Measurement and Evaluation of the Activation Resonance Integral of 146Nd, 148Nd, and 150Nd

1973 ◽  
Vol 51 (13) ◽  
pp. 1454-1462 ◽  
Author(s):  
M. D. Ricabarra ◽  
R. Turjanski ◽  
G. H. Ricabarra

Values of the ratio of the reduced activition resonance integral to the thermal cross section, I′/σ0, of 146Nd, 148Nd, and 150Nd were determined relative to gold by measuring cadmium ratios. A lithium-drifted germanium gamma-ray spectrometer was used to resolve the activities of the irradiated samples. The results are: for 146Nd I′/σ0 = 1.42 ± 0.10 and with an assumed σ0 = 1.4 b, I′ = 1.99 ± 0.20 b; for 148Nd I′/σ0 = 4.22 ± 0.14 and with an assumed σ0 = 2.5 b, I′ = 10.5 ± 0.9 b; and for 150Nd I′/σ0 = 13.7 ± 0.8 and with an assumed σ0 = 1.2 b, I′ = 16.4 ± 2.8 b.The resolved and unresolved epithermal integrals of 146Nd, 148Nd, and 150Nd were calculated. Values of the spectral correction factor were also calculated, so the resonance integral could be obtained from the epithermal integral data measured in our reactor spectrum in this experiment. Epithermal integral and spectral correction factors are listed in the text.The most important result of this investigation is that the 148Nd activation reduced resonance integral is about half of the previously recommended value and consequently the radiative width for 148Nd is also about half of the previously accepted value.

1961 ◽  
Vol 39 (8) ◽  
pp. 1184-1192 ◽  
Author(s):  
W. H. Walker ◽  
R. E. Green

Cadmium ratio measurements have been made in similar lattice positions in ZEEP with thin foils of Sm152 and gold. From a comparison of these cadmium ratios we find[Formula: see text]If gσ0 is assumed to be 212 ± 12 barns, then I′ = 3100 ± 200 barns. On the assumption that only one resonance in Sm152, at 8 ev, contributes appreciably to both the resonance integral and the thermal cross section, it follows that g = 1 and that Γ, the width at half-maximum of the total cross section resonance, is 193 ± 5 milli-ev. Because of the appreciable disagreement between this value and one reported earlier, a new time-of-flight measurement of the resonance parameters has been made, and it is reported in the next paper (Chrien 1961).


2019 ◽  
Vol 55 (11) ◽  
Author(s):  
T. Wright ◽  
S. Bennett ◽  
S. Heinitz ◽  
U. Köster ◽  
R. Mills ◽  
...  

Abstract.Ampoules of amorphous 99.5% enriched 13C were irradiated at the PF1b neutron beam line at the high-flux ILL research reactor in order to produce 14C atoms. The precise ratio of 14C/13C was subsequently measured at the VERA Accelerator Mass Spectrometer, allowing the 13C(n,$ \gamma$γ)14C thermal cross section to be accurately determined. This is the first measurement of this cross section at sub-eV energies via this technique and the result of $ 1.52 \pm 0.07$1.52±0.07 mb for the thermal cross section is in good agreement with other recent measurements which were performed via Prompt Gamma-ray Activation Analysis.


1970 ◽  
Vol 48 (20) ◽  
pp. 2362-2370 ◽  
Author(s):  
M. D. Ricabarra ◽  
R. Turjanski ◽  
G. H. Ricabarra

Values of the reduced activity resonance integral relative to the thermal cross section, I′/σ0, of 96Zr and 94Zr were determined relative to gold by measuring cadmium ratios in a reactor spectrum.Due to the anomalous characteristics of 96Zr a measurement of I′/σ0 for 96Zr was undertaken in a "quasi" thermal spectrum.96Zr and 94Zr activation resonance integrals were also determined by measuring the ratio of effective activation cross section of zirconium to 55Mn. International Atomic Energy Agency (IAEA) calibrated gamma sources were used to determine the samples' absolute activities. A lithium-drifted germanium γ-ray spectrometer was used in all cases to resolve the activities of the irradiated samples.The results for 96Zr are I′/σ0 = 879 ± 96, I′ = 4.97 ± 0.50 b, and σ0 = 5.7 ± 10 mb; for 94Zr I′/σ0 = 5.87 ± 0.05, I′ = 0.369 ± 0.037 b, and derived σ0 = 63 ± 8 mb.I′/σ0 for 96Zr is an order of magnitude or more greater than that found for stable isotopes. This suggests that almost 100% of the activation resonance integral of 96Zr consists of p-neutron captures. This fact is not consistent with the present knowledge of p-strength functions in the 90 < A < 130 mass region.


1960 ◽  
Vol 38 (1) ◽  
pp. 57-77 ◽  
Author(s):  
W. H. Walker ◽  
C. H. Westcott ◽  
T. K. Alexander

An apparatus is described which detects γ-rays emitted by a thin target placed in a well-denned neutron beam. It has been used to determine the Cd ratios of Au and Pu-240, from which the ratio of the resonance integral to the 2200 m/s cross section for radiative neutron capture in Pu-240 has been deduced, using Au as a reference standard. Using this ratio and previously measured values of the resonance integral of Pu-240 and its effective cross section in two positions in the NRX reactor, three separate estimates of the 2200 m/s cross section of Pu-240 have been made. The mean value is 270 ± 17 barns.In an auxiliary experiment to indicate the shape of the epithermal spectrum of the neutron beam, the activation Cd ratios of Mn and In were compared with that of Au. These results, combined with the known 2200 m/s capture cross sections of these nuclides, yield new values of the radiative capture resonance integrals for both Mn and In.


2002 ◽  
Vol 39 (sup2) ◽  
pp. 441-443 ◽  
Author(s):  
Nora Lía Maidana ◽  
Vito Roberto Vanin ◽  
Paulo Regmaldo Pascholati ◽  
Mauro da Silva Dias ◽  
Marina Fallone Koskinas

2014 ◽  
Vol 24 (3S2) ◽  
pp. 29-37
Author(s):  
Nguyen Van Do ◽  
Pham Duc Khue ◽  
Kim Tien Thanh ◽  
Nguyen Thi Hien ◽  
Kim Guinyun

Thermal neutron capture cross section and resonance integral for the $^{45}$Sc(n,$\gamma )^{46}$Sc reaction were measured by the activation method using the $^{197}$Au(n,$\gamma )^{198}$Au reaction as a single comparator. The high-purity scandium and gold samples with and without Cd cover with the thickness of 0.5 mm were irradiated in a pulsed neutron field of the 100 MeV electron linac of the Pohang Accelerator Laboratory (PAL). The induced activities in the activated foils were measured with a well calibrated HPGe detector. In order to improve the accuracy of the experimental results the effect of the non-ideal epithermal spectrum was taken in to account by determining the neutron spectrum shape factor ($\alpha )$, and the corrections for the thermal (G$_{th})$ and the resonance (G$_{epi})$ neutron self-shielding effects, the $\gamma $-ray attenuation (F$_{g})$ and the $\gamma $-ray coincidence summing effect were made. The thermal neutron cross-section for the $^{45}$Sc(n,$\gamma )^{46}$Sc reaction has been determined to be $\sigma _{o}$ = 27.6 $\pm $ 0.8 barn. By assuming the cadmium cut-off energy of 0.55 eV, the resonance integral for the $^{45}$Sc(n,$\gamma )^{46}$Sc reaction has been determined to be I$_{o}$ = 12.7 $\pm $ 0.7 bar. The present results are compared with the reference data and discussed.


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