scholarly journals Rare-earth tuned magnetism and magnetocaloric effects in double perovskites R2NiMnO6

Author(s):  
Anzar Ali ◽  
Kanika Pasrija ◽  
Gyaneshwar Sharma ◽  
Sanjeev Kumar ◽  
Yogesh Singh

Abstract We present a comprehensive experimental study of magnetization {\color {blue} ($2 < T < 300$~K, $1 < H < 8$~T)} and magnetocaloric effect in double perovskite materials $R_2$NiMnO$_6$ with $R =$ Pr, Nd, Sm, Gd, Tb, and Dy. While a paramagnetic to ferromagnetic transition, with T$_{\rm C}$ in the range $\sim 100 - 200~$K, is a common feature that can be attributed to the ordering of Mn$^{4+}$ and Ni$^{2+}$ magnetic moments, qualitatively distinct behavior depending on the choice of $R$ is observed at low temperatures. These low-temperature anomalies in magnetization are also manifest in the change in magnetic entropy, $-\Delta S_{M}$, whose sign depends on the choice of $R$. In order to understand these results, we present theoretical analysis based on mean-field approximation and Monte Carlo simulations on a minimal spin model. The model correctly captures the key features of the experimental observations.

2013 ◽  
Vol 2013 ◽  
pp. 1-6
Author(s):  
Hadey K. Mohamad

The magnetic properties of a ferrimagnetic mixed spin-3/2 and spin-5/2 Ising model with different anisotropies are investigated by using the mean-field approximation (MFA). In particular, the effect of magnetic anisotropies on the compensation phenomenon, acting on A-atoms and B-ones for the mixed-spin model, has been considered in a zero field. The free energy of a mixed-spin Ising ferrimagnetic system from MFA of the Hamiltonian is calculated. By minimizing the free energy, we obtain the equilibrium magnetizations and the compensation points. The phase diagram of the system in the anisotropy dependence of transition temperature has been discussed as well. Our results of this model predict the existence of many (two or three) compensation points in the ordered system on a simple cubic lattice.


Author(s):  
Robert H. Swendsen

Chapter 17 presented one example of a phase transition, the van der Waals gas. This chapter provides another, the Ising model, a widely studied model of phase transitions. We first give the solution for the Ising chain (one-dimensional model), including the introduction of the transfer matrix method. Higher dimensions are treated in the Mean Field Approximation (MFA), which is also extended to Landau theory. The Ising model is deceptively simple. It can be defined in a few words, but it displays astonishingly rich behavior. It originated as a model of ferromagnetism in which the magnetic moments were localized on lattice sites and had only two allowed values.


Author(s):  
Irina V. Tyulkina ◽  
Denis S. Goldobin ◽  
Lyudmila S. Klimenko ◽  
Igor S. Poperechny ◽  
Yuriy L. Raikher

The problem of magnetic transitions between the low-temperature (macrospin ordered) phases in two-dimensional XY arrays is addressed. The system is modelled as a plane structure of identical single-domain particles arranged in a square lattice and coupled by the magnetic dipole–dipole interaction; all the particles possess a strong easy-plane magnetic anisotropy. The basic state of the system in the considered temperature range is an antiferromagnetic (AF) stripe structure, where the macrospins (particle magnetic moments) are still involved in thermofluctuational motion: the superparamagnetic blocking T b temperature is lower than that ( T af ) of the AF transition. The description is based on the stochastic equations governing the dynamics of individual magnetic moments, where the interparticle interaction is added in the mean-field approximation. With the technique of a generalized Ott–Antonsen theory, the dynamics equations for the order parameters (including the macroscopic magnetization and the AF order parameter) and the partition function of the system are rigorously obtained and analysed. We show that inside the temperature interval of existence of the AF phase, a static external field tilted to the plane of the array is able to induce first-order phase transitions from AF to ferromagnetic state; the phase diagrams displaying stable and metastable regions of the system are presented. This article is part of the theme issue ‘Patterns in soft and biological matters’.


MRS Advances ◽  
2020 ◽  
Vol 5 (51) ◽  
pp. 2639-2645
Author(s):  
Banhi Chatterjee ◽  
Jindřich Kolorenč

AbstractWe investigate whether first-principles calculations with an improved description of electronic correlations can explain the large magnetic moments and the strong magnetocrystalline anisotropy in the ferromagnetic compound UGa2. The correlations are treated within a static mean-field approximation DFT+U combining the density functional theory (DFT) with an onsite Hubbard interaction U. We find that DFT+U improves the agreement of the magnetic moments with the experiment compared to DFT but worsens the theoretical description of the magnetocrystalline anisotropy.


1997 ◽  
Vol 50 (1) ◽  
pp. 123
Author(s):  
N. Ishii ◽  
H. Asami ◽  
W. Bentz ◽  
K. Yazaki

The nucleon and the delta are described as solutions of the relativistic Faddeev equation in the NJL model. We discuss the dependence of the baryon masses on the particular form of the four-Fermi interaction Lagrangians. Using the quark–diquark wave function, we calculate some bound state matrix elements such as the axial coupling constants, magnetic moments of the nucleon, the pion-nucleon sigma term and the proton-neutron mass difference. We also try to compare two pictures of describing the baryons in the NJL model, i.e. the mean-field approximation and the relativistic Faddeev approach. As a first step, we discuss how to improve the mean-field approximation by introducing an effective interaction. We also discuss the perturbative estimate of the deformation of the `vacuum" in the Faddeev approach.


2009 ◽  
Vol 20 (09) ◽  
pp. 1335-1343
Author(s):  
YUSUKE TOMITA ◽  
SHUNSUKE YANAI ◽  
HAJIME TAKAYAMA

Using the mean-field approximation, we study the reorientation transition in a discrete dipolar spin model. We array the d-dimensional spins in the d-1-dimensional hypercubic lattice points, and apply the magnetic anisotropy in the dth direction. Even though the long-range dipolar interaction is truncated to the nearest-neighbor interaction, the model exhibits the reorientation transition. The effects of the exchange interaction on the dipolar system are also studied.


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