Polarization control of laser-driven x-ray

Author(s):  
Shao-Wei Chou ◽  
Chun-Cheng Chu ◽  
Wei-Cheng Liu ◽  
Shih-Hung Chen ◽  
Ming-Wei Lin ◽  
...  
Keyword(s):  
X Ray ◽  
2021 ◽  
Vol 31 (1) ◽  
Author(s):  
Jun Miyawaki ◽  
Susumu Yamamoto ◽  
Yasuyuki Hirata ◽  
Masafumi Horio ◽  
Yoshihisa Harada ◽  
...  

AbstractAn X-ray is the well-known probe to examine structure of materials, including our own bodies. The X-ray beam, especially at the wavelength of nanometers, has also become significant to directly investigate electronic states of a sample. Such an X-ray is called a soft X-ray and polarization dependence of the light-matter interaction further unveils the microscopic properties, such as orbitals or spins of electrons. Generation of high brilliant beams of the polarized X-ray has linked to development of our experimental science, and it has been made by radiation from relativistic electrons at the synchrotron radiation facilities over the world. Recently, we constructed a new polarization-controlled X-ray source, the segmented cross undulator, at SPring-8, the largest synchrotron radiation facility in the world. The operation is based on interference of X-ray beams, which is sharply contrast to the conventional method of regulating electron trajectory by the mechanical control of magnets. The paradigm shift opened the measurement innovations and allowed us to design new experimental approaches to capture signals that have been hidden in materials. The present review describes the novel X-ray source with the principle of operation and the technical details of optimization. Examples of the frontier spectroscopies that use unique optical properties of the source are introduced, followed by the future prospects for next generation synchrotron radiation facilities.


2021 ◽  
Vol 4 (1) ◽  
Author(s):  
Markus Ilchen ◽  
Philipp Schmidt ◽  
Nikolay M. Novikovskiy ◽  
Gregor Hartmann ◽  
Patrick Rupprecht ◽  
...  

AbstractShort-wavelength free-electron lasers with their ultrashort pulses at high intensities have originated new approaches for tracking molecular dynamics from the vista of specific sites. X-ray pump X-ray probe schemes even allow to address individual atomic constituents with a ‘trigger’-event that preludes the subsequent molecular dynamics while being able to selectively probe the evolving structure with a time-delayed second X-ray pulse. Here, we use a linearly polarized X-ray photon to trigger the photolysis of a prototypical chiral molecule, namely trifluoromethyloxirane (C3H3F3O), at the fluorine K-edge at around 700 eV. The created fluorine-containing fragments are then probed by a second, circularly polarized X-ray pulse of higher photon energy in order to investigate the chemically shifted inner-shell electrons of the ionic mother-fragment for their stereochemical sensitivity. We experimentally demonstrate and theoretically support how two-color X-ray pump X-ray probe experiments with polarization control enable XFELs as tools for chiral recognition.


2016 ◽  
Vol 10 (7) ◽  
pp. 468-472 ◽  
Author(s):  
Alberto A. Lutman ◽  
James P. MacArthur ◽  
Markus Ilchen ◽  
Anton O. Lindahl ◽  
Jens Buck ◽  
...  

2015 ◽  
Author(s):  
E. A. Schneidmiller ◽  
M. V. Yurkov
Keyword(s):  
X Ray ◽  

2014 ◽  
Vol 21 (3) ◽  
pp. 466-472 ◽  
Author(s):  
Motohiro Suzuki ◽  
Yuichi Inubushi ◽  
Makina Yabashi ◽  
Tetsuya Ishikawa

A diamond phase retarder was applied to control the polarization states of a hard X-ray free-electron laser (XFEL) in the photon energy range 5–20 keV. The horizontal polarization of the XFEL beam generated from the planar undulators of the SPring-8 Angstrom Compact Free-Electron Laser (SACLA) was converted into vertical or circular polarization of either helicity by adjusting the angular offset of the diamond crystal from the exact Bragg condition. Using a 1.5 mm-thick crystal, a high degree of circular polarization, 97%, was obtained for 11.56 keV monochromatic X-rays, whereas the degree of vertical polarization was 67%, both of which agreed with the estimations including the energy bandwidth of the Si 111 beamline monochromator.


2016 ◽  
Vol 87 (8) ◽  
pp. 083113 ◽  
Author(s):  
G. Hartmann ◽  
A. O. Lindahl ◽  
A. Knie ◽  
N. Hartmann ◽  
A. A. Lutman ◽  
...  

2020 ◽  
Vol 27 (5) ◽  
pp. 1131-1140 ◽  
Author(s):  
Grant Cutler ◽  
Daniele Cocco ◽  
Elaine DiMasi ◽  
Simon Morton ◽  
Manuel Sanchez del Rio ◽  
...  

This paper presents a novel cantilevered liquid-nitrogen-cooled silicon mirror design for the first optic in a new soft X-ray beamline that is being developed as part of the Advanced Light Source Upgrade (ALS-U) (Lawrence Berkeley National Laboratory, USA). The beamline is optimized for photon energies between 400 and 1400 eV with full polarization control. Calculations indicate that, without correction, this design will achieve a Strehl ratio greater than 0.85 for the entire energy and polarization ranges of the beamline. With a correction achieved by moving the focus 7.5 mm upstream, the minimum Strehl ratio is 0.99. This design is currently the baseline plan for all new ALS-U insertion device beamlines.


2020 ◽  
Vol 47 (5) ◽  
pp. 0500015
Author(s):  
高张峰 Gao Zhangfeng ◽  
邓海啸 Deng Haixiao ◽  
刘波 Liu Bo ◽  
王东 Wang Dong

2011 ◽  
Vol 23 (3) ◽  
pp. 765-769
Author(s):  
耿会平 Geng Huiping ◽  
贾启卡 Jia Qika ◽  
李和廷 Li Heting

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