A case study of the impact of boundary layer aerosol size distribution on the surface UV irradiance

2001 ◽  
Vol 35 (30) ◽  
pp. 5041-5051 ◽  
Author(s):  
Ülle Kikas ◽  
Aivo Reinart ◽  
Mai Vaht ◽  
Uno Veismann
Keyword(s):  
Boundary Layer ◽  
Size Distribution ◽  
Aerosol Size Distribution ◽  
Uv Irradiance ◽  
The Impact

scholarly journals The impact of a foehn wind on PM10 concentrations and the urban boundary layer in complex terrain: a case study from Kraków, Poland

Tellus B ◽  
2021 ◽  
Vol 73 (1) ◽  
pp. 1-26
Author(s):  
Piotr Sekuła ◽  
Anita Bokwa ◽  
Zbigniew Ustrnul ◽  
Mirosław Zimnoch ◽  
Bogdan Bochenek
Keyword(s):  
Boundary Layer ◽  
Complex Terrain ◽  
Urban Boundary Layer ◽  
The Impact

scholarly journals Evaluating model parameterizations of submicron aerosol scattering and absorption with in situ data from ARCTAS 2008

2016 ◽  
Vol 16 (14) ◽  
pp. 9435-9455 ◽  
Author(s):  
Matthew J. Alvarado ◽  
Chantelle R. Lonsdale ◽  
Helen L. Macintyre ◽  
Huisheng Bian ◽  
Mian Chin ◽  
...  
Keyword(s):  
Optical Properties ◽  
Size Distribution ◽  
Aerosol Size Distribution ◽  
Visible Radiation ◽  
Submicron Aerosol ◽  
In Situ Data ◽  
Aerosol Absorption ◽  
Aerosol Scattering ◽  
The Impact

Abstract. Accurate modeling of the scattering and absorption of ultraviolet and visible radiation by aerosols is essential for accurate simulations of atmospheric chemistry and climate. Closure studies using in situ measurements of aerosol scattering and absorption can be used to evaluate and improve models of aerosol optical properties without interference from model errors in aerosol emissions, transport, chemistry, or deposition rates. Here we evaluate the ability of four externally mixed, fixed size distribution parameterizations used in global models to simulate submicron aerosol scattering and absorption at three wavelengths using in situ data gathered during the 2008 Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) campaign. The four models are the NASA Global Modeling Initiative (GMI) Combo model, GEOS-Chem v9-02, the baseline configuration of a version of GEOS-Chem with online radiative transfer calculations (called GC-RT), and the Optical Properties of Aerosol and Clouds (OPAC v3.1) package. We also use the ARCTAS data to perform the first evaluation of the ability of the Aerosol Simulation Program (ASP v2.1) to simulate submicron aerosol scattering and absorption when in situ data on the aerosol size distribution are used, and examine the impact of different mixing rules for black carbon (BC) on the results. We find that the GMI model tends to overestimate submicron scattering and absorption at shorter wavelengths by 10–23 %, and that GMI has smaller absolute mean biases for submicron absorption than OPAC v3.1, GEOS-Chem v9-02, or GC-RT. However, the changes to the density and refractive index of BC in GC-RT improve the simulation of submicron aerosol absorption at all wavelengths relative to GEOS-Chem v9-02. Adding a variable size distribution, as in ASP v2.1, improves model performance for scattering but not for absorption, likely due to the assumption in ASP v2.1 that BC is present at a constant mass fraction throughout the aerosol size distribution. Using a core-shell mixing rule in ASP overestimates aerosol absorption, especially for the fresh biomass burning aerosol measured in ARCTAS-B, suggesting the need for modeling the time-varying mixing states of aerosols in future versions of ASP.

scholarly journals Combining airborne in situ and ground-based lidar measurements for attribution of aerosol layers

2018 ◽  
Author(s):  
Anna Nikandrova ◽  
Ksenia Tabakova ◽  
Antti Manninen ◽  
Riikka Väänänen ◽  
Tuukka Petäjä ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Size Distribution ◽  
Aerosol Size Distribution ◽  
Long Range Transport ◽  
Back Trajectories ◽  
Clear Sky ◽  
Temporal And Spatial Variability ◽  
Range Transport ◽  
Temporal And Spatial

Abstract. Understanding the distribution of aerosol layers is important for determining long range transport and aerosol radiative forcing. In this study we combine airborne in situ measurements of aerosol with data obtained by a ground-based High Spectral Resolution Lidar (HSRL) and radiosonde profiles to investigate the temporal and vertical variability of aerosol properties in the lower troposphere. The HSRL was deployed in Hyytiälä, Southern Finland, from January to September 2014 as a part of the US DoE ARM (Atmospheric Radiation Measurement) mobile facility during the BAECC (Biogenic Aerosols – Effects on Cloud and Climate) Campaign. Two flight campaigns took place in April and August 2014 with instruments measuring the aerosol size distribution from 10 nm to 10 µm at altitudes up to 3800 m. Two case studies from the flight campaigns, when several aerosol layers were identified, were selected for further investigation: one clear sky case, and one partly cloudy case. During the clear sky case, turbulent mixing ensured low temporal and spatial variability in the measured aerosol size distribution in the boundary layer whereas mixing was not as homogeneous in the boundary layer during the partly cloudy case. The elevated layers exhibited greater temporal and spatial variability in aerosol size distribution, indicating a lack of mixing. New particle formation was observed in the boundary layer during the clear sky case, and nucleation mode particles were also seen in the elevated layers that were not mixing with the boundary layer. Interpreting local measurements of elevated layers in terms of long-range transport can be achieved using back trajectories from Lagrangian models, but care should be taken in selecting appropriate arrival heights, since the modelled and observed layer heights did not always coincide. We conclude that higher confidence in attributing elevated aerosol layers with their air mass origin is attained when back trajectories are combined with lidar and radiosonde profiles.

scholarly journals A global off-line model of size-resolved aerosol microphysics: I. Model development and prediction of aerosol properties

2005 ◽  
Vol 5 (8) ◽  
pp. 2227-2252 ◽  
Author(s):  
D. V. Spracklen ◽  
K. J. Pringle ◽  
K. S. Carslaw ◽  
M. P. Chipperfield ◽  
G. W. Mann
Keyword(s):  
Boundary Layer ◽  
Sulfuric Acid ◽  
Size Distribution ◽  
Marine Boundary Layer ◽  
Transport Model ◽  
Model Development ◽  
Aerosol Size Distribution ◽  
Chemical Transport Model ◽  
Cloud Processing ◽  
Nucleation Mechanisms

Abstract. A GLObal Model of Aerosol Processes (GLOMAP) has been developed as an extension to the TOMCAT 3-D Eulerian off-line chemical transport model. GLOMAP simulates the evolution of the global aerosol size distribution using a sectional two-moment scheme and includes the processes of aerosol nucleation, condensation, growth, coagulation, wet and dry deposition and cloud processing. We describe the results of a global simulation of sulfuric acid and sea spray aerosol. The model captures features of the aerosol size distribution that are well established from observations in the marine boundary layer and free troposphere. Modelled condensation nuclei (CN>3nm) vary between about 250–500 cm-3 in remote marine boundary layer regions and are generally in good agreement with observations. Modelled continental CN concentrations are lower than observed, which may be due to lack of some primary aerosol sources or the neglect of nucleation mechanisms other than binary homogeneous nucleation of sulfuric acid-water particles. Remote marine CN concentrations increase to around 2000–10 000 cm

scholarly journals Evaluating Model Parameterizations of Submicron Aerosol Scattering and Absorption with In Situ Data from ARCTAS 2008

2016 ◽  
Author(s):  
M. J. Alvarado ◽  
C. R. Lonsdale ◽  
H. L. Macintyre ◽  
H. Bian ◽  
M. Chin ◽  
...  
Keyword(s):  
Optical Properties ◽  
Size Distribution ◽  
Aerosol Size Distribution ◽  
Visible Radiation ◽  
Submicron Aerosol ◽  
In Situ Data ◽  
Aerosol Absorption ◽  
Aerosol Scattering ◽  
The Impact

Abstract. Accurate modeling of the scattering and absorption of ultraviolet and visible radiation by aerosols is essential for accurate simulations of atmospheric chemistry and climate. Closure studies using in situ measurements of aerosol scattering and absorption can be used to evaluate and improve models of aerosol optical properties without interference from model errors in aerosol emissions, transport, chemistry, or deposition rates. Here we evaluate the ability of four externally mixed, fixed size distribution parameterizations used in global models to simulate submicron aerosol scattering and absorption at three wavelengths using in situ data gathered during the 2008 Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) campaign. The four models are the NASA Global Modeling Initiative (GMI) Combo model, GEOS-Chem v9-02, the baseline configuration of a version of GEOS-Chem with online radiative transfer calculations (called GC-RT), and the Optical Properties of Aerosol and Clouds (OPAC v3.1) package. We also use the ARCTAS data to perform the first evaluation of the ability of the Aerosol Simulation Program (ASP v2.1) to simulate submicron aerosol scattering and absorption when in situ data on the aerosol size distribution is used, and examine the impact of different mixing rules for black carbon (BC) on the results. We find that the GMI model tends to overestimate submicron scattering and absorption at shorter wavelengths by 10–23 %, and that GMI has smaller absolute mean biases for submicron absorption than OPAC v3.1, GEOS-Chem v9-02, or GC-RT. However, the changes to the density and refractive index of BC in GC-RT improve the simulation of submicron aerosol absorption at all wavelengths relative to GEOS-Chem v9-02. Adding in situ size distribution information, as in ASP v2.1, improves model performance for scattering but not for absorption, likely due to the assumption in ASP v2.1 that BC is present at a constant mass fraction through out the aerosol size distribution. Using a core-shell mixing state in ASP overestimates aerosol absorption, especially for the fresh biomass burning aerosol measured in ARCTAS-B, suggesting the need for time-varying mixing states in future versions of ASP.

scholarly journals Evaluation of Second-Hand Exposure to Electronic Cigarette Vaping under a Real Scenario: Measurements of Ultrafine Particle Number Concentration and Size Distribution and Comparison with Traditional Tobacco Smoke

Toxics ◽  
2019 ◽  
Vol 7 (4) ◽  
pp. 59 ◽  
Author(s):  
Jolanda Palmisani ◽  
Alessia Di Gilio ◽  
Laura Palmieri ◽  
Carmelo Abenavoli ◽  
Marco Famele ◽  
...  
Keyword(s):  
Size Distribution ◽  
Tobacco Smoke ◽  
Ultrafine Particles ◽  
Natural Ventilation ◽  
Ultrafine Particle ◽  
Inhalation Exposure ◽  
Number Concentration ◽  
Aerosol Size Distribution ◽  
High Temporal Resolution ◽  
The Impact

The present study aims to evaluate the impact of e-cig second-hand aerosol on indoor air quality in terms of ultrafine particles (UFPs) and potential inhalation exposure levels of passive bystanders. E-cig second-hand aerosol characteristics in terms of UFPs number concentration and size distribution exhaled by two volunteers vaping 15 different e-liquids inside a 49 m3 room and comparison with tobacco smoke are discussed. High temporal resolution measurements were performed under natural ventilation conditions to simulate a realistic exposure scenario. Results showed a systematic increase in UFPs number concentration (part cm−3) related to a 20-min vaping session (from 6.56 × 103 to 4.01 × 104 part cm−3), although this was one up to two order of magnitude lower than that produced by one tobacco cigarette consumption (from 1.12 × 105 to 1.46 × 105 part cm−3). E-cig second-hand aerosol size distribution exhibits a bimodal behavior with modes at 10.8 and 29.4 nm in contrast with the unimodal typical size distribution of tobacco smoke with peak mode at 100 nm. In the size range 6–26 nm, particles concentration in e-cig second-hand aerosol were from 2- (Dp = 25.5 nm) to 3800-fold (Dp = 9.31 nm) higher than in tobacco smoke highlighting that particles exhaled by users and potentially inhaled by bystanders are nano-sized with high penetration capacity into human airways.

scholarly journals Optical Properties of the Urban Aerosol Particles Obtained from Ground Based Measurements and Satellite-Based Modelling Studies

2015 ◽  
Vol 2015 ◽  
pp. 1-12 ◽  
Author(s):  
Genrik Mordas ◽  
Nina Prokopciuk ◽  
Steigvilė Byčenkienė ◽  
Jelena Andriejauskienė ◽  
Vidmantas Ulevicius
Keyword(s):  
Optical Properties ◽  
Light Scattering ◽  
Urban Environment ◽  
Size Distribution ◽  
Number Concentration ◽  
Scattering Coefficient ◽  
Dust Particles ◽  
Aerosol Size Distribution ◽  
Air Masses ◽  
The Impact

Applications of satellite remote sensing data combined with ground measurements and model simulation were applied to study aerosol optical properties as well as aerosol long-range transport under the impact of large scale circulation in the urban environment in Lithuania (Vilnius). Measurements included the light scattering coefficients at 3 wavelengths (450, 550, and 700 nm) measured with an integrating nephelometer and aerosol particle size distribution (0.5–12 μm) and number concentration (Dpa> 0.5 μm) registered by aerodynamic particle sizer. Particle number concentration and mean light scattering coefficient varied from relatively low values of 6.0 cm−3and 12.8 Mm−1associated with air masses passed over Atlantic Ocean to relatively high value of 119 cm−3and 276 Mm−1associated with South-Western air masses. Analysis shows such increase in the aerosol light scattering coefficient (276 Mm−1) during the 3rd of July 2012 was attributed to a major Sahara dust storm. Aerosol size distribution with pronounced coarse particles dominance was attributed to the presence of dust particles, while resuspended dust within the urban environment was not observed.

Can the Deforestation Breeze Change the Rainfall in Amazonia? A Case Study for the BR-163 Highway Region

2010 ◽  
Vol 14 (18) ◽  
pp. 1-25 ◽  
Author(s):  
Sandra I. Saad ◽  
Humberto R. da Rocha ◽  
Maria A. F. Silva Dias ◽  
Rafael Rosolem
Keyword(s):  
Boundary Layer ◽  
Large Scale ◽  
Three Dimensional ◽  
Atmospheric Modeling ◽  
Thermal Cell ◽  
Soil Wetness ◽  
Soil Dryness ◽  
Regional Atmospheric Modeling ◽  
The Impact

Abstract The authors simulated the effects of Amazonian mesoscale deforestation in the boundary layer and in rainfall with the Brazilian Regional Atmospheric Modeling System (BRAMS) model. They found that both the area and shape (with respect to wind incidence) of deforestation and the soil moisture status contributed to the state of the atmosphere during the time scale of several weeks, with distinguishable patterns of temperature, humidity, and rainfall. Deforestation resulted in the development of a three-dimensional thermal cell, the so-called deforestation breeze, slightly shifted downwind to large-scale circulation. The boundary layer was warmer and drier above 1000-m height and was slightly wetter up to 2000-m height. Soil wetness affected the circulation energetics proportionally to the soil dryness (for soil wetness below ∼0.6). The shape of the deforestation controlled the impact on rainfall. The horizontal strips lined up with the prevailing wind showed a dominant increase in rainfall, significant up to about 60 000 km2. On the other hand, in the patches aligned in the opposite direction (north–south), there was both increase and decrease in precipitation in two distinct regions, as a result of clearly separated upward and downward branches, which caused the precipitation to increase for patches up to 15 000 km2. The authors’ estimates for the size of deforestation impacting the rainfall contributed to fill up the low spatial resolution in other previous studies.

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