Reactivity of dolomite in water-saturated supercritical carbon dioxide: Significance for carbon capture and storage and for enhanced oil and gas recovery

2013 ◽  
Vol 65 ◽  
pp. 564-573 ◽  
Author(s):  
Xiuyu Wang ◽  
Vladimir Alvarado ◽  
Norbert Swoboda-Colberg ◽  
John P. Kaszuba
Author(s):  
Naimish Agarwal

Abstract: More than ever, the fate of anthropogenic CO2 emissions is in our hands. Since the advent of industrialization, there has been an increase in the use of fossil fuels to fulfil rising energy demands. The usage of such fuels results in the release of carbon dioxide (CO2) and other greenhouse gases, which result in increased temperature. Such warming is extremely harmful to life on Earth. The development of technology to counter the climate change and spreading it for widespread adoptions. We need to establish a framework to provide overarching guidance for the well-functioning of technology and mechanism development of Carbon Capture and Storage. Carbon capture and storage (CCS) is widely regarded as a critical approach for achieving the desired CO2 emission reduction. Various elements of CCS, such as state-of-the-art technology for CO2 collection, separation, transport, storage, politics, opportunities, and innovations, are examined and explored in this paper. Carbon capture and storage is the process of capturing and storing carbon dioxide (CO2) before it is discharged into the environment (CCS). The technology can capture high amounts of CO2 produced by fossil fuel combustion in power plants and industrial processes. CO2 is compressed and transferred by pipeline, ship, or road tanker once it has been captured. CO2 can then be piped underground, usually to depths of 1km or more, and stored in depleted oil and gas reservoirs, coalbeds, or deep saline aquifers, depending on the geology. CO2 could also be used to produce commercially marketable products. With the goal of keeping world average temperatures below 1.5°C (2.7°F) and preventing global average temperature rises of more than 2°C (3.6°F) over pre-industrial levels, CCS model should be our priority to be implemented with the proper economical map


2021 ◽  
Vol 9 ◽  
Author(s):  
Wang Huiru ◽  
You Zhanping ◽  
Mo Fan ◽  
Liu Bin ◽  
Han Peng

In the carbon capture and storage (CCS) infrastructure, the risk of a high-pressure buried pipeline rupture possibly leads to catastrophic accidents due to the release of tremendous amounts of carbon dioxide (CO2). Therefore, a comprehensive understanding of the effects of CO2 dispersion pattern after release from CCS facilities is essential to allow the appropriate safety precautions to be taken. Due to variations in topography above the pipeline, the pattern of CO2 dispersion tends to be affected by the real terrain features, such as trees and hills. However, in most previous studies, the dynamic impact of trees on the wind field was often approximated to linear treatment or even ignored. In this article, a computational fluid dynamics (CFD) model was proposed to predict CO2 dispersion over shrubbery areas. The shrubs were regarded as a kind of porous media, and the model was validated against the results from experiment. It was found that shrubbery affected the flow field near the ground, enhancing the lateral dispersion of CO2. Compared with that of the shrub-free terrain, the coverage area of the three shrub terrains at 60 s increased by 8.1 times, 6.7 times, and 9.1 times, respectively. The influence of shrub height and porosity on CO2 dispersion is nonlinear. This research provides reliable data for the risk assessment of CCS.


2013 ◽  
Vol 13 ◽  
pp. 78-86 ◽  
Author(s):  
Yolanda Sanchez-Vicente ◽  
Trevor C. Drage ◽  
Martyn Poliakoff ◽  
Jie Ke ◽  
Michael W. George

2014 ◽  
Vol 86 (24) ◽  
pp. 12191-12198 ◽  
Author(s):  
Robert van Geldern ◽  
Martin E. Nowak ◽  
Martin Zimmer ◽  
Alexandra Szizybalski ◽  
Anssi Myrttinen ◽  
...  

Author(s):  
Magali Roger ◽  
Thomas C. P. Reed ◽  
Frank Sargent

Escherichia coli is gram-negative bacterium that is a workhorse for biotechnology. The organism naturally performs a mixed-acid fermentation under anaerobic conditions where it synthesises formate hydrogenlyase (FHL-1). The physiological role of the enzyme is the disproportionation of formate in to H 2 and CO 2 . However, the enzyme has been observed to catalyse hydrogenation of CO 2 given the correct conditions, and so has possibilities in bio-based carbon capture and storage if it can be harnessed as a hydrogen-dependent CO 2 -reductase (HDCR). In this study, an E. coli host strain was engineered for the continuous production of formic acid from H 2 and CO 2 during bacterial growth in a pressurised batch bioreactor. Incorporation of tungsten, in place of molybdenum, in FHL-1 helped to impose a degree of catalytic bias on the enzyme. This work demonstrates that it is possible to couple cell growth to simultaneous, unidirectional formate production from carbon dioxide and develops a process for growth under pressurised gases. IMPORTANCE Greenhouse gas emissions, including waste carbon dioxide, are contributing to global climate change. A basket of solutions is needed to steadily reduce emissions, and one approach is bio-based carbon capture and storage. Here we present out latest work on harnessing a novel biological solution for carbon capture. The Escherichia coli formate hydrogenlyase (FHL-1) was engineered to be constitutively expressed. Anaerobic growth under pressurised H 2 and CO 2 gases was established and aqueous formic acid was produced as a result. Incorporation of tungsten in to the enzyme in place of molybdenum proved useful in poising FHL-1 as a hydrogen-dependent CO 2 reductase (HDCR).


2019 ◽  
Vol 38 (4) ◽  
pp. 733-750
Author(s):  
Sébastien Chailleux

Analyzing the case of France, this article aims to explain how the development of enhanced oil recovery techniques over the last decade contributed to politicizing the subsurface, that is putting underground resources at the center of social unrest and political debates. France faced a decline of its oil and gas activity in the 1990s, followed by a renewal with subsurface activity in the late 2000s using enhanced oil recovery techniques. An industrial demonstrator for carbon capture and storage was developed between 2010 and 2013 , while projects targeting unconventional oil and gas were pushed forward between 2008 and 2011 before eventually being canceled. We analyze how the credibility, legitimacy, and governance of those techniques were developed and how conflicts made the role of the subsurface for energy transition the target of political choices. The level of political and industrial support and social protest played a key role in building project legitimacy, while the types of narratives and their credibility determined the distinct trajectories of hydraulic fracturing and carbon capture and storage in France. The conflicts over enhanced oil recovery techniques are also explained through the critical assessment of the governance framework that tends to exclude civil society stakeholders. We suggest that these conflicts illustrated a new type of politicization of the subsurface by merging geostrategic concerns with social claims about governance, ecological demands about pollution, and linking local preoccupations to global climate change.


2013 ◽  
Vol 318 ◽  
pp. 519-521 ◽  
Author(s):  
Xiao Lan Liu ◽  
Jian Gang Liu ◽  
Hong Bo Niu

Some novel drilling technology has promoted the exploration of unconventional oil and gas resources greatly, such as gas drilling, long horizontal section well drilling and so on. As special matter, Supercritical carbon dioxide has many useful characteristic. For example, relative higher gravity like water, lower viscosity like gas and wonderful crude oil displacement characteristics, these could play some important role if being used in exploration of unconventional oil and gas. Therefore, the feasibility study of supercritical carbon dioxide drilling technology and equipment matching plan are discussed in this article to make the preliminary studies and preparation of related technology. On the basis of a lot of research and study, This paper carries out a feasibility study of supercritical carbon dioxide drilling equipment.


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