Abstract. Long-range-transported Canadian smoke layers in the stratosphere over
northern France were detected by three lidar systems in August 2017. The
peaked optical depth of the stratospheric smoke layer
exceeds 0.20 at 532 nm, which is
comparable with the simultaneous tropospheric aerosol optical depth. The
measurements of satellite sensors revealed that the observed stratospheric
smoke plumes were transported from Canadian wildfires after being lofted by
strong pyro-cumulonimbus. Case studies at two observation sites, Lille (lat
50.612, long 3.142, 60 m a.s.l.) and Palaiseau (lat 48.712, long 2.215,
156 m a.s.l.), are presented in detail. Smoke particle depolarization
ratios are measured at three wavelengths: over 0.20 at 355 nm, 0.18–0.19 at
532 nm, and 0.04–0.05 at 1064 nm. The high depolarization ratios and their
spectral dependence are possibly caused by the irregular-shaped aged smoke
particles and/or the mixing with dust particles. Similar results are found by
several European lidar stations and an explanation that can fully resolve
this question has not yet been found. Aerosol inversion based on lidar
2α+3β data derived a smoke effective radius of about
0.33 µm for both cases. The retrieved single-scattering albedo is
in the range of 0.8 to 0.9, indicating that the smoke plumes are absorbing.
The absorption can cause perturbations to the temperature vertical profile,
as observed by ground-based radiosonde, and it is also related to the ascent
of the smoke plumes when exposed in sunlight. A direct radiative
forcing (DRF) calculation is performed using the obtained optical and
microphysical properties. The calculation revealed that the smoke plumes in
the stratosphere can significantly reduce the radiation arriving at the
surface, and the heating rate of the plumes is about 3.5 K day−1. The
study provides a valuable characterization for aged smoke in the
stratosphere, but efforts are still needed in reducing and quantifying the
errors in the retrieved microphysical properties as well as radiative forcing
estimates.
Long-range-transported Canadian smoke plumes in the lower stratosphere over northern France
