Anomalous complex shift of low‐frequency out‐of‐plane vibrations in aniline‐M van der Waals complexes (M=He, Ne, Ar)

1994 ◽  
Vol 100 (10) ◽  
pp. 7087-7092 ◽  
Author(s):  
Bruno Coutant ◽  
Philippe Brechignac
Keyword(s):  
Van Der Waals ◽  
Low Frequency ◽  
Van Der Waals Complexes ◽  
Out Of Plane

scholarly journals Consecutive Vibrational Redistribution and Predissociation Processes in s-Tetrazine–Argon Van Der Waals Complexes

1983 ◽  
Vol 2 (3-4) ◽  
pp. 125-135 ◽  
Author(s):  
J. J. F. Ramaekers ◽  
L. B. Krijnen ◽  
H. J. Lips ◽  
J. Langelaar ◽  
R. P. H. Rettschnick
Keyword(s):  
Decay Time ◽  
Van Der Waals ◽  
Stagnation Pressure ◽  
Van Der Waals Complexes ◽  
Supersonic Expansion ◽  
Vibrational Predissociation ◽  
Out Of Plane ◽  
Spectrally Resolved ◽  
Plane Mode

s-Tetrazine argon complexes T−Arn (n = 1, 2) are formed in a supersonic expansion of argon seeded with s-tetrazine. The expansion was conducted through a nozzle of 50 or 100 μm with an argon stagnation pressure between 1 and 1.5 bar. From spectrally resolved measurements it is clear that vibrational redistribution processes as well as vibrational predissociation processes take place after SVL excitation within the complex.From rise and decay time experiments it can be concluded, that after excitation of the 6a1 complex level, the above mentioned processes are consecutive and not parallel. It appears that the out of plane mode 16a couples with the Van der Waals stretching mode. The predissociation rate of the 16a2 complex is observed to be 2.3 × 109 s−1.

scholarly journals Non-linear Terahertz driving of plasma waves in layered cuprates

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Francesco Gabriele ◽  
Mattia Udina ◽  
Lara Benfatto
Keyword(s):  
Low Frequency ◽  
Plasma Waves ◽  
Meissner Effect ◽  
High Energy ◽  
Plasma Mode ◽  
Light Pulses ◽  
High Frequency Plasma ◽  
Non Linear ◽  
Out Of Plane ◽  
Layered Cuprates

AbstractThe hallmark of superconductivity is the rigidity of the quantum-mechanical phase of electrons, responsible for superfluid behavior and Meissner effect. The strength of the phase stiffness is set by the Josephson coupling, which is strongly anisotropic in layered cuprates. So far, THz light pulses have been used to achieve non-linear control of the out-of-plane Josephson plasma mode, whose frequency lies in the THz range. However, the high-energy in-plane plasma mode has been considered insensitive to THz pumping. Here, we show that THz driving of both low-frequency and high-frequency plasma waves is possible via a general two-plasmon excitation mechanism. The anisotropy of the Josephson couplings leads to markedly different thermal effects for the out-of-plane and in-plane response, linking in both cases the emergence of non-linear photonics across Tc to the superfluid stiffness. Our results show that THz light pulses represent a preferential knob to selectively drive phase excitations in unconventional superconductors.

scholarly journals How accurate is the determination of equilibrium structures for van der Waals complexes? The dimer N2O⋯CO as an example

2021 ◽  
Vol 154 (19) ◽  
pp. 194302
Author(s):  
Jean Demaison ◽  
Natalja Vogt ◽  
Yan Jin ◽  
Rizalina Tama Saragi ◽  
Marcos Juanes ◽  
...  
Keyword(s):  
Van Der Waals ◽  
Van Der Waals Complexes ◽  
Equilibrium Structures

scholarly journals Carrier-capture-assisted optoelectronics based on van der Waals materials to imitate medicine-acting metaplasticity

2021 ◽  
Vol 5 (1) ◽  
Author(s):  
Qianfan Nie ◽  
Caifang Gao ◽  
Feng-Shou Yang ◽  
Ko-Chun Lee ◽  
Che-Yi Lin ◽  
...  
Keyword(s):  
Weight Change ◽  
Synaptic Weight ◽  
Van Der Waals ◽  
Low Frequency ◽  
Photonic Devices ◽  
Frequency Noise ◽  
Carrier Capture ◽  
Electronic Engineering ◽  
Neural Simulation ◽  
Van Der Waals Materials

AbstractRecently, researchers have focused on optoelectronics based on two-dimensional van der Waals materials to realize multifunctional memory and neuron applications. Layered indium selenide (InSe) semiconductors satisfy various requirements as photosensitive channel materials, and enable the realization of intriguing optoelectronic applications. Herein, we demonstrate InSe photonic devices with different trends of output currents rooted in the carrier capture/release events under various gate voltages. Furthermore, we reported an increasing/flattening/decreasing synaptic weight change index (∆Wn) via a modulated gate electric field, which we use to imitate medicine-acting metaplasticity with effective/stable/ineffective features analogous to the synaptic weight change in the nervous system of the human brain. Finally, we take advantage of the low-frequency noise (LFN) measurements and the energy-band explanation to verify the rationality of carrier capture-assisted optoelectronics applied to neural simulation at the device level. Utilizing optoelectronics to simulate essential biomedical neurobehaviors, we experimentally demonstrate the feasibility and meaningfulness of combining electronic engineering with biomedical neurology.

scholarly journals Intercorrelated ferroelectrics in 2D van der Waals materials

2021 ◽  
Author(s):  
Yan Liang ◽  
Shiying Shen ◽  
Baibiao Huang ◽  
Ying Dai ◽  
Yandong Ma
Keyword(s):  
Van Der Waals ◽  
Out Of Plane ◽  
Fundamental Phenomenon ◽  
Van Der Waals Materials

2D intercorrelated ferroelectrics, exhibiting a coupled in-plane and out-of-plane ferroelectricity, is a fundamental phenomenon in the field of condensed-mater physics. The current research is based on the paradigm of bi-directional...

scholarly journals A van der Waals antiferromagnetic topological insulator with weak interlayer magnetic coupling

2020 ◽  
Vol 11 (1) ◽  
Author(s):  
Chaowei Hu ◽  
Kyle N. Gordon ◽  
Pengfei Liu ◽  
Jinyu Liu ◽  
Xiaoqing Zhou ◽  
...  
Keyword(s):  
Van Der Waals ◽  
Surface States ◽  
Magnetic Coupling ◽  
Anomalous Hall Effect ◽  
Saturation Field ◽  
Angle Resolved Photoemission Spectroscopy ◽  
Ideal System ◽  
Out Of Plane ◽  
Weak Interlayer ◽  
Quantum Phenomena

AbstractMagnetic topological insulators (TI) provide an important material platform to explore quantum phenomena such as quantized anomalous Hall effect and Majorana modes, etc. Their successful material realization is thus essential for our fundamental understanding and potential technical revolutions. By realizing a bulk van der Waals material MnBi4Te7 with alternating septuple [MnBi2Te4] and quintuple [Bi2Te3] layers, we show that it is ferromagnetic in plane but antiferromagnetic along the c axis with an out-of-plane saturation field of ~0.22 T at 2 K. Our angle-resolved photoemission spectroscopy measurements and first-principles calculations further demonstrate that MnBi4Te7 is a Z2 antiferromagnetic TI with two types of surface states associated with the [MnBi2Te4] or [Bi2Te3] termination, respectively. Additionally, its superlattice nature may make various heterostructures of [MnBi2Te4] and [Bi2Te3] layers possible by exfoliation. Therefore, the low saturation field and the superlattice nature of MnBi4Te7 make it an ideal system to investigate rich emergent phenomena.

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