Generation of 1-10 Ps Hard X-Rav Pulses for Time Resolved X-Ray Diffraction

1995 ◽  
Vol 39 ◽  
pp. 95-102
Author(s):  
P. Chen ◽  
I.V. Tomov ◽  
P. M. Rentzepis

We present a further improvement of our experimental system for the generation of hard x-ray pulses in the range 1-10 ps, A laser system based on a cw mode locked Nd:YLF laser is utilized for the emission of deep UV pulses at 193 nm with duration 1.5 ps and repetition rate of 300 Hz, This UV radiation is used to pump an x-ray diode which produces CuKa x-ray pulses with a duration shorter than 10 ps at 300 Hz.

2020 ◽  
Vol 27 (2) ◽  
pp. 371-377 ◽  
Author(s):  
Sota Takagi ◽  
Kouhei Ichiyanagi ◽  
Atsushi Kyono ◽  
Shunsuke Nozawa ◽  
Nobuaki Kawai ◽  
...  

The combination of high-power laser and synchrotron X-ray pulses allows us to observe material responses under shock compression and release states at the crystal structure on a nanosecond time scale. A higher-power Nd:glass laser system for laser shock experiments was installed as a shock driving source at the NW14A beamline of PF-AR, KEK, Japan. It had a maximum pulse energy of 16 J, a pulse duration of 12 ns and a flat-top intensity profile on the target position. The shock-induced deformation dynamics of polycrystalline aluminium was investigated using synchrotron-based time-resolved X-ray diffraction (XRD) under laser-induced shock. The shock pressure reached up to about 17 GPa with a strain rate of at least 4.6 × 107 s–1 and remained there for nanoseconds. The plastic deformation caused by the shock-wave loading led to crystallite fragmentation. The preferred orientation of the polycrystalline aluminium remained essentially unchanged during the shock compression and release processes in this strain rate. The newly established time-resolved XRD experimental system can provide useful information for understanding the complex dynamic compression and release behaviors.


2021 ◽  
Vol 28 (3) ◽  
Author(s):  
Matthias Rössle ◽  
Wolfram Leitenberger ◽  
Matthias Reinhardt ◽  
Azize Koç ◽  
Jan Pudell ◽  
...  

The time-resolved hard X-ray diffraction endstation KMC-3 XPP for optical pump/X-ray probe experiments at the electron storage ring BESSY II is dedicated to investigating the structural response of thin film samples and heterostructures after their excitation with ultrashort laser pulses and/or electric field pulses. It enables experiments with access to symmetric and asymmetric Bragg reflections via a four-circle diffractometer and it is possible to keep the sample in high vacuum and vary the sample temperature between ∼15 K and 350 K. The femtosecond laser system permanently installed at the beamline allows for optical excitation of the sample at 1028 nm. A non-linear optical setup enables the sample excitation also at 514 nm and 343 nm. A time-resolution of 17 ps is achieved with the `low-α' operation mode of the storage ring and an electronic variation of the delay between optical pump and hard X-ray probe pulse conveniently accesses picosecond to microsecond timescales. Direct time-resolved detection of the diffracted hard X-ray synchrotron pulses use a gated area pixel detector or a fast point detector in single photon counting mode. The range of experiments that are reliably conducted at the endstation and that detect structural dynamics of samples excited by laser pulses or electric fields are presented.


1994 ◽  
Vol 38 ◽  
pp. 21-33
Author(s):  
I. V. Tomov ◽  
P. Chen ◽  
P. M. Rentzepis

Abstract We report the development of a novel, pulsed x-ray diffraction system with picosecond time resolution. The system has been used to study the heat transport in gold, platinum and silicon crystals heated by 10 ps, 193 nm laser pulses. Further developments and applications of time resolved picosecond x-ray diffraction are discussed.


2014 ◽  
Vol 21 (5) ◽  
pp. 1090-1104 ◽  
Author(s):  
Karsten Holldack ◽  
Johannes Bahrdt ◽  
Andreas Balzer ◽  
Uwe Bovensiepen ◽  
Maria Brzhezinskaya ◽  
...  

Here the major upgrades of the femtoslicing facility at BESSY II (Khanet al., 2006) are reviewed, giving a tutorial on how elliptical-polarized ultrashort soft X-ray pulses from electron storage rings are generated at high repetition rates. Employing a 6 kHz femtosecond-laser system consisting of two amplifiers that are seeded by one Ti:Sa oscillator, the total average flux of photons of 100 fs duration (FWHM) has been increased by a factor of 120 to up to 106 photons s−1(0.1% bandwidth)−1on the sample in the range from 250 to 1400 eV. Thanks to a new beamline design, a factor of 20 enhanced flux and improvements of the stability together with the top-up mode of the accelerator have been achieved. The previously unavoidable problem of increased picosecond-background at higher repetition rates, caused by `halo' photons, has also been solved by hopping between different `camshaft' bunches in a dedicated fill pattern (`3+1 camshaft fill') of the storage ring. In addition to an increased X-ray performance at variable (linear and elliptical) polarization, the sample excitation in pump–probe experiments has been considerably extended using an optical parametric amplifier that supports the range from the near-UV to the far-IR regime. Dedicated endstations covering ultrafast magnetism experiments based on time-resolved X-ray circular dichroism have been either upgraded or, in the case of time-resolved resonant soft X-ray diffraction and reflection, newly constructed and adapted to femtoslicing requirements. Experiments at low temperatures down to 6 K and magnetic fields up to 0.5 T are supported. The FemtoSpeX facility is now operated as a 24 h user facility enabling a new class of experiments in ultrafast magnetism and in the field of transient phenomena and phase transitions in solids.


Author(s):  
P. Zhou ◽  
S. Kahle ◽  
U. Shymanovich ◽  
M. Nicoul ◽  
K. Sokolowski-Tinten ◽  
...  

2020 ◽  
Vol 91 (9) ◽  
pp. 095113
Author(s):  
Satoshi Okumura ◽  
Kentaro Uesugi ◽  
Tatsuya Sakamaki ◽  
Akio Goto ◽  
Masayuki Uesugi ◽  
...  

2014 ◽  
Vol 104 (2) ◽  
pp. 021906 ◽  
Author(s):  
H. A. Navirian ◽  
D. Schick ◽  
P. Gaal ◽  
W. Leitenberger ◽  
R. Shayduk ◽  
...  

2003 ◽  
Vol 780 ◽  
Author(s):  
C. Essary ◽  
V. Craciun ◽  
J. M. Howard ◽  
R. K. Singh

AbstractHf metal thin films were deposited on Si substrates using a pulsed laser deposition technique in vacuum and in ammonia ambients. The films were then oxidized at 400 °C in 300 Torr of O2. Half the samples were oxidized in the presence of ultraviolet (UV) radiation from a Hg lamp array. X-ray photoelectron spectroscopy, atomic force microscopy, and grazing angle X-ray diffraction were used to compare the crystallinity, roughness, and composition of the films. It has been found that UV radiation causes roughening of the films and also promotes crystallization at lower temperatures.Furthermore, increased silicon oxidation at the interface was noted with the UVirradiated samples and was shown to be in the form of a mixed layer using angle-resolved X-ray photoelectron spectroscopy. Incorporation of nitrogen into the film reduces the oxidation of the silicon interface.


2020 ◽  
Vol 4 (6) ◽  
Author(s):  
A. Mandal ◽  
B. J. Jensen ◽  
M. C. Hudspeth ◽  
S. Root ◽  
R. S. Crum ◽  
...  

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