The Application of the Combined Fission Matrix Theory in Fast Reactors

The combined fission matrix theory is a recently-developed hybrid neutron transport method. It features high efficiency, fidelity, and resolution whole-core transport calculation. The theory is based on the assumption that the fission matrix element ai,j is dominated by the property of the destination cell i. This assumption can be well explained in thermal reactors, and the combined fission matrix method has been validated in a series of thermal neutron system benchmarks. This work examines the feasibility of the combined fission matrix theory in fast reactors. The European Sodium Fast Reactor is used as the numerical benchmark. Compared to the Monte Carlo method, the combined fission matrix theory reports a 64 pcm keff difference and 8.3% 2D RMS error. The error is much larger than that in thermal reactors, and the correction ratio cannot significantly reduce the material discontinuity error in fast reactors. Overall, the combined fission matrix theory is more suited for thermal reactor transport calculations. Its application in fast reactors needs further developments.

Axial Shuffling on Pebble Bed Reactor using PRAKTIK 3D-HTR

With moving fuel, the pebble bed reactor (PBR) provides flexibility in the fuel management process due to the capability of online fuel refueling. This capability allows the reactor to operate at any given time without the need to shut down for refueling. The complexity of the depletion and burnup analysis requires the problem to be solved with sophisticated and robust computer codes that can handle the fuel shuffling. Since the fuel refueling is conducted from top to bottom, the shuffling and fuel movement in the axial direction should be modeled with acceptable accuracy. The purpose of the simulation is to obtain the equilibrium or even a critical condition of the reactor. The model used is based on the simplified pebble bed reactor with 200 MWt of thermal reactor power, 3 meters of core diameter, and 10 meters of core height. To model the axial shuffling on the reactor, a neutronic computer code called PRAKTIK 3D-HTR is used. The code utilizes the diffusion method in a three-dimensional cylindrical geometry to model the neutronic phenomena in the reactor. Moreover, PRAKTIK 3D-HTR is equipped with the burnup calculation and depletion analysis to be able to handle fuel movement. Finally, the axial shuffling mechanism is implemented using the once-through-then-out (OTTO) method. Implementing this method to the reactor, an equilibrium condition can be obtained. In this condition, the reactor condition in terms of criticality and flux shape is relatively constant. The critical condition can also be searched using PRAKTIK 3D-HTR to obtain the condition when the multiplication factor is equal to unity. The criticality search is conducted by changing the fuel movement speed. If the multiplication factor is less than 1, then the shuffling speed needs to be increased. Otherwise, if it is more than 1, the shuffling speed will be decreased.

Solar-thermal production of graphitic carbon and hydrogen via methane decomposition

This work reports a process in which concentrated irradiation from a simulated solar source converts methane to high-value graphitic carbon and hydrogen gas. Methane flows within a photo-thermal reactor through the pores of a thin substrate irradiated by several thousand suns at the focal peak. The methane decomposes primarily into hydrogen while depositing highly graphitic carbon that grows conformally over ligaments in the porous substrate. The localized solar heating of the porous substrate serves to capture the solid carbon into a readily extractable and useful form while maintaining active deposition site density with persistent catalytic activity. Results indicate a strong temperature dependence with high decomposition occurring in the central heating zone with concentration factors and temperatures above 1000 suns and 1300 K, respectively. Even with a large flow area through regions of lower irradiation and temperature, methane conversion and hydrogen yields of approx. 70\% are achieved, and 58\% of the inlet carbon is captured in graphitic form.

Solar-thermal production of graphitic carbon and hydrogen via methane decomposition

This work reports a process in which concentrated irradiation from a simulated solar source converts methane to high-value graphitic carbon and hydrogen gas. Methane flows within a photo-thermal reactor through the pores of a thin substrate irradiated by several thousand suns at the focal peak. The methane decomposes primarily into hydrogen while depositing highly graphitic carbon that grows conformally over ligaments in the porous substrate. The localized solar heating of the porous substrate serves to capture the solid carbon into a readily extractable and useful form while maintaining active deposition site density with persistent catalytic activity. Results indicate a strong temperature dependence with high decomposition occurring in the central heating zone with concentration factors and temperatures above 1000 suns and 1300 K, respectively. Even with a large flow area through regions of lower irradiation and temperature, methane conversion and hydrogen yields of approx. 70\% are achieved, and 58\% of the inlet carbon is captured in graphitic form.

Preliminary Neutronic Analysis of 150 MWt High-Temperature Gas Reactor to Produced Electricity in Small Area

There are small areas in Indonesia with insufficient electricity. High-Temperature Gas Reactor (HTGR) is a promising nuclear power plant that can be used in such areas as its capability to produce electricity and co-generation applications. A preliminary study on the neutronic aspect of the 150 MWt HTGR design is performed in this research. High Temperature Engineering Test Reactor (HTTR) is used as a basic model. The calculation was performed by Standard Thermal Reactor Analysis Code (SRAC) code, and Japanese Evaluated Nuclear Data Library (JENDL) 4.0 as nuclear data library. As a result, by increasing HTTR fuel assembly geometry to 1.5 times its original and using higher uranium enrichment, the reactor can be operated for five years.

Model and Results of a Study of the Synthesis of Finely Dispersed Silicon Carbide in an Electro-Thermal Reactor

The high-temperature synthesis of silicon carbide (SiC) in an electro-thermal fluidized bed reactor (EFB) has advantages, in comparison with the production in resistance furnaces, in terms of specific energy consumption, productivity and the level of automation of the technological process. The basic equations of the fluidized-bed carbide formation process model are presented in the paper. The results of calculating the synthesis parameters of finely dispersed SiC in the stationary operation mode of the EFB reactor are also presented. The correspondence between the calculated and available experimental results on the output of the final product is shown.

Dependence of N2O/NO Decomposition and Formation on Temperature and Residence Time in Thermal Reactor

Nitrogen dioxide (N2O) is a greenhouse gas that is harmful to the ozone layer and contributes to global warming. Many other nitrogen oxide emissions are controlled using the selective non-catalytic reaction (SNCR) process, but N2O reduction methods are few. To avoid future air pollution problems, N2O reduction from industrial sources is essential. In this study, a N2O decomposition and NO formation under an argon atmospheric N2O gas mixture were observed in a lab-scale SNCR system. The reaction rate and mechanism of N2O were calculated using a reaction path analyzer (CHEMKIN-PRO). The residence time of the gas mixture and the temperature in the reactor were set as experimental variables. The results confirmed that most of the N2O was converted to N2 and NO. The change in the N2O reduction rate increased with the residence time at 1013 and 1113 K, but decreased at 1213 K due to the inverse reaction. NO concentration increased with the residence time at 1013 and 1113 K, but decreased at 1213 K owing to the conversion of NO back to N2O.