scholarly journals Radiative signature of absorbing aerosol over the eastern Mediterranean basin

2014 ◽  
Vol 14 (14) ◽  
pp. 7213-7231 ◽  
Author(s):  
A. K. Mishra ◽  
K. Klingmueller ◽  
E. Fredj ◽  
J. Lelieveld ◽  
Y. Rudich ◽  
...  
Keyword(s):  
Radiative Transfer ◽  
Eastern Mediterranean ◽  
Eastern Mediterranean Region ◽  
Radiation Budget ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Aerosol Layer ◽  
Marine Aerosol ◽  
Model Calculations ◽  
Aerosol Types

Abstract. The effects of absorbing aerosols on the atmospheric radiation budget and dynamics over the eastern Mediterranean region are studied using satellites and ground-based observations, and radiative transfer model calculations, under summer conditions. Climatology of aerosol optical depth (AOD), single scattering albedo (SSA) and size parameters were analyzed using multi-year (1999–2012) observations from Moderate Resolution Imaging Spectroradiometer (MODIS), Multi-angle Imaging SpectroRadiometer (MISR) and AErosol RObotic NETwork (AERONET). Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP)-derived aerosol vertical distributions and their classifications are used to calculate the AOD of four dominant aerosol types: dust, polluted dust, polluted continental, and marine aerosol over the region. The seasonal mean (June–August 2010) AODs are 0.22 ± 0.02, 0.11 ± 0.04, 0.10 ± 0.04 and 0.06 ± 0.01 for polluted dust, polluted continental, dust and marine aerosol, respectively. Changes in the atmospheric temperature profile as a function of absorbing aerosol loading were derived for the same period using observations from the AIRS satellite. We inferred heating rates in the aerosol layer of ~1.7 ± 0.8 K day−1 between 925 and 850 hPa, which is attributed to aerosol absorption of incoming solar radiation. Radiative transfer model (RTM) calculations show significant atmospheric warming for dominant absorbing aerosol over the region. A maximum atmospheric forcing of +16.7 ± 7.9 Wm−2 is calculated in the case of polluted dust, followed by dust (+9.4 ± 4.9 Wm−2) and polluted continental (+6.4 ± 4.5 Wm−2). RTM-derived heating rate profiles for dominant absorbing aerosol show warming of 0.1–0.9 K day−1 in the aerosol layer (< 3.0 km altitudes), which primarily depend on AODs of the different aerosol types. Diabatic heating due to absorbing aerosol stabilizes the lower atmosphere, which could significantly reduce the atmospheric ventilation. These conditions can enhance the "pollution pool" over the eastern Mediterranean.

scholarly journals Radiative signature of absorbing aerosol over the Eastern Mediterranean Basin

2014 ◽  
Vol 14 (2) ◽  
pp. 2403-2447 ◽  
Author(s):  
A. K. Mishra ◽  
K. Klingmueller ◽  
E. Fredj ◽  
J. Lelieveld ◽  
Y. Rudich ◽  
...  
Keyword(s):  
Eastern Mediterranean ◽  
Eastern Mediterranean Region ◽  
Lower Atmosphere ◽  
Radiation Budget ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Aerosol Layer ◽  
Marine Aerosol ◽  
Model Calculations ◽  
Aerosol Types

Abstract. The effects of absorbing aerosols on the atmospheric radiation budget and dynamics over the Eastern Mediterranean region are studied using satellites and ground-based observations, and model calculations, under summer conditions. Climatology of aerosol optical depth (AOD), single scattering albedo (SSA) and size parameters were analyzed using multi-year (1999–2012) observations from MODIS, MISR and AERONET. CALIOP-derived aerosol vertical distributions and their classifications are used to calculate the AOD of 4 dominant aerosol types: dust, polluted dust, polluted continental and marine aerosol over the region. The seasonal mean (June–August 2010) AODs are 0.22 ± 0.02, 0.11 ± 0.04, 0.10 ± 0.04 and 0.06 ± 0.01 for polluted dust, polluted continental, dust and marine aerosol, respectively. Changes in the atmospheric temperature profile as a function of absorbing aerosol loading were derived for the same period using observations from the AIRS satellite. We inferred heating rates in the aerosol layer of ~1.7 ± 0.8 K day−1 between 925 and 850 hPa, which is attributed to aerosol absorption of incoming solar radiation. Radiative transfer model (RTM) calculations show significant atmospheric warming for dominant absorbing aerosol over the region. A maximum atmospheric forcing of +16.5 ± 7.5 W m−2 is calculated in the case of polluted dust, followed by polluted continental (+7.6 ± 4.4 W m−2) and dust (+7.1 ± 4.3 W m−2). RTM-derived heating rate profiles for dominant absorbing aerosol show warming of 0.1–0.9 K day−1 in the aerosol layer (< 3.0 km altitudes), which primarily depend on AODs of the different aerosol types. Diabatic heating due to absorbing aerosol stabilizes the lower atmosphere, which could significantly reduce the atmospheric ventilation. These conditions can enhance the "pollution pool" over the Eastern Mediterranean.

Radiative forcing over the Arctic of aerosols from the August 2017 Canadian and Greenlandic wildfires

2021 ◽  
Author(s):  
Filippo Calì Quaglia ◽  
Daniela Meloni ◽  
Alcide Giorgio di Sarra ◽  
Tatiana Di Iorio ◽  
Virginia Ciardini ◽  
...  
Keyword(s):  
Radiative Transfer ◽  
Radiative Forcing ◽  
Solar Zenith Angle ◽  
Surface Albedo ◽  
High Arctic ◽  
The Arctic ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Aerosol Layer ◽  
Radiative Effect

&lt;p&gt;Extended and intense wildfires occurred in Northern Canada and, unexpectedly, on the Greenlandic West coast during summer 2017. The thick smoke plume emitted into the atmosphere was transported to the high Arctic, producing one of the largest impacts ever observed in the region. Evidence of Canadian and Greenlandic wildfires was recorded at the Thule High Arctic Atmospheric Observatory (THAAO, 76.5&amp;#176;N, 68.8&amp;#176;W, www.thuleatmos-it.it) by a suite of instruments managed by ENEA, INGV, Univ. of Florence, and NCAR. Ground-based observations of the radiation budget have allowed quantification of the surface radiative forcing at THAAO.&amp;#160;&lt;/p&gt;&lt;p&gt;Excess biomass burning chemical tracers such as CO, HCN, H2CO, C2H6, and NH3 were&amp;#160; measured in the air column above Thule starting from August 19 until August 23. The aerosol optical depth (AOD) reached a peak value of about 0.9 on August 21, while an enhancement of wildfire compounds was&amp;#160; detected in PM10. The measured shortwave radiative forcing was -36.7 W/m2 at 78&amp;#176; solar zenith angle (SZA) for AOD=0.626.&lt;/p&gt;&lt;p&gt;MODTRAN6.0 radiative transfer model (Berk et al., 2014) was used to estimate the aerosol radiative effect and the heating rate profiles at 78&amp;#176; SZA. Measured temperature profiles, integrated water vapour, surface albedo, spectral AOD and aerosol extinction profiles from CALIOP onboard CALIPSO were used as model input. The peak&amp;#160; aerosol heating rate (+0.5 K/day) was&amp;#160; reached within the aerosol layer between 8 and 12 km, while the maximum radiative effect (-45.4 W/m2) is found at 3 km, below the largest aerosol layer.&lt;/p&gt;&lt;p&gt;The regional impact of the event that occurred on August 21 was investigated using a combination of atmospheric radiative transfer modelling with measurements of AOD and ground surface albedo from MODIS. The aerosol properties used in the radiative transfer model were constrained by in situ measurements from THAAO. Albedo data over the ocean have been obtained from Jin et al. (2004). Backward trajectories produced through HYSPLIT simulations (Stein et al., 2015) were also employed to trace biomass burning plumes.&lt;/p&gt;&lt;p&gt;The radiative forcing efficiency (RFE) over land and ocean was derived, finding values spanning from -3 W/m2 to -132 W/m2, depending on surface albedo and solar zenith angle. The fire plume covered a vast portion of the Arctic, with large values of the daily shortwave RF (&lt; -50 W/m2) lasting for a few days. This large amount of aerosol is expected to influence cloud properties in the Arctic, producing significant indirect radiative effects.&lt;/p&gt;

scholarly journals Evaluation of Cirrus Parameterizations for Radiative Flux Computations in Climate Models Using TOVS–ScaRaB Satellite Observations

2007 ◽  
Vol 20 (17) ◽  
pp. 4459-4475 ◽  
Author(s):  
C. J. Stubenrauch ◽  
F. Eddounia ◽  
J. M. Edwards ◽  
A. Macke
Keyword(s):  
Optical Properties ◽  
Radiative Transfer ◽  
Climate Models ◽  
Radiative Flux ◽  
Satellite Observations ◽  
Radiation Budget ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Ice Crystal ◽  
Infrared Observation

Abstract Combined simultaneous satellite observations are used to evaluate the performance of parameterizations of the microphysical and optical properties of cirrus clouds used for radiative flux computations in climate models. Atmospheric and cirrus properties retrieved from Television and Infrared Observation Satellite (TIROS-N) Operational Vertical Sounder (TOVS) observations are given as input to the radiative transfer model developed for the Met Office climate model to simulate radiative fluxes at the top of the atmosphere (TOA). Simulated cirrus shortwave (SW) albedos are then compared to those retrieved from collocated Scanner for Radiation Budget (ScaRaB) observations. For the retrieval, special care has been given to angular direction models. Three parameterizations of cirrus ice crystal optical properties are represented in the Met Office radiative transfer model. These parameterizations are based on different physical approximations and different hypotheses on crystal habit. One parameterization assumes pristine ice crystals and two ice crystal aggregates. By relating the cirrus ice water path (IWP) retrieved from the effective infrared emissivity to the cirrus SW albedo, differences between the parameterizations are amplified. This study shows that pristine crystals seem to be plausible only for cirrus with IWP less than 30 g m−2. For larger IWP, ice crystal aggregates lead to cirrus SW albedos in better agreement with the observations. The data also indicate that climate models should allow the cirrus effective ice crystal diameter (De) to increase with IWP, especially in the range up to 30 g m−2. For cirrus with IWP less than 20 g m−2, this would lead to SW albedos that are about 0.02 higher than the ones of a constant De of 55 μm.

scholarly journals Aerosol trends as a potential driver of regional climate in the central United States: evidence from observations

2017 ◽  
Vol 17 (22) ◽  
pp. 13559-13572 ◽  
Author(s):  
Daniel H. Cusworth ◽  
Loretta J. Mickley ◽  
Eric M. Leibensperger ◽  
Michael J. Iacono
Keyword(s):  
United States ◽  
Radiative Transfer ◽  
Southeastern United States ◽  
Radiant Energy ◽  
Surface Radiation ◽  
Radiation Budget ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Clear Sky

Abstract. In situ surface observations show that downward surface solar radiation (SWdn) over the central and southeastern United States (US) has increased by 0.58–1.0 Wm−2 a−1 over the 2000–2014 time frame, simultaneously with reductions in US aerosol optical depth (AOD) of 3.3–5.0  ×  10−3 a−1. Establishing a link between these two trends, however, is challenging due to complex interactions between aerosols, clouds, and radiation. Here we investigate the clear-sky aerosol–radiation effects of decreasing US aerosols on SWdn and other surface variables by applying a one-dimensional radiative transfer to 2000–2014 measurements of AOD at two Surface Radiation Budget Network (SURFRAD) sites in the central and southeastern United States. Observations characterized as clear-sky may in fact include the effects of thin cirrus clouds, and we consider these effects by imposing satellite data from the Clouds and Earth's Radiant Energy System (CERES) into the radiative transfer model. The model predicts that 2000–2014 trends in aerosols may have driven clear-sky SWdn trends of +1.35 Wm−2 a−1 at Goodwin Creek, MS, and +0.93 Wm−2 a−1 at Bondville, IL. While these results are consistent in sign with observed trends, a cross-validated multivariate regression analysis shows that AOD reproduces 20–26 % of the seasonal (June–September, JJAS) variability in clear-sky direct and diffuse SWdn at Bondville, IL, but none of the JJAS variability at Goodwin Creek, MS. Using in situ soil and surface flux measurements from the Ameriflux network and Illinois Climate Network (ICN) together with assimilated meteorology from the North American Land Data Assimilation System (NLDAS), we find that sunnier summers tend to coincide with increased surface air temperature and soil moisture deficits in the central US. The 1990–2015 trends in the NLDAS SWdn over the central US are also of a similar magnitude to our modeled 2000–2014 clear-sky trends. Taken together, these results suggest that climate and regional hydrology in the central US are sensitive to the recent reductions in aerosol concentrations. Our work has implications for severely polluted regions outside the US, where improvements in air quality due to reductions in the aerosol burden could inadvertently pose an enhanced climate risk.

Process-Based Decomposition of the Decadal Climate Difference between 2002–13 and 1984–95

2017 ◽  
Vol 30 (12) ◽  
pp. 4373-4393 ◽  
Author(s):  
Xiaoming Hu ◽  
Yana Li ◽  
Song Yang ◽  
Yi Deng ◽  
Ming Cai
Keyword(s):  
Radiative Transfer ◽  
Heat Storage ◽  
Decomposition Analysis ◽  
Arctic Region ◽  
The Arctic ◽  
Radiative Transfer Model ◽  
Transfer Model ◽  
Model Calculations ◽  
Surface Warming ◽  
Decadal Climate

This study examines at the process level the climate difference between 2002–13 and 1984–95 in ERA-Interim. A linearized radiative transfer model is used to calculate the temperature change such that its thermal radiative cooling would balance the energy flux perturbation associated with the change of an individual process, without regard to what causes the change of the process in the first place. The global mean error of the offline radiative transfer model calculations is 0.09 K, which corresponds to the upper limit of the uncertainties from a single term in the decomposition analysis. The process-based decomposition indicates that the direct effect of the increase of CO2 (0.15 K) is the largest contributor to the global warming between the two periods (about 0.27 K). The second and third largest contributors are the cloud feedback (0.14 K) and the combined effect of the oceanic heat storage and evaporation terms (0.11 K), respectively. The largest warming associated with the oceanic heat storage term is found in the tropical Pacific and Indian Oceans, with relatively weaker warming over the tropical Atlantic Ocean. The increase in atmospheric moisture adds another 0.1 K to the global surface warming, but the enhancement in tropical convections acts to reduce the surface warming by 0.17 K. The ice-albedo and atmospheric dynamical feedbacks are the two leading factors responsible for the Arctic polar warming amplification (PWA). The increase of atmospheric water vapor over the Arctic region also contributes substantially to the Arctic PWA pattern.

scholarly journals Parameterizing radiative transfer to convert MAX-DOAS dSCDs into near-surface box-averaged mixing ratios

2013 ◽  
Vol 6 (6) ◽  
pp. 1521-1532 ◽  
Author(s):  
R. Sinreich ◽  
A. Merten ◽  
L. Molina ◽  
R. Volkamer
Keyword(s):  
Boundary Layer ◽  
Radiative Transfer ◽  
Mexico City ◽  
Vertical Gradient ◽  
Radiative Transfer Model ◽  
Optical Absorption Spectroscopy ◽  
Transfer Model ◽  
Model Calculations ◽  
Near Surface ◽  
Mixing Ratios

Abstract. We present a novel parameterization method to convert multi-axis differential optical absorption spectroscopy (MAX-DOAS) differential slant column densities (dSCDs) into near-surface box-averaged volume mixing ratios. The approach is applicable inside the planetary boundary layer under conditions with significant aerosol load, and builds on the increased sensitivity of MAX-DOAS near the instrument altitude. It parameterizes radiative transfer model calculations and significantly reduces the computational effort, while retrieving ~ 1 degree of freedom. The biggest benefit of this method is that the retrieval of an aerosol profile, which usually is necessary for deriving a trace gas concentration from MAX-DOAS dSCDs, is not needed. The method is applied to NO2 MAX-DOAS dSCDs recorded during the Mexico City Metropolitan Area 2006 (MCMA-2006) measurement campaign. The retrieved volume mixing ratios of two elevation angles (1° and 3°) are compared to volume mixing ratios measured by two long-path (LP)-DOAS instruments located at the same site. Measurements are found to agree well during times when vertical mixing is expected to be strong. However, inhomogeneities in the air mass above Mexico City can be detected by exploiting the different horizontal and vertical dimensions probed by the MAX-DOAS and LP-DOAS instruments. In particular, a vertical gradient in NO2 close to the ground can be observed in the afternoon, and is attributed to reduced mixing coupled with near-surface emission inside street canyons. The existence of a vertical gradient in the lower 250 m during parts of the day shows the general challenge of sampling the boundary layer in a representative way, and emphasizes the need of vertically resolved measurements.

scholarly journals A neural network radiative transfer model approach applied to the Tropospheric Monitoring Instrument aerosol height algorithm

2019 ◽  
Vol 12 (12) ◽  
pp. 6619-6634 ◽  
Author(s):  
Swadhin Nanda ◽  
Martin de Graaf ◽  
J. Pepijn Veefkind ◽  
Mark ter Linden ◽  
Maarten Sneep ◽  
...  
Keyword(s):  
Neural Network ◽  
Radiative Transfer ◽  
European Space Agency ◽  
Forward Model ◽  
Radiative Transfer Model ◽  
Retrieval Algorithm ◽  
Transfer Model ◽  
Aerosol Layer ◽  
Layer Height ◽  
Monitoring Instrument

Abstract. To retrieve aerosol properties from satellite measurements of the oxygen A-band in the near-infrared, a line-by-line radiative transfer model implementation requires a large number of calculations. These calculations severely restrict a retrieval algorithm's operational capability as it can take several minutes to retrieve the aerosol layer height for a single ground pixel. This paper proposes a forward modelling approach using artificial neural networks to speed up the retrieval algorithm. The forward model outputs are trained into a set of neural network models to completely replace line-by-line calculations in the operational processor. Results comparing the forward model to the neural network alternative show an encouraging outcome with good agreement between the two when they are applied to retrieval scenarios using both synthetic and real measured spectra from TROPOMI (TROPOspheric Monitoring Instrument) on board the European Space Agency (ESA) Sentinel-5 Precursor mission. With an enhancement of the computational speed by 3 orders of magnitude, TROPOMI's operational aerosol layer height processor is now able to retrieve aerosol layer heights well within operational capacity.

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