scholarly journals Constraining the aerosol influence on cloud liquid water path

2019 ◽  
Vol 19 (8) ◽  
pp. 5331-5347 ◽  
Author(s):  
Edward Gryspeerdt ◽  
Tom Goren ◽  
Odran Sourdeval ◽  
Johannes Quaas ◽  
Johannes Mülmenstädt ◽  
...  

Abstract. The impact of aerosols on cloud properties is one of the largest uncertainties in the anthropogenic radiative forcing of the climate. Significant progress has been made in constraining this forcing using observations, but uncertainty remains, particularly in the magnitude of cloud rapid adjustments to aerosol perturbations. Cloud liquid water path (LWP) is the leading control on liquid-cloud albedo, making it important to observationally constrain the aerosol impact on LWP. Previous modelling and observational studies have shown that multiple processes play a role in determining the LWP response to aerosol perturbations, but that the aerosol effect can be difficult to isolate. Following previous studies using mediating variables, this work investigates use of the relationship between cloud droplet number concentration (Nd) and LWP for constraining the role of aerosols. Using joint-probability histograms to account for the non-linear relationship, this work finds a relationship that is broadly consistent with previous studies. There is significant geographical variation in the relationship, partly due to role of meteorological factors (particularly relative humidity). The Nd–LWP relationship is negative in the majority of regions, suggesting that aerosol-induced LWP reductions could offset a significant fraction of the instantaneous radiative forcing from aerosol–cloud interactions (RFaci). However, variations in the Nd–LWP relationship in response to volcanic and shipping aerosol perturbations indicate that the Nd–LWP relationship overestimates the causal Nd impact on LWP due to the role of confounding factors. The weaker LWP reduction implied by these “natural experiments” means that this work provides an upper bound to the radiative forcing from aerosol-induced changes in the LWP.

2018 ◽  
Author(s):  
Edward Gryspeerdt ◽  
Tom Goren ◽  
Odran Sourdeval ◽  
Johannes Quaas ◽  
Johannes Mülmenstädt ◽  
...  

Abstract. The impact of aerosols on cloud properties is one of the largest uncertainties in the anthropogenic radiative forcing of the climate. In recent years, significant progress has been made in constraining this forcing using observations, but uncertainty still remains, particularly in the adjustments of cloud properties to aerosol perturbations. Cloud liquid water path (LWP) is the leading control on liquid-cloud albedo, making it important to observationally constrain the aerosol impact LWP. Previous modelling and observational studies have shown that multiple processes play a role in determining the LWP response to aerosol perturbations, but that the aerosol effect can be difficult to isolate. Following previous studies using mediating variables, this work investigates use of the relationship between cloud droplet number concentration (Nd) and LWP for constraining the role of aerosols. Using joint probability histograms to account for the non-linear relationship, this work finds a relationship that is broadly consistent with previous studies. There is significant geographical variation in the relationship, partly due to role of meteorological factors (particularly relative humidity) in the relationship. However, the Nd-LWP relationship is negative in the majority of regions, suggesting that aerosol induced LWP reductions could offset a significant fraction of the radiative forcing from aerosol-cloud interactions (RFaci). However, variations in the Nd-LWP relationship in response to volcanic and shipping aerosol perturbations indicate that the Nd-LWP relationship overestimates the Nd impact on LWP. As such, the estimate of LWP changes due to aerosol in this work provides an upper bound to the radiative forcing from aerosol-induced changes in the LWP.


2008 ◽  
Vol 8 (6) ◽  
pp. 20399-20425 ◽  
Author(s):  
H. Guo ◽  
Y. Liu ◽  
P. H. Daum ◽  
X. Zeng ◽  
X. Li ◽  
...  

Abstract. We undertook three-dimensional numerical studies of a marine stratus deck under a strong inversion using an interactive shortwave- and longwave-radiation module. A suite of sensitivity tests were conducted to address the effects of model resolution on entrainment (inversion heights), cloud-radiation interactions, and cloud radiative-forcings by varying model horizontal resolution only, varying vertical resolution only, and varying horizontal- and vertical-resolution simultaneously but with a fixed aspect ratio of 2.5. Our results showed that entrainment (inversion height) is more sensitive to vertical- than to horizontal-resolution. A vertical resolution finer than 40 m can simulate spatial- and temporal-variations in the inversion height well. The inversion height decreases with increasing vertical resolution, but tends to increase with increasing horizontal resolution. Cloud liquid water path doubles after refining both the vertical- and horizontal-resolution by a factor of four. This doubling is associated with a positive feedback between cloud water and cloud top radiative cooling, which amplifies small differences initiated by changes in the model resolution. The magnitude of the cloud radiative-forcing tends to increase with increasing model resolution, mainly attributable to the increase in the cloud liquid water path. Shortwave radiative forcing is dominant, and more sensitive to model resolution than the longwave counterpart.


2015 ◽  
Vol 54 (8) ◽  
pp. 1809-1825 ◽  
Author(s):  
Yaodeng Chen ◽  
Hongli Wang ◽  
Jinzhong Min ◽  
Xiang-Yu Huang ◽  
Patrick Minnis ◽  
...  

AbstractAnalysis of the cloud components in numerical weather prediction models using advanced data assimilation techniques has been a prime topic in recent years. In this research, the variational data assimilation (DA) system for the Weather Research and Forecasting (WRF) Model (WRFDA) is further developed to assimilate satellite cloud products that will produce the cloud liquid water and ice water analysis. Observation operators for the cloud liquid water path and cloud ice water path are developed and incorporated into the WRFDA system. The updated system is tested by assimilating cloud liquid water path and cloud ice water path observations from Global Geostationary Gridded Cloud Products at NASA. To assess the impact of cloud liquid/ice water path data assimilation on short-term regional numerical weather prediction (NWP), 3-hourly cycling data assimilation and forecast experiments with and without the use of the cloud liquid/ice water paths are conducted. It is shown that assimilating cloud liquid/ice water paths increases the accuracy of temperature, humidity, and wind analyses at model levels between 300 and 150 hPa after 5 cycles (15 h). It is also shown that assimilating cloud liquid/ice water paths significantly reduces forecast errors in temperature and wind at model levels between 300 and 150 hPa. The precipitation forecast skills are improved as well. One reason that leads to the improved analysis and forecast is that the 3-hourly rapid update cycle carries over the impact of cloud information from the previous cycles spun up by the WRF Model.


2001 ◽  
Vol 106 (D13) ◽  
pp. 14485-14500 ◽  
Author(s):  
James C. Liljegren ◽  
Eugene E. Clothiaux ◽  
Gerald G. Mace ◽  
Seiji Kato ◽  
Xiquan Dong

2004 ◽  
Vol 17 (24) ◽  
pp. 4760-4782 ◽  
Author(s):  
Manajit Sengupta ◽  
Eugene E. Clothiaux ◽  
Thomas P. Ackerman

Abstract A 4-yr climatology (1997–2000) of warm boundary layer cloud properties is developed for the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) Program Southern Great Plains (SGP) site. Parameters in the climatology include cloud liquid water path, cloud-base height, and surface solar flux. These parameters are retrieved from measurements produced by a dual-channel microwave radiometer, a millimeter-wave cloud radar, a micropulse lidar, a Belfort ceilometer, shortwave radiometers, and atmospheric temperature profiles amalgamated from multiple sources, including radiosondes. While no significant interannual differences are observed in the datasets, there are diurnal variations with nighttime liquid water paths consistently higher than daytime values. The summer months of June, July, and August have the lowest liquid water paths and the highest cloud-base heights. Model outputs of cloud liquid water paths from the European Centre for Medium-Range Weather Forecasts (ECMWF) model and the Eta Model for 104 model output location time series (MOLTS) stations in the environs of the SGP central facility are compared to observations. The ECMWF and MOLTS median liquid water paths are greater than 3 times the observed values. The MOLTS data show lower liquid water paths in summer, which is consistent with observations, while the ECMWF data exhibit the opposite tendency. A parameterization of normalized cloud forcing that requires only cloud liquid water path and solar zenith angle is developed from the observations. The parameterization, which has a correlation coefficient of 0.81 with the observations, provides estimates of surface solar flux that are comparable to values obtained from explicit radiative transfer calculations based on plane-parallel theory. This parameterization is used to estimate the impact on the surface solar flux of differences in the liquid water paths between models and observations. Overall, there is a low bias of 50% in modeled normalized cloud forcing resulting from the excess liquid water paths in the two models. Splitting the liquid water path into two components, cloud thickness and liquid water content, shows that the higher liquid water paths in the model outputs are primarily a result of higher liquid water contents, although cloud thickness may a play a role, especially for the ECMWF model results.


2008 ◽  
Vol 21 (8) ◽  
pp. 1721-1739 ◽  
Author(s):  
Christopher W. O’Dell ◽  
Frank J. Wentz ◽  
Ralf Bennartz

Abstract This work describes a new climatology of cloud liquid water path (LWP), termed the University of Wisconsin (UWisc) climatology, derived from 18 yr of satellite-based passive microwave observations over the global oceans. The climatology is based on a modern retrieval methodology applied consistently to the Special Sensor Microwave Imager (SSM/I), the Tropical Rainfall Measuring Mission (TRMM) Microwave Imager (TMI), and the Advanced Microwave Scanning Radiometer (AMSR) for Earth Observing System (EOS) (AMSR-E) microwave sensors on eight different satellite platforms, beginning in 1988 and continuing through 2005. It goes beyond previously published climatologies by explicitly solving for the diurnal cycle of cloud liquid water by providing statistical error estimates, and includes a detailed discussion of possible systematic errors. A novel methodology for constructing the climatology is used in which a mean monthly diurnal cycle as well as monthly means of the liquid water path are derived simultaneously from the data on a 1° grid; the methodology also produces statistical errors for these quantities, which decrease toward the end of the time record as the number of observations increases. The derived diurnal cycles are consistent with previous findings in the tropics, but are also derived for higher latitudes and contain more information than in previous studies. The new climatology exhibits differences with previous observationally based climatologies and is found to be more consistent with the 40-yr ECMWF Re-Analysis (ERA-40) than are the previous climatologies. Potential systematic errors of the order of 15%–30% or higher exist in the LWP climatology. A previously unexplored source of systematic error is caused by the assumption that all microwave-based retrievals of LWP must make regarding the partitioning of cloud water and rainwater, which cannot be determined using microwave observations alone. The potentially large systematic errors that result may hamper the usefulness of microwave-based climatologies of both cloud liquid water and especially rain rate, particularly in certain regions of the tropics and midlatitudes where the separation of rain from liquid cloud water is most critical.


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