Application of seawater to enhance SO2 removal from simulated flue gas through hollow fiber membrane contactor

2008 ◽  
Vol 312 (1-2) ◽  
pp. 6-14 ◽  
Author(s):  
Xueyan Sun ◽  
Fangang Meng ◽  
Fenglin Yang
2016 ◽  
Vol 2016 ◽  
pp. 1-9 ◽  
Author(s):  
Ziyi Qu ◽  
Li Zhang ◽  
Yunfei Yan ◽  
Shunxiang Ju

Hollow fiber membrane contactor is a new, highly efficient, and the most promising technology for CO2absorption in flue gas. There is still SO2that exists in the flue gas after desulfurization tower of power plant. This paper studied the influence of SO2on CO2absorption characteristic in flue gas by hollow fiber membrane contactor with absorbent of EDA, EDA + MEA (0.6 : 0.4), and EDA + MEA + PZ (0.4 : 0.4 : 0.2). The influences of SO2concentration, cycle absorption and desorption characteristic of absorbent, absorbent concentration, and liquid-gas flow rate ratio are studied to analyze the influence of SO2on CO2absorption characteristic. The appropriate absorbent composition ratio and appropriate parameter range that can inhibit the influence of SO2are proposed by studying the hybrid sorbent with activating agent, appropriate absorbent concentration, and ratio of liquid-gas flow rate. Among the three kinds of absorbents, EDA + MEA + PZ (0.4 : 0.4 : 0.2) had the best tolerance ability to SO2and the highest efficiency. With comprehensive consideration of CO2removal efficiency and operating cost, under the condition of 1000 ppm SO2, the appropriate concentration and liquid-gas flow rate ratio of EDA, EDA + MEA, and EDA + MEA + PZ are proposed.


2012 ◽  
Vol 616-618 ◽  
pp. 1546-1549
Author(s):  
Wei Feng Zhang ◽  
Jian Shao

A small hollow-fiber membrane contactor system was used to test the absorption and desorption CO2 using mixed absorption solution of SG/PG and TEA. The results showed that absorption effect of SG was better than PG under low concentrations, but their desorption was the opposite. With the increase of concentration, the absorption effect of SG tended to weak, while the desorption was enhanced. And, PG was contrary. The absorption effect of mixed solution(SG+TEA, PG+TEA) was excellent when adding small amount of TEA. And, the absorption effect of TEA-SG mixed solution was amazing under the low concentration of SG. With the concentration of mixed solution increased, the auxo-action of TEA weakened. Instead, TEA played a active effect on promoting the absorption of TEA+PG mixture with the increasing of concentration. The hybrid experimental results shown that 3mol/L PG+0.1 mol/L TEA mixture absorption solution was best in absorption experiments, and 1mol/L PG+0.2 mol/L TEA mixture absorption solution was best in desorption experiments.


2014 ◽  
Vol 16 (2) ◽  
pp. 354-373 ◽  

<div> <p>With the aggravation of the unprecedented greenhouse effect, the reduction of greenhouse gases which mainly consist of CO<sub>2</sub> has caught high attention by global scholars. The membrane absorption of CO<sub>2</sub> from the flue gas seems a promising alternative to conventional absorption methods like chemical absorption. In this article, the principles of the membrane absorption process were discussed. The research development and current status of CO<sub>2</sub> capture in flue gas using a hollow fiber membrane contactor were reviewed. The affecting factors included the membrane structure and material, module connection form, gas and liquid flow pattern and absorbent. Also, these factors that affected the separation performance of mass transfer processes, as well as the mass transfer coefficients and models for CO<sub>2</sub> absorption were critically discussed in the tube side, shell side and membrane. Also, an experiment system for CO<sub>2</sub> absorption in a membrane contactor was dipicted. The modeling works were validated with experimental results. Additionally, the deficiencies of present development in membrane gas absorption of acid gases and recommendations for future pilot-scale applications were proposed.&nbsp;</p> </div> <p>&nbsp;</p>


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