Methods of femtosecond spectroscopy and time-resolved electron diffraction

Nanosilicon ◽  
2014 ◽  
pp. 579-614
Author(s):  
David C. Joy

Electron channeling patterns (ECP) were first found by Coates (1967) while observing a large bulk, single crystal of silicon in a scanning electron microscope. The geometric pattern visible was shown to be produced as a result of the changes in the angle of incidence, between the beam and the specimen surface normal, which occur when the sample is examined at low magnification (Booker, Shaw, Whelan and Hirsch 1967).A conventional electron diffraction pattern consists of an angularly resolved intensity distribution in space which may be directly viewed on a fluorescent screen or recorded on a photographic plate. An ECP, on the other hand, is produced as the result of changes in the signal collected by a suitable electron detector as the incidence angle is varied. If an integrating detector is used, or if the beam traverses the surface at a fixed angle, then no channeling contrast will be observed. The ECP is thus a time resolved electron diffraction effect. It can therefore be related to spatially resolved diffraction phenomena by an application of the concepts of reciprocity (Cowley 1969).


2015 ◽  
Vol 17 (6) ◽  
pp. 063004 ◽  
Author(s):  
Pengfei Zhu ◽  
Y Zhu ◽  
Y Hidaka ◽  
L Wu ◽  
J Cao ◽  
...  

2019 ◽  
Vol 74 (1) ◽  
pp. 24-29 ◽  
Author(s):  
Hyun Woo Kim ◽  
Kyu-Ha Jang ◽  
In Hyung Baek ◽  
Kitae Lee ◽  
Young Uk Jeong ◽  
...  

2019 ◽  
Vol 205 ◽  
pp. 09007
Author(s):  
Rui Xian ◽  
Stuart A. Hayes ◽  
Gaston Corthey ◽  
Carole A. Morrison ◽  
Alexander Marx ◽  
...  

The photochemistry of the triiodide anion has been investigated by femtosecond electron diffraction. The time-resolved signal indicates the presence of reaction products and large-amplitude coherent motion produced by participating species. To reconstruct the atomic detail of the reaction and identify the major contributors to the detected signal, we outline the approach for atomic-level reconstruction.


2009 ◽  
Vol 80 (2) ◽  
Author(s):  
B. Krenzer ◽  
A. Hanisch-Blicharski ◽  
P. Schneider ◽  
Th. Payer ◽  
S. Möllenbeck ◽  
...  

2009 ◽  
Vol 94 (10) ◽  
pp. 101910 ◽  
Author(s):  
M. Ligges ◽  
I. Rajkovic ◽  
P. Zhou ◽  
O. Posth ◽  
C. Hassel ◽  
...  

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