A rational computational study of surface defect-mediated stabilization of low-dimensional Pt nanostructures on TiN(100)

2015 ◽  
Vol 17 (15) ◽  
pp. 9680-9686 ◽  
Author(s):  
Young Joo Tak ◽  
Woosun Jang ◽  
Norina A. Richter ◽  
Aloysius Soon
Keyword(s):  
Fuel Cell ◽  
High Performance ◽  
Surface Defect ◽  
Computational Study ◽  
Cell Technology ◽  
Support Interaction ◽  
Metal Support Interaction ◽  
Metal Support ◽  
Low Dimensional ◽  
Computational Platform

A rational computational platform to design surface defect-mediated low-dimensional Pt/TiN nanocatalysts for next generation high-performance fuel cell technology via strong electronic metal–support interaction.

Enhancing metal–support interaction by in situ ion-exchanging strategy for high performance Pt catalysts in hydrogen evolution reaction

2020 ◽  
Vol 8 (32) ◽  
pp. 16582-16589 ◽  
Author(s):  
Xulei Sui ◽  
Lei Zhang ◽  
Junjie Li ◽  
Kieran Doyle-Davis ◽  
Ruying Li ◽  
...  
Keyword(s):  
Hydrogen Evolution ◽  
Hydrogen Evolution Reaction ◽  
High Performance ◽  
Pt Catalysts ◽  
Acidic Media ◽  
Support Interaction ◽  
Metal Support Interaction ◽  
Metal Support ◽  
Metal Support Interactions

A facile in situ ion-exchanging strategy directly enhances metal–support interactions between Pt and support and promotes HER electrocatalytic performance in acidic media.

Ruthenium nanoclusters dispersed on titania nanorods and nanoparticles as high-performance catalysts for aqueous-phase Fischer–Tropsch synthesis

2016 ◽  
Vol 6 (23) ◽  
pp. 8355-8363 ◽  
Author(s):  
Jing-Wen Yu ◽  
Wei-Zhen Li ◽  
Tao Zhang ◽  
Ding Ma ◽  
Ya-Wen Zhang
Keyword(s):  
Aqueous Phase ◽  
High Performance ◽  
Tropsch Synthesis ◽  
Fischer Tropsch ◽  
Fischer Tropsch Synthesis ◽  
Support Interaction ◽  
Metal Support Interaction ◽  
Metal Support

The high AFTS activity and C5+ selectivity of the serial Ru/TiO2 nanocatalysts were favoured by the increasing metallic Ru sites due to H2 reduction pretreatment and weak metal–support interaction.

High performance Pt/Ti3O5Mo0.2Si0.4 electrocatalyst with outstanding methanol oxidation activity

2019 ◽  
Vol 9 (15) ◽  
pp. 4118-4124 ◽  
Author(s):  
Reza Alipour Moghadam Esfahani ◽  
Reza B. Moghaddam ◽  
E. Bradley Easton
Keyword(s):  
Activation Energy ◽  
Charge Transfer ◽  
Methanol Oxidation ◽  
High Performance ◽  
Charge Transfer Resistance ◽  
Oxidation Activity ◽  
Transfer Resistance ◽  
Support Interaction ◽  
Metal Support Interaction ◽  
Metal Support

The strong metal–support interaction in Pt/Ti3O5Mo0.2Si0.4 enhances the methanol oxidation activity by decreasing the charge transfer resistance and activation energy.

scholarly journals Transition metal on topological chiral semimetal PdGa with tailored hydrogen adsorption and reduction

2021 ◽  
Vol 7 (1) ◽  
Author(s):  
Qun Yang ◽  
Guowei Li ◽  
Yudi Zhang ◽  
Jian Liu ◽  
Jiancun Rao ◽  
...  
Keyword(s):  
High Performance ◽  
Hydrogen Adsorption ◽  
Surface States ◽  
Catalytic Performance ◽  
Support Interaction ◽  
Adsorption Behaviors ◽  
Metal Support Interaction ◽  
High Efficient ◽  
Metal Support ◽  
Topological Surface

AbstractThe difficulties in designing high-performance hydrogen evolution reaction (HER) catalysts lie in the manipulation of adsorption behaviors of transition metals (TMs). Topological chiral semimetals with super-long Fermi arc surface states provide an ideal platform for engineering the catalytic performance of TMs through the metal-support interaction. We found the adsorption trends of TMs can be modified significantly when deposited at the surface of the PdGa chiral crystal. The electron transfer from the TMs to the surface states of the PdGa reshapes the d band structure of TMs and weakens the hydrogen intermediate bonding. Especially, W/PdGa is expected to be a good HER catalyst with close to zero Gibbs free energy. Experimentally, we found a Pt-like exchange current density and turnover frequency when depositing W atoms at the PdGa nanostructures surface. The findings provide a way to develop high-efficient electrocatalysts by the interplay between topological surface states and metal-support interaction.

MOF-derived PtCo/Co3O4 nanocomposites in carbonaceous matrices as high-performance ORR electrocatalysts synthesized via Laser Ablation techniques

2021 ◽  
Author(s):  
Erick Leonar Ribeiro ◽  
Elijah M Davis ◽  
Mahshid Mokhtarnejad ◽  
Sheng Hu ◽  
Dibyendu Mukherjee ◽  
...  
Keyword(s):  
Fuel Cell ◽  
Laser Ablation ◽  
Energy Conversion ◽  
High Performance ◽  
Sustainable Energy ◽  
Ablation Techniques ◽  
Global Energy ◽  
Cell Technology ◽  
Energy Demands ◽  
Rational Development

Rapidly expanding global energy demands due to fast-paced human-technology interfaces have propelled fuel cell technology as a sustainable energy-conversion alternative. Nonetheless, the rational development of such technology demands the engineering...

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