scholarly journals German Spent Nuclear Fuel Legacy: Characteristics and High-Level Waste Management Issues

2013 ◽  
Vol 2013 ◽  
pp. 1-11 ◽  
Author(s):  
A. Schwenk-Ferrero
Keyword(s):  
Nuclear Fuel ◽  
Power Plants ◽  
Spent Nuclear Fuel ◽  
Fuel Cycle ◽  
Fission Products ◽  
High Level Waste ◽  
Minor Actinides ◽  
Spent Fuel ◽  
Cycle Simulation ◽  
High Level

Germany is phasing-out the utilization of nuclear energy until 2022. Currently, nine light water reactors of originally nineteen are still connected to the grid. All power plants generate high-level nuclear waste like spent uranium or mixed uranium-plutonium dioxide fuel which has to be properly managed. Moreover, vitrified high-level waste containing minor actinides, fission products, and traces of plutonium reprocessing loses produced by reprocessing facilities has to be disposed of. In the paper, the assessments of German spent fuel legacy (heavy metal content) and the nuclide composition of this inventory have been done. The methodology used applies advanced nuclear fuel cycle simulation techniques in order to reproduce the operation of the German nuclear power plants from 1969 till 2022. NFCSim code developed by LANL was adopted for this purpose. It was estimated that ~10,300 tonnes of unreprocessed nuclear spent fuel will be generated until the shut-down of the ultimate German reactor. This inventory will contain ~131 tonnes of plutonium, ~21 tonnes of minor actinides, and 440 tonnes of fission products. Apart from this, ca.215 tonnes of vitrified HLW will be present. As fission products and transuranium elements remain radioactive from 104to 106years, the characteristics of spent fuel legacy over this period are estimated, and their impacts on decay storage and final repository are discussed.

Integrated Model of Korean Spent Fuel and High Level Waste Disposal Options

2009 ◽  
Author(s):  
Yongsoo Hwang ◽  
Ian Miller
Keyword(s):  
Nuclear Fuel ◽  
Spent Nuclear Fuel ◽  
Fuel Cycle ◽  
Near Field ◽  
Integrated Model ◽  
High Level Waste ◽  
Spent Fuel ◽  
Parameter Uncertainties ◽  
Design Concepts ◽  
High Level

This paper describes an integrated model developed by the Korean Atomic Energy Research Institute (KAERI) to simulate options for disposal of spent nuclear fuel (SNF) and reprocessing products in South Korea. A companion paper (Hwang and Miller, 2009) describes a systems-level model of Korean options for spent nuclear fuel (SNF) management in the 21’st century. The model addresses alternative design concepts for disposal of SNF of different types (CANDU, PWR), high level waste, and fission products arising from a variety of alternative fuel cycle back ends. It uses the GoldSim software to simulate the engineered system, near-field and far-field geosphere, and biosphere, resulting in long-term dose predictions for a variety of receptor groups. The model’s results allow direct comparison of alternative repository design concepts, and identification of key parameter uncertainties and contributors to receptor doses.

scholarly journals Modern Methods of Radiochemical Reprocessing of Spent Nuclear Fuel

2019 ◽  
pp. 52-57
Author(s):  
T. Maltseva ◽  
А. Shyshuta ◽  
S. Lukashyn
Keyword(s):  
Nuclear Fuel ◽  
Large Scale ◽  
Spent Nuclear Fuel ◽  
Fuel Cycle ◽  
Fission Products ◽  
Purex Process ◽  
Minor Actinides ◽  
Closed Fuel Cycle ◽  
Highly Active ◽  
High Level

The paper is devoted to the history of development and the current state of technological and scientific advances in radiochemical reprocessing of spent nuclear fuel from water-cooled power reactors. Regarding spent nuclear fuel (SNF) of NPP power reactors, long-term energy security involves adopting a version of its radiochemical treatment, conditioning and recirculation. Recycling SNF is required for the implementation of a closed fuel cycle and the re-use of regeneration products as energy reactor fuels. The basis of modern technological schemes for the reprocessing of the spent nuclear fuel is the “Purex” process, developed since the 60s in the USA. The classic approach to the use of U and Pu nuclides contained in spent nuclear fuel is to separate them from fission products, re-enrich regenerated uranium and use plutonium for the production of mixed-oxide (MOX) fuel with depleted uranium. The modern reprocessing plants are able to deal with fuel with further increase of its main characteristics without significant changes in the initial project. In order to close the fuel cycle, it is needed to add the following technological steps: (1) removal of high-level and long-lived components and minor actinides; (2) return of actinides to the technological cycle; (3) safe disposal of unused components. Each of these areas is under investigation now. Several new promising multi-cycle hydrometallurgical processes based on the joint extraction of trivalent lanthanides and minor actinides with their subsequent separation have been developed. A number of promising materials is suggested to be potential matrices for the immobilization of high-level components of radioactive wastes. To improve the compatibility of fuel processing with the environment, non-aqueous technologies are being developed, for instance, pyro-chemical methods for the reprocessing of various types of highly active fuels based on metals, oxides, carbides, or nitrides. An important scientific and technological task under investigation is transmutation of actinides. The results of international large-scale experiments on the partitioning and transmutation of fuel with various minor actinides and long-lived fission products confirm the real possibility and expediency of closing the nuclear fuel cycle.

Centralization of Canada’s Spent Nuclear Fuel

2013 ◽  
Author(s):  
Krista Nicholson ◽  
John McDonald ◽  
Shona Draper ◽  
Brian M. Ikeda ◽  
Igor Pioro
Keyword(s):  
Nuclear Fuel ◽  
Site Selection ◽  
Nuclear Power ◽  
Power Plants ◽  
Spent Nuclear Fuel ◽  
Selection Process ◽  
Spent Fuel ◽  
Geologic Repository ◽  
Candu Reactors ◽  
High Level

Currently in Canada, spent fuel produced from Nuclear Power Plants (NPPs) is in the interim storage all across the country. It is Canada’s long-term strategy to have a national geologic repository for the disposal of spent nuclear fuel for CANada Deuterium Uranium (CANDU) reactors. The initial problem is to identify a means to centralize Canada’s spent nuclear fuel. The objective of this paper is to present a solution for the transportation issues that surround centralizing the waste. This paper reviews three major components of managing and the transporting of high-level nuclear waste: 1) site selection, 2) containment and 3) the proposed transportation method. The site has been selected based upon several factors including proximity to railways and highways. These factors play an important role in the site-selection process since the location must be accessible and ideally to be far from communities. For the containment of the spent fuel during transportation, a copper-shell container with a steel structural infrastructure was selected based on good thermal, structural, and corrosion resistance properties has been designed. Rail has been selected as the method of transporting the container due to both the potential to accommodate several containers at once and the extensive railway system in Canada.

Deep Geological Disposal of Spent Nuclear Fuel and High-Level Waste

2015 ◽  
pp. 367-399
Author(s):  
Želimir Veinović ◽  
Biljana Kovačević Zelić ◽  
Dubravko Domitrović
Keyword(s):  
Nuclear Fuel ◽  
Power Plants ◽  
Spent Nuclear Fuel ◽  
High Level Waste ◽  
Modern World ◽  
Geological Disposal ◽  
Long Term Storage ◽  
Deep Geological Disposal ◽  
Safety Cases ◽  
High Level

Management of Spent Nuclear Fuel (SF) and High-Level Waste (HLW) is one of the most important and challenging problems of the modern world. Otherwise a clean, cheap, constant, and secure way to produce electricity, nuclear power plants create large amounts of highly hazardous waste. Repositories—deep Geological Disposal Facilities (GDF)—for these types of waste must prevent radionuclides from reaching the biosphere, for up to 1,000,000 years, migrating from a deep (more than 300m), stable geological environment. At present, there are no operating GDFs for SF and/or HLW, mostly due to the difficult and complex task of preparing safety cases and licensing. The purpose of this chapter is to validate the generic R&D activities in this area and present alternative concepts of Radioactive Waste (RW) management: retrievability, reversibility, regional GDFs, long-term storage, and deep borehole disposal, demonstrating the main engineering tasks in solving the problem of RW management and disposal.

Characteristics and quantities of radioactive wastes

1986 ◽  
Vol 319 (1545) ◽  
pp. 5-16 ◽  
Keyword(s):  
Nuclear Power ◽  
Small Volume ◽  
Fuel Cycle ◽  
Residual Activity ◽  
Fission Products ◽  
High Level Waste ◽  
Spent Fuel ◽  
Fuel Cladding ◽  
Waste Streams ◽  
High Level

Estimates are given of the total quantities of radioactivity, and of the contribution from different isotopes to this total, arising in the wastes from civil nuclear power generation; the figures are normalized to 1 GW (e) y of power production. The intensity of the heat and y-radiation emitted by the spent fuel has been calculated, and their decrease as the radioactivity decays. Reprocessing the spent fuel results in 95% or more of the fission products and higher actinides being concentrated in a small volume of high-level, heat-emitting waste. The total decay curve of unreprocessed spent fuel or of the separated high-level waste is dominated by the decay of some fission products for a few hundred years and then by the decay of some actinide isotopes for some tens of thousands of years. The residual activity is compared with that of the original uranium ore. Some of the long-lived activity will appear in other waste streams, particularly on the fuel cladding, and the volumes and activities of these wastes arising in this country are recorded. The long-lived activity arising from reactor decommissioning will be small compared with the annual arisings from the fuel cycle.

Simulation and Analysis: The Dose Distribution of KBS-3 Spent Nuclear Fuel Canister by MCNP

2010 ◽  
Author(s):  
Bo Yang ◽  
He-xi Wu ◽  
Yi-bao Liu
Keyword(s):  
Cast Iron ◽  
Radioactive Waste ◽  
Nuclear Fuel ◽  
Nuclear Power ◽  
Power Plants ◽  
Spent Nuclear Fuel ◽  
Ductile Cast Iron ◽  
Nuclear Industry ◽  
Spent Fuel ◽  
High Level

With the sustained and rapid development of the nuclear power plants, the spent fuel which is produced by the nuclear power plants will be rapidly rising. Spent fuel is High-level radioactive waste and should be disposed safely, which is important for the environment of land, public safety and health of the nuclear industry, the major issues of sustainable development and it is also necessary part for the nuclear industry activities. It is important to study and resolve the high-level radioactive waste repository problem. Spent nuclear fuel is an important component in the radioactive waste, The KBS-3 canister for geological disposal of spent nuclear fuel in Sweden consists of a ductile cast iron insert and a copper shielding. The ductile cast iron insert provides the mechanical strength whereas the copper protects the canister from corrosion. The canister inserts material were referred to as I24, I25 and I26, Spent nuclear fuel make the repository in high radiant intensity. The radiation analysis of canister insert is important in canister transport, the dose analysis of repository and groundwater radiolysis. Groundwater radiolysis, which produces oxidants (H2O2 and O2), will break the deep repository for spent nuclear fuel. The dose distribution of canister surface with different kinds of canister inserts (I24, I25 and I26) is calculated by MCNP (Ref. 1). Analysing the calculation results, we offer a reference for selecting canister inserts material.

scholarly journals Natural Clay Minerals as a Starting Material for Matrices for the Immobilization of Radioactive Waste from Pyrochemical Processing of SNF

2021 ◽  
Vol 13 (19) ◽  
pp. 10780
Author(s):  
Anna V. Matveenko ◽  
Andrey P. Varlakov ◽  
Alexander A. Zherebtsov ◽  
Alexander V. Germanov ◽  
Ivan V. Mikheev ◽  
...  
Keyword(s):  
Radioactive Waste ◽  
Nuclear Fuel ◽  
Storage Time ◽  
Spent Nuclear Fuel ◽  
Fission Products ◽  
Bentonite Clay ◽  
Ceramic Materials ◽  
High Level Waste ◽  
Natural Clay ◽  
High Level

Pyrochemistry is a promising technology that can provide benefits for the safe reprocessing of relatively fresh spent nuclear fuel with a short storage time (3–5 years). The radioactive waste emanating from this process is an electrolyte (LiCl–KCl) mixture with fission products included. Such wastes are rarely immobilized through common matrices such as cement and glass. In this study, samples of ceramic materials, based on natural bentonite clay, were studied as matrices for radioactive waste in the form of LiCl–KCl eutectic. The phase composition of the samples, and their mechanical, hydrolytic, and radiation resistance were characterized. The possibility of using bentonite clay as a material for immobilizing high-level waste arising from pyrochemical processing of spent nuclear fuel is further discussed in this paper.

Transport of MOX Fuel: A Continuous Challenge

2010 ◽  
Author(s):  
Je´roˆme Galtier
Keyword(s):  
Nuclear Fuel ◽  
Nuclear Power ◽  
Power Plants ◽  
Spent Nuclear Fuel ◽  
Fuel Cycle ◽  
Nuclear Industry ◽  
Spent Fuel ◽  
Radioactive Materials ◽  
Mox Fuel ◽  
Increasing Demand

For 45 years TN International has been involved in the radioactive materials transportation field. Since the beginning the spent nuclear fuel transportation has been its core business. During all these years TN International, now part of AREVA, has been able to anticipate and fulfill the needs for new transport or storage casks designed to fit the nuclear industry evolutions. A whole fleet of casks able to transport all the materials of the nuclear fuel cycle has been developed. In this presentation we will focus on the casks used to transport the fresh and used MOX fuel. To transport the fresh MOX BWR and PWR fuel, TN International has developed two designs of casks: the MX 6 and the MX 8. These casks are and have been used to transport MOX fuel for French, German, Swiss and in a near future Japanese nuclear power plants. A complete set of baskets have been developed to optimize the loading in terms of integrated dose and also of course capacity. MOX used fuel has now its dedicated cask: the TN112 which certificate of approval has been obtained in July 2008. This cask is able to transport 12 MOX spent fuel elements with a short cooling time. The first loading of the cask has been performed in September 2008 in the EDF nuclear power plant of Saint-Laurent-des-Eaux. By its continuous involvement in the nuclear transportation field, TN International has been able to face the many challenges linked to the radioactive materials transportation especially talking of MOX fuel. TN International will also have to face the increasing demand linked to the nuclear renaissance.

scholarly journals Assessment of the Radiotoxicity of Spent Nuclear Fuel from a Fleet of PWR Reactors

Energies ◽  
2021 ◽  
Vol 14 (11) ◽  
pp. 3094
Author(s):  
Mikołaj Oettingen
Keyword(s):  
Isotopic Composition ◽  
Nuclear Fuel ◽  
Nuclear Power ◽  
Spent Nuclear Fuel ◽  
Fuel Cycle ◽  
Spent Fuel ◽  
Pressurized Water ◽  
Hybrid Energy ◽  
Cycle Simulation ◽  
Water Reactors

The paper presents the methodology for the estimation of the long-term actinides radiotoxicity and isotopic composition of spent nuclear fuel from a fleet of Pressurized Water Reactors (PWR). The methodology was developed using three independent numerical tools: the Spent Fuel Isotopic Composition database, the Nuclear Fuel Cycle Simulation System and the Monte Carlo Continuous Energy Burnup Code. The validation of spent fuel isotopic compositions obtained in the numerical modeling was performed using the available experimental data. A nuclear power embarking country benchmark was implemented for the verification and testing of the methodology. The obtained radiotoxicity reaches the reference levels at about 1.3 × 105 years, which is common for the PWR spent nuclear fuel. The presented methodology may be incorporated into a more versatile numerical tool for the modeling of hybrid energy systems.

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