scholarly journals Dual-wavelength linear depolarization ratio of volcanic aerosols: Lidar measurements of the Eyjafjallajökull plume over Maisach, Germany

2012 ◽  
Vol 48 ◽  
pp. 85-96 ◽  
Author(s):  
Silke Groß ◽  
Volker Freudenthaler ◽  
Matthias Wiegner ◽  
Josef Gasteiger ◽  
Alexander Geiß ◽  
...  
Keyword(s):  
Dual Wavelength ◽  
Depolarization Ratio ◽  
Lidar Measurements ◽  
Volcanic Aerosols ◽  
Linear Depolarization Ratio

scholarly journals Benefit of depolarization ratio at λ = 1064 nm for the retrieval of the aerosol microphysics from lidar measurements

2014 ◽  
Vol 7 (11) ◽  
pp. 3773-3781 ◽  
Author(s):  
J. Gasteiger ◽  
V. Freudenthaler
Keyword(s):  
Optical Properties ◽  
Mass Concentration ◽  
Volcanic Ash ◽  
Single Scattering ◽  
Depolarization Ratio ◽  
Complex Relation ◽  
Microphysical Properties ◽  
Lidar Measurements ◽  
Increased Sensitivity ◽  
Linear Depolarization Ratio

Abstract. A better quantification of aerosol properties is required for improving the modelling of aerosol effects on weather and climate. This task is methodologically demanding due to the diversity of the microphysical properties of aerosols and the complex relation between their microphysical and optical properties. Advanced lidar systems provide spatially and temporally resolved information on the aerosol optical properties that is sufficient for the retrieval of important aerosol microphysical properties. Recently, the mass concentration of transported volcanic ash, which is relevant for the flight safety of aeroplanes, was retrieved from measurements of such lidar systems in southern Germany. The relative uncertainty of the retrieved mass concentration was on the order of ±50%. The present study investigates improvements of the retrieval accuracy when the capability of measuring the linear depolarization ratio at 1064 nm is added to the lidar setup. The lidar setups under investigation are based on those of MULIS and POLIS of the Ludwig-Maximilians-Universität in Munich (Germany) which measure the linear depolarization ratio at 355 and 532 nm with high accuracy. The improvements are determined by comparing uncertainties from retrievals applied to simulated measurements of this lidar setup with uncertainties obtained when the depolarization at 1064 nm is added to this setup. The simulated measurements are based on real lidar measurements of transported Eyjafjallajökull volcano ash. It is found that additional 1064 nm depolarization measurements significantly reduce the uncertainty of the retrieved mass concentration and effective particle size. This significant improvement in accuracy is the result of the increased sensitivity of the lidar setup to larger particles. The size dependence of the depolarization does not vary strongly with refractive index, thus we expect similar benefits for the retrieval in case of measurements of other volcanic ash compositions and also for transported desert dust. For the retrieval of the single scattering albedo, which is relevant to the radiative transfer in aerosol layers, no significant improvements were found.

scholarly journals Benefit of depolarization ratio at λ = 1064 nm for the retrieval of the aerosol microphysics from lidar measurements

2014 ◽  
Vol 7 (5) ◽  
pp. 5095-5115
Author(s):  
J. Gasteiger ◽  
V. Freudenthaler
Keyword(s):  
Optical Properties ◽  
Mass Concentration ◽  
Single Scattering ◽  
Sufficient Information ◽  
Depolarization Ratio ◽  
Aerosol Composition ◽  
Microphysical Properties ◽  
Lidar Measurements ◽  
Increased Sensitivity ◽  
Linear Depolarization Ratio

Abstract. A better quantification of aerosol microphysical and optical properties is required to improve the modelling of aerosol effects on weather and climate. This task is methodologically demanding due to the huge diversity of aerosol composition and of their shape and size distribution, and due to the complexity of the relation between the microphysical and optical properties. Lidar remote sensing is a valuable tool to gain spatially and temporally resolved information on aerosol properties. Advanced lidar systems provide sufficient information on the aerosol optical properties for the retrieval of important aerosol microphysical properties. Recently, the mass concentration of transported volcanic ash, which is relevant for the flight safety of airplanes, was retrieved from measurements of such lidar systems in Southern Germany. The relative uncertainty of the retrieved mass concentration was on the order of ±50%. The present study investigates improvements of the retrieval accuracy when the capability of measuring the linear depolarization ratio at 1064 nm is added to the lidar setup. The lidar setups under investigation are based on the setup of MULIS and POLIS of the LMU in Munich which measure the linear depolarization ratio at 355 nm and 532 nm with high accuracy. By comparing results of retrievals applied to simulated lidar measurements with and without the depolarization at 1064 nm it is found that the availability of 1064 nm depolarization measurements reduces the uncertainty of the retrieved mass concentration and effective particle size by a factor of about 2–3. This significant improvement in accuracy is the result of the increased sensitivity of the lidar setup to larger particles. However, the retrieval of the single scattering albedo, which is relevant for the radiative transfer in aerosol layers, does hardly benefit from the availability of 1064 nm depolarization measurements.

scholarly journals Particle settling and convective mixing in the Saharan Air Layer as seen from an integrated model, lidar, and in-situ perspective

2016 ◽  
Author(s):  
Josef Gasteiger ◽  
Silke Groß ◽  
Bernadett Weinzierl ◽  
Daniel Sauer ◽  
Volker Freudenthaler
Keyword(s):  
Dust Particles ◽  
Depolarization Ratio ◽  
Western Atlantic ◽  
Particle Counter ◽  
Convective Mixing ◽  
Saharan Air Layer ◽  
Lidar Measurements ◽  
Linear Depolarization Ratio ◽  
Aerosol Properties

Abstract. Long-range transport of aerosol in the Saharan Air Layer (SAL) across the Atlantic plays an important role for weather, climate, and ocean fertilization. However, processes occurring within the SAL and their effects on aerosol properties are still unclear. In this work we study particle settling and convective mixing within the SAL based on measured and modeled vertical aerosol profiles in the upper 1 km of the transported SAL. We use ground-based POLIS lidar measurements and airborne particle counter measurements over the Western Atlantic, as well as space-based CALIOP lidar measurements from Africa to the Western Atlantic. In our model we take account of the optical properties and the Stokes gravitational settling of irregularly-shaped Saharan dust particles. We test two hypotheses about the occurrence of convective mixing within the SAL over the Atlantic to explain the aerosol properties observed by the lidars and the particle counter. Our first hypothesis (H1) assumes that no mixing occurs in the SAL leading to an altitude separation of super-micron dust particles as a result of settling. The second hypothesis (H2) assumes that convective mixing occurs in the SAL during the day allowing large super-micron dust particles to stay airborne longer than without convective mixing. In general, a decrease of the particle linear depolarization ratio towards the SAL top is found in the measured lidar data but the decrease is much weaker than modeled in case of H1. The in-situ data on particle number concentrations show a presence of large particles near the SAL top that is inconsistent with H1. Furthermore, the analysis of the CALIOP measurements reveals that the average vertical profile of the linear depolarization ratio of the aerosols in the upper 1 km of the SAL does not change along its transport path over the Atlantic. These findings indicate H2 to be much more likely than H1, giving evidence that convective mixing occurs within the SAL over the Atlantic with significant consequences for the evolution of the size distribution of the super-micron dust particles during transport.

scholarly journals The potential of elastic and polarization lidars to retrieve extinction profiles

2020 ◽  
Vol 13 (2) ◽  
pp. 893-905 ◽  
Author(s):  
Elina Giannakaki ◽  
Panos Kokkalis ◽  
Eleni Marinou ◽  
Nikolaos S. Bartsotas ◽  
Vassilis Amiridis ◽  
...  
Keyword(s):  
Aerosol Optical Depth ◽  
Optical Depth ◽  
Dust Particles ◽  
Depolarization Ratio ◽  
Lidar System ◽  
Lidar Measurements ◽  
Lidar Ratio ◽  
Linear Depolarization Ratio ◽  
Aerosol Types ◽  
532 Nm

Abstract. A new method, called ElEx (elastic extinction), is proposed for the estimation of extinction coefficient lidar profiles using only the information provided by the elastic and polarization channels of a lidar system. The method is applicable to lidar measurements both during daytime and nighttime under well-defined aerosol mixtures. ElEx uses the particle backscatter profiles at 532 nm and the vertically resolved particle linear depolarization ratio measurements at the same wavelength. The particle linear depolarization ratio and the lidar ratio values of pure aerosol types are also taken from literature. The total extinction profile is then estimated and compared well with Raman retrievals. In this study, ElEx was applied in an aerosol mixture of marine and dust particles at Finokalia station during the CHARADMExp campaign. Any difference between ElEx and Raman extinction profiles indicates that the nondust component could be probably attributed to polluted marine or polluted continental aerosols. Comparison with sun photometer aerosol optical depth observations is performed as well during daytime. Differences in the total aerosol optical depth are varying between 1.2 % and 72 %, and these differences are attributed to the limited ability of the lidar to correctly represent the aerosol optical properties in the near range due to the overlap problem.

scholarly journals First triple-wavelength lidar observations of depolarization and extinction-to-backscatter ratios of Saharan dust

2021 ◽  
Author(s):  
Moritz Haarig ◽  
Albert Ansmann ◽  
Ronny Engelmann ◽  
Holger Baars ◽  
Dietrich Althausen ◽  
...  
Keyword(s):  
Saharan Dust ◽  
Depolarization Ratio ◽  
Spectral Slope ◽  
Desert Dust ◽  
Lidar Measurements ◽  
Lidar Ratio ◽  
Linear Depolarization Ratio ◽  
First Time ◽  
Dust Case ◽  
Lidar Observations

Abstract. Two Saharan dust layers observed over Leipzig in February and March 2021 were used to provide the first ever lidar measurements of the extinction coefficient at 1064 nm for desert dust. The advanced multiwavelength Raman polarization lidar was able to provide, for the first time, the lidar ratio (extinction-to-backscatter ratio) and particle linear depolarization ratio at all three classical lidar wavelengths (355, 532 and 1064 nm). The pure dust conditions during the first event exhibit lidar ratios of 47±8, 50±5 and 63±13 sr and particle linear depolarization ratios of 0.260±0.026, 0.298±0.017 and 0.214±0.025 at the wavelengths of 355, 532 and 1064 nm, respectively. The second, slightly polluted dust case shows a similar spectral behavior with values of the lidar ratio of 52±8, 47±5 and 61±10 sr and the depolarization ratio of 0.188±0.053, 0.270±0.017 and 0.242±0.007 at 355, 532 and 1064 nm, respectively. The results were compared to AERONET v3 inversions and GRASP retrievals at six and seven wavelengths, which could reproduce the spectral slope of the lidar ratio from 532 to 1064 nm. The spectral slope of the particle linear depolarization ratio could not be reproduced by the AERONET inversions, especially at 1064 nm.

scholarly journals Is Near-Spherical Shape “the New Black” for Smoke ?

2020 ◽  
Vol 237 ◽  
pp. 02017
Author(s):  
Anna Gialitaki ◽  
Alexandra Tsekeri ◽  
Vassilis Amiridis ◽  
Romain Ceolato ◽  
Lucas Paulien ◽  
...  
Keyword(s):  
Spherical Shape ◽  
Wavelength Dependence ◽  
Depolarization Ratio ◽  
Smoke Particles ◽  
Near Ir ◽  
Lidar Measurements ◽  
Lidar Ratio ◽  
T Matrix ◽  
Linear Depolarization Ratio

We present smoke lidar measurements from the Canadian fires of 2017. The advected smoke layers over Europe are detected at both tropospheric and stratospheric heights, with the latter presenting non-typical values of the Particle Linear Depolarization Ratio (PLDR) with strong wavelength dependence from the UV to the Near-IR. Specifically, the PLDR values are of the order of 22, 18 and 4% at 355, 532 and 1064 nm respectively. In an attempt to interpret these results, we apply the hypothesis that smoke particles have near-spherical shapes. Scattering calculations with the T-matrix code support other findings in the literature ([1]- [2]), showing that the near-spherical shape (or closely similar shapes as in [2]), is the only shape that has been shown to reproduce the observed PLDR and Lidar Ratio (LR) values of the stratospheric smoke particles at the three measurement wavelengths.

scholarly journals Wildfire Smoke in the Stratosphere Over Europe–First Measurements of Depolarization and Lidar Ratios at 355, 532, and 1064 nm

2020 ◽  
Vol 237 ◽  
pp. 02036
Author(s):  
Moritz Haarig ◽  
Holger Baars ◽  
Albert Ansmann ◽  
Ronny Engelmann ◽  
Kevin Ohneiser ◽  
...  
Keyword(s):  
Lower Stratosphere ◽  
Wavelength Dependence ◽  
Depolarization Ratio ◽  
Wildfire Smoke ◽  
Lidar Measurements ◽  
Smoke Layer ◽  
Lidar Ratio ◽  
Linear Depolarization Ratio ◽  
532 Nm

Canadian wildfire smoke was detected in the troposphere and lower stratosphere over Europe in August and September 2017. Lidar measurements from various stations of the European Aerosol Research Lidar Network (EARLINET) observed the stratospheric smoke layer. Triple-wavelength (355, 532, and 1064 nm) lidar measurements of the depolarization and the lidar ratio are reported from Leipzig, Germany. The particle linear depolarization ratio of the wildfire smoke in the stratosphere had an exceptional strong wavelength dependence reaching from 0.22 at 355 nm, to 0.18 at 532 nm, and 0.04 at 1064 nm. The lidar ratio increased with wavelength from 40±16 sr at 355 nm, to 66±12 sr at 532 nm, and 92±27 sr at 1064 nm. The development of the stratospheric smoke plume over several months was studied by long-term lidar measurements in Cyprus. The stratospheric smoke layers increased in altitude up to 24 km height.

scholarly journals Experimental calibration assessment of a MPLNET/Micro-Pulse Lidar system in comparison with EARLINET lidar measurements for aerosol optical properties retrieval

2020 ◽  
Author(s):  
Carmen Córdoba-Jabonero ◽  
Albert Ansmann ◽  
Cristofer Jiménez ◽  
Holger Baars ◽  
María-Ángeles López-Cayuela ◽  
...  
Keyword(s):  
Optical Properties ◽  
Depolarization Ratio ◽  
Backscatter Coefficient ◽  
Experimental Calibration ◽  
Experimental Procedure ◽  
Lidar Measurements ◽  
Total Particle ◽  
Linear Depolarization Ratio ◽  
Micro Pulse Lidar ◽  
The Impact

Abstract. Simultaneous observations of a polarized Micro-Pulse Lidar (P-MPL) system, currently operative within MPLNET (NASA Micro-Pulse Lidar Network), with two referenced EARLINET (European Aerosol Research Lidar Network) lidars, running at Leipzig site (Germany, 51.4º N 12.4º E, 125 m a.s.l.), were performed during a comprehensive two-month field campaign in summer 2019. A calibration assessment regarding the overlap (OVP) correction of the P-MPL signal profiles and its impact in the retrieval of the optical properties is achieved, describing also the experimental procedure used. The optimal lidar-specific OVP function for correcting the P-MPL measurements is experimentally determined, highlighting that the OVP function as delivered by the P-MPL manufacturer cannot be used. Among the OVP functions examined, the averaged one between those obtained from the comparison of the P-MPL observations with those of the other two referenced lidars seems to be the best proxy at both near- and far-field ranges. In addition, the impact of the OVP function in the accuracy of the retrieved profiles of the total particle backscatter coefficient (PBC) and the particle linear depolarization ratio (PLDR) is examined. First, the volume linear depolarization ratio (VLDR) profile is obtained and compared to the reference lidars, showing it needs to be corrected by a small offset value within a good accuracy. Once P-MPL measurements are optimally OVP-corrected, the PBC profiles (and hence the PLDR ones) can be derived using the Klett-Fernald approach. In addition, an alternative method based on the separation of the total PBC into their aerosol components is presented in order to estimate the total particle extinction coefficient (PEC) profile, and hence the Aerosol Optical Depth, from elastic P-MPL measurements. A dust event as observed at Leipzig in June 2019 is used for illustration. In overall, an adequate OVP function is needed to be determined in a regular basis to calibrate the P-MPL system in order to derive suitable aerosol products.

scholarly journals Multi-wavelength Raman lidar observations of the Eyjafjallajökull volcanic cloud over Potenza, Southern Italy

2011 ◽  
Vol 11 (4) ◽  
pp. 12763-12803 ◽  
Author(s):  
L. Mona ◽  
A. Amodeo ◽  
G. D'Amico ◽  
A. Giunta ◽  
F. Madonna ◽  
...  
Keyword(s):  
Southern Italy ◽  
Saharan Dust ◽  
Depolarization Ratio ◽  
Raman Lidar ◽  
Lidar Measurements ◽  
Ångström Exponent ◽  
Multi Wavelength ◽  
Lidar Ratio ◽  
Linear Depolarization Ratio ◽  
532 Nm

Abstract. Multi-wavelength Raman lidar measurements were performed at CNR-IMAA Atmospheric Observatory (CIAO) during the entire Eyjafjallajökull explosive eruptive period in April–May 2010, whenever weather conditions permitted. A methodology for volcanic layer identification and accurate aerosol typing has been developed on the basis both of the multi-wavelength Raman lidar measurements and EARLINET measurements performed at CIAO since 2000. The aerosol mask for lidar measurements performed at CIAO during the 2010 Eyjafjallajökull eruption has been obtained. Volcanic aerosol layers have been observed in different periods: 19–22 April, 27–29 April, 8–9 May, 13–14 May and 18–19 May. A maximum aerosol optical depth of about 0.12–0.13 was observed on 20 April, 22:00 UTC and 13 May, 20:30 UTC. Volcanic particles have been detected both at low altitudes, in the free troposphere and in the upper troposphere. Intrusions into the PBL have been revealed on 21–22 April and 13 May. In the April–May period Saharan dust intrusions typically occur in Southern Italy. For the period under investigations, a Saharan dust intrusion was observed on 13–14 May: dust and volcanic particles have been simultaneously observed at CIAO both at separated different levels and mixed within the same layer. Lidar ratios at 355 and 532 nm, Ångström exponent at 355/532 nm, backscatter related Ångström exponent at 532/1064 nm and particle linear depolarization ratio at 532 nm measured inside the detected volcanic layers have been discussed. The dependence of these quantities on relative humidity (RH) has been investigated by using co-located microwave profiler measurements. The particle linear depolarization ratio increasing with RH, lidar ratio values at 355 nm around 80 sr, and values of the ratio of lidar ratios greater than 1 suggest the presence of sulfates mixed with continental aerosol. Lower lidar ratio values (around 40 sr) increasing with RH and values of the ratio of lidar ratios lower than 1 indicate the presence of some aged ash inside these sulfate layers.

scholarly journals First triple-wavelength lidar observations of depolarization and extinction-to-backscatter ratios of Saharan dust

2022 ◽  
Vol 22 (1) ◽  
pp. 355-369
Author(s):  
Moritz Haarig ◽  
Albert Ansmann ◽  
Ronny Engelmann ◽  
Holger Baars ◽  
Carlos Toledano ◽  
...  
Keyword(s):  
Wavelength Dependence ◽  
Saharan Dust ◽  
Depolarization Ratio ◽  
Shape Model ◽  
Lidar Measurements ◽  
Fine Mode ◽  
Lidar Ratio ◽  
Linear Depolarization Ratio ◽  
Dust Case ◽  
Lidar Observations

Abstract. Two layers of Saharan dust observed over Leipzig, Germany, in February and March 2021 were used to provide the first-ever lidar measurements of the dust lidar ratio (extinction-to-backscatter ratio) and linear depolarization ratio at all three classical lidar wavelengths (355, 532 and 1064 nm). The pure-dust conditions during the first event exhibit lidar ratios of 47 ± 8, 50 ± 5 and 69 ± 14 sr and particle linear depolarization ratios of 0.242 ± 0.024, 0.299 ± 0.018 and 0.206 ± 0.010 at wavelengths of 355, 532 and 1064 nm, respectively. The second, slightly polluted-dust case shows a similar spectral behavior of the lidar and depolarization ratio with values of the lidar ratio of 49 ± 4, 46 ± 5 and 57 ± 9 sr and the depolarization ratio of 0.174 ± 0.041, 0.298 ± 0.016 and 0.242 ± 0.007 at 355, 532 and 1064 nm, respectively. The results were compared with Aerosol Robotic Network (AERONET) version 3 (v3) inversion solutions and the Generalized Retrieval of Aerosol and Surface Properties (GRASP) at six and seven wavelengths. Both retrieval schemes make use of a spheroid shape model for mineral dust. The spectral slope of the lidar ratio from 532 to 1064 nm could be well reproduced by the AERONET and GRASP retrieval schemes. Higher lidar ratios in the UV were retrieved by AERONET and GRASP. The enhancement was probably caused by the influence of fine-mode pollution particles in the boundary layer which are included in the columnar photometer measurements. Significant differences between the measured and retrieved wavelength dependence of the particle linear depolarization ratio were found. The potential sources for these uncertainties are discussed.

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