scholarly journals Fast-timing measurements in neutron-rich odd-mass zirconium isotopes using LaBr3:Ce detectors coupled with Gammasphere

2018 ◽  
Vol 193 ◽  
pp. 05004 ◽  
Author(s):  
E.R. Gamba ◽  
S. Lalkovski ◽  
M. Rudigier ◽  
A.M. Bruce ◽  
S. Bottoni ◽  
...  
Keyword(s):  
Standard Deviation ◽  
Excited States ◽  
Timing Analysis ◽  
National Laboratory ◽  
Argonne National Laboratory ◽  
Quadrupole Deformation ◽  
Fast Timing ◽  
Lifetime Value ◽  
Quadrupole Deformation Parameter ◽  
Decay Of Excited States

A fast-timing experiment was performed at the Argonne National Laboratory to measure the lifetimes of the lowest lying states of nuclei belonging to the deformed regions around mass number A≃110 and A≃150. These regions were populated via spontaneous fission of 252Cf and the gamma radiation following the decay of excited states in the fission fragments was measured using 51 Gammasphere detectors coupled with 25 LaBr3:Ce detectors. A brief description of the acquisition system and some preliminary results from the fast-timing analysis of the fission fragment 100Zr are presented. The lifetime value of τ = 840(65) ps was found for the 2+ state in 100Zr consistent within one standard deviation of the adopted value with 791 +26 -35ps. This is associated with a quadrupole deformation parameter of 0.36(2) which is within one standard deviation of the literature value of 0.3556+82 -57.

CLUSTERING CORRELATIONS AND TRIAXIALITY IN THE sd-SHELL REGION

2011 ◽  
Vol 20 (04) ◽  
pp. 1046-1049 ◽  
Author(s):  
YASUTAKA TANIGUCHI ◽  
MASAAKI KIMURA ◽  
YOSHIKO KANADA-EN'YO ◽  
HISASHI HORIUCHI
Keyword(s):  
Excited States ◽  
Deformation Parameter ◽  
Cluster Structure ◽  
Quadrupole Deformation ◽  
Generator Coordinate Method ◽  
Generator Coordinate ◽  
Cluster Distance ◽  
Quadrupole Deformation Parameter ◽  
Different Shapes ◽  
Shell Region

Effects of cluster correlations on triaxiality have been studied using the antisymmetrized molecular dynamics. Low-lying states in 28 Si and 40 Ca are obtained by the the generator coordinate method (GCM), and the GCM basis are calculated by energy variations with constraints on quadrupole deformation parameter β and inter-cluster distance. The GCM obtain prolate superdeformed (SD) states in 28 Si and triaxial normal-deformed (ND) states in 40 Ca , which contain prolate α-24 Mg and triaxial α-36 Ar cluster structure components, respectively. Different shapes of prolate 24 Mg and oblate 36 Ar clusters cause difference of triaxiality of total systems. Cluster correlations which have oblate cluster enhance triaxiality in excited states.

Electron and ion irradiation-induced dissolution of mechanical twins in the intermetalic U3Si: An in situ HVEM study

1989 ◽  
Vol 47 ◽  
pp. 652-653
Author(s):  
Charles W. Allen ◽  
Robert C. Birtcher
Keyword(s):  
Elevated Temperatures ◽  
Ion Irradiation ◽  
Ion Beam ◽  
National Laboratory ◽  
Argonne National Laboratory ◽  
Heavy Ion ◽  
High Energy ◽  
Mechanical Twinning ◽  
In Situ Experiments

The uranium silicides, including U3Si, are under study as candidate low enrichment nuclear fuels. Ion beam simulations of the in-reactor behavior of such materials are performed because a similar damage structure can be produced in hours by energetic heavy ions which requires years in actual reactor tests. This contribution treats one aspect of the microstructural behavior of U3Si under high energy electron irradiation and low dose energetic heavy ion irradiation and is based on in situ experiments, performed at the HVEM-Tandem User Facility at Argonne National Laboratory. This Facility interfaces a 2 MV Tandem ion accelerator and a 0.6 MV ion implanter to a 1.2 MeV AEI high voltage electron microscope, which allows a wide variety of in situ ion beam experiments to be performed with simultaneous irradiation and electron microscopy or diffraction.At elevated temperatures, U3Si exhibits the ordered AuCu3 structure. On cooling below 1058 K, the intermetallic transforms, evidently martensitically, to a body-centered tetragonal structure (alternatively, the structure may be described as face-centered tetragonal, which would be fcc except for a 1 pet tetragonal distortion). Mechanical twinning accompanies the transformation; however, diferences between electron diffraction patterns from twinned and non-twinned martensite plates could not be distinguished.

Environmental cell studies of deformation and fracture

1990 ◽  
Vol 48 (4) ◽  
pp. 516-517
Author(s):  
H. K. Birnbaum ◽  
I. M. Robertson
Keyword(s):  
National Laboratory ◽  
Argonne National Laboratory ◽  
Damage Threshold ◽  
Chromatic Aberration ◽  
Good Choice ◽  
Point Of View ◽  
Deformation And Fracture ◽  
Environmental Cell ◽  
Gas Molecules ◽  
The University

Studies of the effects of hydrogen environments on the deformation and fracture of fcc, bcc and hep metals and alloys have been carried out in a TEM environmental cell. The initial experiments were performed in the environmental cell of the HVEM facility at Argonne National Laboratory. More recently, a dedicated environmental cell facility has been constructed at the University of Illinois using a JEOL 4000EX and has been used for these studies. In the present paper we will describe the general design features of the JEOL environmental cell and some of the observations we have made on hydrogen effects on deformation and fracture.The JEOL environmental cell is designed to operate at 400 keV and below; in part because of the available accelerating voltage of the microscope and in part because the damage threshold of most materials is below 400 keV. The gas pressure at which chromatic aberration due to electron scattering from the gas molecules becomes excessive does not increase rapidly with with accelerating voltage making 400 keV a good choice from that point of view as well. A series of apertures were placed above and below the cell to control the pressures in various parts of the column.

scholarly journals NEW STRUCTURES IN 178HF AND COULOMB EXCITATION OF ISOMERS

2011 ◽  
Vol 20 (02) ◽  
pp. 474-481 ◽  
Author(s):  
A.B. HAYES ◽  
D. CLINE ◽  
C. Y. WU ◽  
A.M. HURST ◽  
M.P. CARPENTER ◽  
...  
Keyword(s):  
Angular Momentum ◽  
Ground State ◽  
Coulomb Excitation ◽  
National Laboratory ◽  
Argonne National Laboratory ◽  
Particle Detector ◽  
Ground State Band ◽  
Rotational Bands ◽  
Coincidence Data ◽  
State Band

A 985 MeV 178 Hf beam was Coulomb excited by a 208 Pb target at the ATLAS accelerator of Argonne National Laboratory. Gammasphere and the CHICO particle detector recorded particle-γ coincidence data. The aim was to populate and determine the mechanism of previously observed Coulomb excitation of the Kπ = 6+ (t1/2 = 77 ns ), 8- (4 s ) and 16+ (31 y ) isomer bands. New rotational bands were identified including an aligned band which appears to mix with the ground-state band (GSB) and the γ-vibrational band above ~ 12 ħ of angular momentum. Newly observed γ-decay transitions into the three isomer bands may elucidate the K-mixing which allows Coulomb excitation of these isomer bands, but direct decays from the GSB into the 16+ isomer band have not yet been confirmed.

scholarly journals Dissolution Testing of a Metallic Waste Form in Chloride Brine

2006 ◽  
Vol 985 ◽  
Author(s):  
Dawn E. Janney
Keyword(s):  
National Laboratory ◽  
Bulk Composition ◽  
Argonne National Laboratory ◽  
Corrosion Products ◽  
Localized Corrosion ◽  
Waste Form ◽  
Ph Values ◽  
Surface Areas ◽  
Sample Edge ◽  
Static Immersion

AbstractArgonne National Laboratory has developed an electrometallurgical process for conditioning spent sodium-bonded metallic reactor fuel from the Experimental Breeder Reactor II (EBR-II). One waste stream from this process consists of a metal waste form (MWF) whose baseline composition is stainless steel alloyed with 15 wt% Zr (SS-15Zr) and whose microstructure is a eutectic intergrowth of iron solid solutions and Fe-Zr-Cr-Ni intermetallics. This paper reports scanning electron microscope (SEM) observations of corrosion products formed during static immersion tests in which coupons of surrogate MWF containing 10 wt% U (SS-15Zr-10U) were immersed in solutions with nominal pH values of 3 and 4 and 1000 ppm added chloride for 70 days at 50 °C. Although the majority of the surface areas of the coupons appear unchanged, linear areas with localized corrosion products apparently consisting of porous materials overlying corrosion-product-filled channels formed on both coupons, cross-cutting phase boundaries in the original eutectic microstructures. Many of the linear areas intersected the sample edge at notches present before the tests or followed linear flaws visible in pre-test images. Compositions of corrosion products differed significantly from the bulk composition, and the maximum observed concentration of U exceeded that reported in actinide-bearing phases in uncorroded surrogate MWF samples with comparable concentrations of U.

Synchrotron X-ray studies of metal-organic framework M2(2,5-dihydroxyterephthalate), M = (Mn, Co, Ni, Zn) (MOF74)

2012 ◽  
Vol 27 (4) ◽  
pp. 256-262 ◽  
Author(s):  
W. Wong-Ng ◽  
J. A. Kaduk ◽  
H. Wu ◽  
M. Suchomel
Keyword(s):  
Powder Diffraction ◽  
Metal Organic Framework ◽  
National Laboratory ◽  
Argonne National Laboratory ◽  
Lattice Parameter ◽  
X Ray ◽  
Metal Organic ◽  
Sorbent Materials ◽  
Diffraction Patterns ◽  
Unsaturated Metal Sites

M2(dhtp)·nH2O (M = Mn, Co, Ni, Zn; dhtp = 2,5-dihydroxyterephthalate), known as MOF74, is a family of excellent sorbent materials for CO2 that contains coordinatively unsaturated metal sites and a honeycomb-like structure featuring a broad one-dimensional channel. This paper describes the structural feature and provides reference X-ray powder diffraction patterns of these four isostructural compounds. The structures were determined using synchrotron diffraction data obtained at beam line 11-BM at the Advanced Photon Source (APS) in the Argonne National Laboratory. The samples were confirmed to be hexagonal R 3 (No. 148). From M = Mn, Co, Ni, to Zn, the lattice parameter a of MOF74 ranges from 26.131 73(4) Å to 26.5738(2) Å, c from 6.651 97(5) to 6.808 83(8) Å, and V ranges from 3948.08 Å3 to 4163.99 Å3, respectively. The four reference X-ray powder diffraction patterns have been submitted for inclusion in the Powder Diffraction File (PDF).

scholarly journals TRUEX Processing of Plutonium Analytical Solutions at Argonne National Laboratory

1997 ◽  
Vol 32 (1-4) ◽  
pp. 303-326 ◽  
Author(s):  
David B. Chamberlain ◽  
Cliff Conner ◽  
Joseph C. Hutter ◽  
Ralph A. Leonard ◽  
David G. Wygmans ◽  
...  
Keyword(s):  
Analytical Solutions ◽  
National Laboratory ◽  
Argonne National Laboratory
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