads to an unrealistic MBL structure. Nonlocal mixing of the MBL caused by LE leads to the formation of a well-mixed MBL with a vertical structure close to the observed one. LE lead to an increase in the sensible and latent heat surface fluxes by 50%–100% and transport a significant amount of large spray droplets upward. Microphysical processes lead to formation of spray-induced drizzling clouds with cloud base near the 200-m level.

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A numerical framework for simulating episodic emissions of high-temperature marine INPs

10.5194/acp-2021-316 ◽

2021 ◽

Author(s):

Isabelle Steinke ◽

Paul J. DeMott ◽

Grant Deane ◽

Thomas C. J. Hill ◽

Mathew Maltrud ◽

...

Keyword(s):

Boundary Layer ◽

High Temperature ◽

Atmospheric Boundary Layer ◽

Heterotrophic Bacteria ◽

Sea Spray ◽

Surface Microlayer ◽

Partial Explanation ◽

Sea Surface Microlayer ◽

Sea Spray Aerosol ◽

Field Campaigns

Abstract. We present a framework for estimating concentrations of episodically elevated high-temperature marine ice nucleating particles (INPs) in the sea surface microlayer and their subsequent emission into the atmospheric boundary layer. These episodic INPs have been observed in multiple ship-based and coastal field campaigns, but the processes controlling their ocean concentrations and transfer to the atmosphere are not yet fully understood. We use a combination of empirical constraints and simulation outputs from an Earth System Model to explore different hypotheses for explaining the variability of INP concentrations, and the occurrence of episodic INPs, in the marine atmosphere. In our calculations, we examine two proposed oceanic sources of high-temperature INPs: heterotrophic bacteria and marine biopolymer aggregates (MBPAs). Furthermore, we assume that the emission of these INPs is determined by the production of supermicron sea spray aerosol formed from jet drops, with an entrainment probability that is described by Poisson statistics. The concentration of jet drops is derived from the number concentration of supermicron sea spray aerosol calculated from model runs. We then derive the resulting number concentrations of marine high-temperature INPs (≥ 253 K) in the atmospheric boundary layer and compare their variability to atmospheric observations of INP variability. Specifically, we compare against concentrations of episodically occurring high-temperature INPs observed during field campaigns in the Southern Ocean, the Equatorial Pacific, and the North Atlantic. We find that heterotrophic bacteria and MBPAs acting as INPs provide only a partial explanation for the observed high INP concentrations. We note, however, that there are still substantial knowledge gaps, particularly concerning the identity of the oceanic INPs contributing most frequently to episodic high-temperature INPs, their specific ice nucleation activity, and the enrichment of their concentrations during the sea-air transfer process. Therefore, targeted measurements investigating the composition of these marine INPs as well as drivers for their emission are needed, ideally in combination with modeling studies focused on the potential cloud impacts of these high-temperature INPs.

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Evidence of Sea-State Dependence of Aerosol Concentration in the Marine Atmospheric Boundary Layer

Journal of Physical Oceanography ◽

10.1175/jpo-d-16-0058.1 ◽

2017 ◽

Vol 47 (1) ◽

pp. 69-84 ◽

Cited By ~ 9

Author(s):

Luc Lenain ◽

W. Kendall Melville

Keyword(s):

Boundary Layer ◽

Atmospheric Boundary Layer ◽

Wave Breaking ◽

State Dependence ◽

Aerosol Concentration ◽

Sea Spray ◽

Marine Atmospheric Boundary Layer ◽

Sea State ◽

Wave Parameters ◽

Interaction Experiment

AbstractSea spray aerosols represent a large fraction of the aerosols present in the maritime environment. Despite evidence of the importance of surface wave– and wave breaking–related processes in coupling the ocean with the atmosphere, sea spray source generation functions are traditionally parameterized by the 10-m wind speed U10 alone. It is clear that unless the wind and wave field are fully developed, the source function will be a function of both wind and wave parameters. This study reports primarily on the aerosol component of an air–sea interaction experiment, the phased-resolved High-Resolution Air–Sea Interaction Experiment (HIRES), conducted off the coast of northern California in June 2010. Detailed measurements of aerosol number concentration in the marine atmospheric boundary layer (MABL) at altitudes ranging from as low as 30 m up to 800 m above mean sea level (MSL) over a broad range of environmental conditions (significant wave height Hs of 2 to 4.5 m and U10 from 10 to 18 m s−1) collected from an instrumented research aircraft are presented. Aerosol number densities and volume are computed over a range of particle diameters from 0.1 to 200 μm, while the sea surface conditions, including Hs, moments of the breaker length distribution Λ(c), and wave breaking dissipation, were measured by a suite of electro-optical sensors that included the NASA Airborne Topographic Mapper (ATM). The sea-state dependence of the aerosol concentration in the MABL is evident, stressing the need to incorporate wave parameters in the spray source generation functions that are traditionally parameterized by surface winds alone.

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