Abstract. A fraction of the Himalayan aerosols originate from secondary sources, which are currently poorly quantified. To clarify the climatic importance of regional secondary particle formation at Himalayas, data from 2005 to 2010 of continuous aerosol measurements at a high-altitude (2180 m) Indian Himalayan site, Mukteshwar, were analyzed. For this period, the days were classified, and the particle formation and growth rates were calculated for clear new particle formation (NPF) event days. The NPF events showed a pronounced seasonal cycle. The frequency of the events peaked in spring, when the ratio between event and non-event days was 53 %, whereas the events were truly sporadic on any other seasons. The annual mean particle formation and growth rates were 0.40 cm−3 s−1 and 2.43 nm h−1, respectively. The clear annual cycle was found to be mainly controlled by the seasonal evolution of the Planetary Boundary Layer (PBL) height together with local meteorological conditions. Spring NPF events were connected with increased PBL height, and therefore characterised as boundary layer events, while the rare events in other seasons represented lower free tropospheric particle formation.
Time-resolved characterization of primary particle emissions and secondary
particle formation from a modern gasoline passenger car