scholarly journals Response of dust emissions in southwestern North America to 21st century trends in climate, CO<sub>2</sub> fertilization, and land use: Implications for air quality

2020 ◽  
Author(s):  
Yang Li ◽  
Loretta J. Mickley ◽  
Jed O. Kaplan

Abstract. Climate models predict a shift toward warmer and drier environments in southwestern North America. However, the projected dust trends under climate change are sometimes contradictory. Here we link a dynamic vegetation model (LPJ-LMfire) to a chemical transport model (GEOS-Chem) to assess the impacts of future changes in climate, CO2 fertilization, and land use practices on dust mobilization, and to investigate the consequences for surface air quality. Considering all factors in the most extreme future warming scenario, we find decreasing trends of fine dust emissions over Arizona and New Mexico but increasing emissions along Mexico's northern border in the late-21st century during springtime, the season of maximum dust emissions. These trends result from more densely vegetated environments in the arid southwestern U.S. under future climate, but sparser vegetation in northern Mexico. The two main drivers of dust trends in this region – CO2 fertilization and land use intensification – play opposing roles, with the first driver enhancing vegetation and thus decreasing dust in the southwestern U.S. and the second driver increasing dust in northern Mexico. In the absence of CO2 fertilization, the RCP8.5 scenario places an upper bound on increases in dust, with elevated concentrations widespread over the southwestern North America by 2100 in spring, especially in southeastern New Mexico (up to ~2.0 µg m−3) and along the border between New Mexico and Mexico (up to ~2.5 µg m−3).

2021 ◽  
Vol 21 (1) ◽  
pp. 57-68
Author(s):  
Yang Li ◽  
Loretta J. Mickley ◽  
Jed O. Kaplan

Abstract. Climate models predict a shift toward warmer and drier environments in southwestern North America. The consequences of such a shift for dust mobilization and dust concentration are unknown, but they could have large implications for human health, given the connections between dust inhalation and disease. Here we link a dynamic vegetation model (LPJ-LMfire) to a chemical transport model (GEOS-Chem) to assess the impacts of future changes in three factors – climate, CO2 fertilization, and land use practices – on vegetation in this region. From there, we investigate the impacts of changing vegetation on dust mobilization and assess the net effect on fine dust concentration (defined as dust particles less than 2.5 µm in diameter) on surface air quality. We find that surface temperatures in southwestern North America warm by 3.3 K and precipitation decreases by nearly 40 % by 2100 in the most extreme warming scenario (RCP8.5; RCP refers to Representative Concentration Pathway) in spring (March, April, and May) – the season of greatest dust emissions. Such conditions reveal an increased vulnerability to drought and vegetation die-off. Enhanced CO2 fertilization, however, offsets the modeled effects of warming temperatures and rainfall deficit on vegetation in some areas of the southwestern US. Considering all three factors in the RCP8.5 scenario, dust concentrations decrease over Arizona and New Mexico in spring by the late 21st century due to greater CO2 fertilization and a more densely vegetated environment, which inhibits dust mobilization. Along Mexico's northern border, dust concentrations increase as a result of the intensification of anthropogenic land use. In contrast, when CO2 fertilization is not considered in the RCP8.5 scenario, vegetation cover declines significantly across most of the domain by 2100, leading to widespread increases in fine dust concentrations, especially in southeastern New Mexico (up to ∼ 2.0 µg m−3 relative to the present day) and along the border between New Mexico and Mexico (up to ∼ 2.5 µg m−3). Our results have implications for human health, especially for the health of the indigenous people who make up a large percentage of the population in this region.


2021 ◽  
Author(s):  
Hongbin Yu ◽  
Qian Tan ◽  
Lillian Zhou ◽  
Yaping Zhou ◽  
Huisheng Bian ◽  
...  

Abstract. This study characterizes a massive African dust intrusion into the Caribbean Basin and southern U.S. in June 2020, which is nicknamed the Godzilla dust plume, using a comprehensive set of satellite and ground-based observations (including MODIS, CALIOP, SEVIRI, AERONET, and EPA Air Quality network) and the NASA GEOS global aerosol transport model. The MODIS data record registered this massive dust intrusion event as the most intense episode over the past two decades. During this event, the aerosol optical depth observed by AERONET and MODIS peaked at 3.5 off the coast of West Africa and 1.8 in the Caribbean Basin. CALIOP observations show that the top of dust plume reached altitudes of 6–8 km in West Africa and descended to about 4 km altitude over the Caribbean Basin and 2 km over the U.S. Gulf coast. The dust plume degraded the air quality in Puerto Rico to the hazardous level, with maximum daily PM10 concentration of 453 μg m−3 recorded on June 23. The dust intrusion into the U.S. raised the PM2.5 concentration on June 27 to a level exceeding the EPA air quality standard in about 40 % of the stations in the southern U.S. Satellite observations reveal that dust emissions from convection-generated haboobs and other sources in West Africa were large albeit not extreme on a daily basis. However, the anomalous strength and northern shift of the North Atlantic Subtropical High (NASH) together with the Azores low formed a closed circulation pattern that allowed for accumulation of the dust near the African coast for about four days. When the NASH was weakened and wandered back to south, the dust outflow region was dominated by a strong African Easterly Jet that rapidly transported the accumulated dust from the coastal region toward the Caribbean Basin, resulting in the record-breaking African dust intrusion. In comparison to satellite observations, the GEOS model well reproduced the MODIS observed tracks of the meandering dust plume as it was carried by the wind systems. However, the model substantially underestimated dust emissions from haboobs and did not lift up enough dust to the middle troposphere for ensuing long-range transport. Consequently, the model largely missed the satellite-observed elevated dust plume along the cross-ocean track and underestimated the dust intrusion into the Caribbean Basin by a factor of more than 4. Modeling improvements need to focus on developing more realistic representations of moist convection, haboobs, and the vertical transport of dust.


2011 ◽  
Vol 11 (5) ◽  
pp. 15469-15495 ◽  
Author(s):  
S. Wu ◽  
L. J. Mickley ◽  
J. O. Kaplan ◽  
D. J. Jacob

Abstract. The effects of future land use and land cover change on the chemical composition of the atmosphere and air quality are largely unknown. To investigate the potential effects associated with future changes in vegetation driven by atmospheric CO2 concentrations, climate, and anthropogenic land use over the 21st century, we performed a series of model experiments combining a general circulation model with a dynamic global vegetation model and an atmospheric chemical-transport model. Our results indicate that climate- and CO2-induced changes in vegetation composition and density could lead to decreases in summer afternoon surface ozone of up to 10 ppb over large areas of the northern mid-latitudes. This is largely driven by the substantial increases in ozone dry deposition associated with changes in the composition of temperate and boreal forests where conifer forests are replaced by those dominated by broadleaf tree types, as well as a CO2-driven increase in vegetation density. Climate-driven vegetation changes over the period 2000–2100 lead to general increases in isoprene emissions, globally by 15 % in 2050 and 36 % in 2100. These increases in isoprene emissions result in decreases in surface ozone concentrations where the NOx levels are low, such as in remote tropical rainforests. However, over polluted regions, such as the northeastern United States, ozone concentrations are calculated to increase with higher isoprene emissions in the future. Increases in biogenic emissions also lead to higher concentrations of secondary organic aerosols, which increase globally by 10 % in 2050 and 20 % in 2100. Surface concentrations of secondary organic aerosols are calculated to increase by up to 1 μg m−3 for large areas in Eurasia. When we use a scenario of future anthropogenic land use change, we find less increase in global isoprene emissions due to replacement of higher-emitting forests by lower-emitting cropland. The global atmospheric burden of secondary organic aerosols changes little by 2100 when we account for future land use change, but both secondary organic aerosols and ozone show large regional changes at the surface.


Atmosphere ◽  
2020 ◽  
Vol 11 (7) ◽  
pp. 708 ◽  
Author(s):  
Mathieu Lachatre ◽  
Gilles Foret ◽  
Benoit Laurent ◽  
Guillaume Siour ◽  
Juan Cuesta ◽  
...  

Air pollution in Chinese megacities has reached extremely hazardous levels, and human activities are responsible for the emission or production of large amounts of particulate matter (PM). In addition to PM from anthropogenic sources, natural phenomena, such as dust storms over Asian deserts, may also emit large amounts of PM, which lead episodically to poor air quality over Chinese megacities. In this paper, we quantify the degradation of air quality by dust over Beijing, Chengdu and Shanghai megacities using the three dimensions (3D) chemistry transport model CHIMERE, which simulates dust emission and transport online. In the first part of our work, we evaluate dust emissions using Moderate Resolution Imaging Spectroradiometer (MODIS) and Infrared Atmospheric Sounding Interferometer (IASI) satellite observations of aerosol optical depth, respectively, in the visible and the thermal infrared over source areas. PM simulations were also evaluated compared to surface monitoring stations. Then, mineral dust emissions and their impacts on particle composition of several Chinese megacities were analyzed. Dust emissions and transport over China were simulated during three years (2011, 2013 and 2015). Annual dust contributions to the PM 10 budget over Beijing, Chengdu and Shanghai were evaluated respectively as 6.6%, 9.5% and 9.3%. Dust outbreaks largely contribute to poor air quality events during springtime. Indeed it was found that dust significantly contribute for 22%, 52% and 43% of spring PM 10 events (for Beijing, Chengdu and Shanghai respectively).


2012 ◽  
Vol 12 (3) ◽  
pp. 1597-1609 ◽  
Author(s):  
S. Wu ◽  
L. J. Mickley ◽  
J. O. Kaplan ◽  
D. J. Jacob

Abstract. The effects of future land use and land cover change on the chemical composition of the atmosphere and air quality are largely unknown. To investigate the potential effects associated with future changes in vegetation driven by atmospheric CO2 concentrations, climate, and anthropogenic land use over the 21st century, we performed a series of model experiments combining a general circulation model with a dynamic global vegetation model and an atmospheric chemical-transport model. Our results indicate that climate- and CO2-induced changes in vegetation composition and density between 2100 and 2000 could lead to decreases in summer afternoon surface ozone of up to 10 ppb over large areas of the northern mid-latitudes. This is largely driven by the substantial increases in ozone dry deposition associated with increases in vegetation density in a warmer climate with higher atmospheric CO2 abundance. Climate-driven vegetation changes over the period 2000–2100 lead to general increases in isoprene emissions, globally by 15% in 2050 and 36% in 2100. These increases in isoprene emissions result in decreases in surface ozone concentrations where the NOx levels are low, such as in remote tropical rainforests. However, over polluted regions, such as the northeastern United States, ozone concentrations are calculated to increase with higher isoprene emissions in the future. Increases in biogenic emissions also lead to higher concentrations of secondary organic aerosols, which increase globally by 10% in 2050 and 20% in 2100. Summertime surface concentrations of secondary organic aerosols are calculated to increase by up to 1 μg m−3 and double for large areas in Eurasia over the period of 2000–2100. When we use a scenario of future anthropogenic land use change, we find less increase in global isoprene emissions due to replacement of higher-emitting forests by lower-emitting cropland. The global atmospheric burden of secondary organic aerosols changes little by 2100 when we account for future land use change, but both secondary organic aerosols and ozone show large regional changes at the surface.


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