scholarly journals Improvements of synergetic aerosol retrieval for ENVISAT

2008 ◽  
Vol 8 (24) ◽  
pp. 7651-7672 ◽  
Author(s):  
T. Holzer-Popp ◽  
M. Schroedter-Homscheidt ◽  
H. Breitkreuz ◽  
D. Martynenko ◽  
L. Klüser

Abstract. The synergetic aerosol retrieval method SYNAER (Holzer-Popp et al., 2002a) has been extended to the use of ENVISAT measurements. It exploits the complementary information of a radiometer and a spectrometer onboard one satellite platform to extract aerosol optical depth (AOD) and speciation (as a choice from a representative set of pre-defined mixtures of water-soluble, soot, mineral dust, and sea salt components). SYNAER consists of two retrieval steps. In the first step the radiometer is used for accurate cloud screening, and subsequently to quantify the aerosol optical depth (AOD) at 550 nm and spectral surface brightness through a dark field technique for different pre-defined aerosol mixtures. In the second step the spectrometer is applied to choose the most plausible aerosol mixture through a least square fit of the measured spectrum with simulated spectra using the mixture-dependent values of AOD and surface brightness retrieved in the first step. This method was developed and a first case study evaluation against few (15) multi-spectral ground-based AERONET sun photometer observations was conducted with a sensor pair (ATSR-2 and GOME) onboard ERS-2. Due to instrumental limitations the coverage of SYNAER/ERS-2 is very sparse. Therefore, SYNAER was transferred to similar sensors AATSR and SCIAMACHY onboard ENVISAT. While transferring to the new sensor pair significant improvements in the methodology were made based on a thorough evaluation of the methodology: (1) an update of the aerosol model, (2) improved cloud detection in the tropics and sub tropics, and (3) an enhanced dark field albedo characterization. This paper describes these improvements in detail and assesses their combined impact on the results. After a brief assessment of atmospheric noise impact on comparisons of pixel and station measurements a validation against ground-based measurements establishes error bars for the SYNAER/ENVISAT method version 2.0. A theoretical analysis of the information content with regard to aerosol composition (second retrieval step) is presented to quantify the potential and limitations of this new capability provided by the SYNAER method. Building on this analysis, first seasonal and monthly composition results calculated by applying SYNAER version 2.0 to AATSR and SCIAMACHY are shown to demonstrate the potential of the approach. An inter-comparison to earlier results of SYNAER version 1.0 is made for both the validation and the example datasets.

2008 ◽  
Vol 8 (1) ◽  
pp. 2903-2951 ◽  
Author(s):  
T. Holzer-Popp ◽  
M. Schroedter-Homscheidt ◽  
H. Breitkreuz ◽  
D. Martynenko ◽  
L. Klüser

Abstract. The synergetic aerosol retrieval method SYNAER (Holzer-Popp et al., 2002a) has been extended to the use of ENVISAT measurements. It exploits the complementary information of a radiometer and a spectrometer onboard one satellite platform to extract aerosol optical depth (AOD) and speciation (as choice from a representative set of pre-defined mixtures of water-soluble, soot, mineral dust, and sea salt components). SYNAER consists of two retrieval steps. In the first step the radiometer is used to do accurate cloud screening, and subsequently to quantify the aerosol optical depth (AOD) at 550 nm and spectral surface brightness through a dark field technique. In the second step the spectrometer is applied to choose the most plausible aerosol type through a least square fit of the measured spectrum with simulated spectra using the AOD and surface brightness retrieved in the first step. This method was developed and a first case study evaluation against few (15) multi-spectral ground-based AERONET sun photometer observations was conducted with a sensor pair (ATSR-2 and GOME) onboard ERS-2. However, due to instrumental limitations the coverage of SYNAER/ERS-2 and the AERONET network in 1997/98 is very sparse and thus only few coincidences with AERONET were found. Therefore, SYNAER was transferred to similar sensors AATSR and SCIAMACHY onboard ENVISAT. While transferring to the new sensor pair a thorough evaluation of the synergetic methodology and its information content has been conducted, which led to significant improvements in the methodology: an update of the aerosol model, an improved cloud detection, and an enhanced dark field albedo characterization. This paper describes the information content analysis and these improvements in detail and presents first results of applying the SYNAER methodology to AATSR and SCIAMACHY.


2010 ◽  
Vol 3 (6) ◽  
pp. 1589-1598 ◽  
Author(s):  
D. Martynenko ◽  
T. Holzer-Popp ◽  
H. Elbern ◽  
M. Schroedter-Homscheidt

Abstract. An information content analysis for multi-wavelength SYNergetic AErosol Retrieval algorithm SYNAER was performed to quantify the number of independent pieces of information that can be retrieved. In particular, the capability of SYNAER to discern various aerosol types is assessed. This information content depends on the aerosol optical depth, the surface albedo spectrum and the observation geometry. The theoretical analysis is performed for a large number of scenarios with various geometries and surface albedo spectra for ocean, soil and vegetation. When the surface albedo spectrum and its accuracy is known under cloud-free conditions, reflectance measurements used in SYNAER is able to provide for 2–4° of freedom that can be attributed to retrieval parameters: aerosol optical depth, aerosol type and surface albedo. The focus of this work is placed on an information content analysis with emphasis to the aerosol type classification. This analysis is applied to synthetic reflectance measurements for 40 predefined aerosol mixtures of different basic components, given by sea salt, mineral dust, biomass burning and diesel aerosols, water soluble and water insoluble aerosols. The range of aerosol parameters considered through the 40 mixtures covers the natural variability of tropospheric aerosols. After the information content analysis performed in Holzer-Popp et al. (2008) there was a necessity to compare derived degrees of freedom with retrieved aerosol optical depth for different aerosol types, which is the main focus of this paper. The principle component analysis was used to determine the correspondence between degrees of freedom for signal in the retrieval and derived aerosol types. The main results of the analysis indicate correspondence between the major groups of the aerosol types, which are: water soluble aerosol, soot, mineral dust and sea salt and degrees of freedom in the algorithm and show the ability of the SYNAER to discern between this aerosol types. The results of the work will be further used for the development of the promising methodology of the construction error covariance matrices in the assimilation system.


2018 ◽  
Vol 99 (4) ◽  
pp. 739-755 ◽  
Author(s):  
Z. Q. Li ◽  
H. Xu ◽  
K. T. Li ◽  
D. H. Li ◽  
Y. S. Xie ◽  
...  

AbstractAn overview of Sun–Sky Radiometer Observation Network (SONET) measurements in China is presented. Based on observations at 16 distributed SONET sites in China, atmospheric aerosol parameters are acquired via standardization processes of operational measurement, maintenance, calibration, inversion, and quality control implemented since 2010. A climatology study is performed focusing on total columnar atmospheric aerosol characteristics, including optical (aerosol optical depth, ÅngstrÖm exponent, fine-mode fraction, single-scattering albedo), physical (volume particle size distribution), chemical composition (black carbon; brown carbon; fine-mode scattering component, coarse-mode component; and aerosol water), and radiative properties (aerosol radiative forcing and efficiency). Data analyses show that aerosol optical depth is low in the west but high in the east of China. Aerosol composition also shows significant spatial and temporal variations, leading to noticeable diversities in optical and physical property patterns. In west and north China, aerosols are generally affected by dust particles, while monsoon climate and human activities impose remarkable influences on aerosols in east and south China. Aerosols in China exhibit strong light-scattering capability and result in significant radiative cooling effects.


2006 ◽  
Vol 6 (12) ◽  
pp. 4809-4821 ◽  
Author(s):  
G. Myhre ◽  
A. Grini ◽  
S. Metzger

Abstract. A thermodynamical model for treatment of gas/aerosol partitioning of semi volatile inorganic aerosols has been implemented in a global chemistry and aerosol transport model (Oslo CTM2). The sulphur cycle and sea salt particles have been implemented earlier in the Oslo CTM2 and the focus of this study is on nitrate partitioning to the aerosol phase and if particulate nitrate is expected to form in fine or coarse mode aerosols. Modelling of the formation of fine mode nitrate particles is complicated since it depends on other aerosol components and aerosol precursors as well as meteorological condition. The surface concentrations from the model are compared to observed surface concentrations at around 20 sites around Europe for nitrate and ammonium. The agreement for nitrate is good but the modelled values are somewhat underestimated compared to observations at high concentrations, whereas for ammonium the agreement is very good. However, we underscore that such a comparison is not of large importance for the aerosol optical depth of particulate nitrate since the vertical profile of aerosol components and their precursors are so important. Fine mode nitrate formation depends on vertical profiles of both ammonia/ammonium and sulphate. The model results show that fine mode particulate nitrate play a non-negligible role in the total aerosol composition in certain industrialized regions and therefore have a significant local radiative forcing. On a global scale the aerosol optical depth of fine mode nitrate is relatively small due to limited availability of ammonia and loss to larger sea salt particles. Inclusion of sea salt in the calculations reduces the aerosol optical depth and burden of fine mode nitrate by 25% on a global scale but with large regional variations.


2013 ◽  
Vol 6 (1) ◽  
pp. 2227-2251 ◽  
Author(s):  
L. Mei ◽  
Y. Xue ◽  
A. A. Kokhanovsky ◽  
W. von Hoyningen-Huene ◽  
G. de Leeuw ◽  
...  

Abstract. The Advanced Very High Resolution Radiometer (AVHRR) radiance data provide a global, long-term, consistent time series having high spectral and spatial resolution and thus being valuable for the retrieval of surface spectral reflectance, albedo and surface temperature. Long term time series of such data products are necessary for studies addressing climate change, sea ice distribution and movement, and ice sheet coastal configuration. These data have also been used to retrieve aerosol properties over ocean and land surfaces. However, the retrieval of aerosol over land and land surface albedo are challenging because of the information content of the measurement is limited and the inversion of these data products being ill defined. Solving the radiative transfer equations requires additional information and knowledge to reduce the number of unknowns. In this contribution we utilise an empirical linear relationship between the surface reflectances in the AVHRR channels at wavelengths of 3.75 μm and 2.1 μm, which has been identified in Moderate Resolution Imaging Spectroradiometer (MODIS) data. Next, following the MODIS dark target approach, the surface reflectance at 0.64 μm was obtained. The comparison of the estimated surface reflectance at 0.64 μm with MODIS reflectance products (MOD09) shows a strong correlation (R = 0.7835). Once this was established, the MODIS "dark-target" aerosol retrieval method was adapted to Advanced Very High Resolution Radiometer (AVHRR) data. A simplified Look-Up Table (LUT) method, adopted from Bremen AErosol Retrieval (BAER) algorithm, was used in the retrieval. The Aerosol Optical Depth (AOD) values retrieved from AVHRR with this method compare favourably with ground-based measurements, with a correlation coefficient R = 0.861 and Root Mean Square Error (RMSE) = 0.17. This method can be easily applied to other satellite instruments which do not have a 2.1 μm channel, such as those currently planned to geostationary satellites.


2014 ◽  
Vol 7 (8) ◽  
pp. 2411-2420 ◽  
Author(s):  
L. L. Mei ◽  
Y. Xue ◽  
A. A. Kokhanovsky ◽  
W. von Hoyningen-Huene ◽  
G. de Leeuw ◽  
...  

Abstract. The Advanced Very High Resolution Radiometer (AVHRR) provides a global, long-term, consistent time series of radiance data in several wavebands which are used for the retrieval of surface spectral reflectance, albedo and surface temperature. Long-term time series of such data products are necessary for studies addressing climate change, sea ice distribution and movement, and ice sheet coastal configuration. AVHRR radiances have also been used to retrieve aerosol properties over ocean and land surfaces. However, the retrieval of aerosol over land is challenging because of the limited information content in the data which renders the inversion problem ill defined. Solving the radiative transfer equations requires additional information to reduce the number of unknowns. In this contribution we utilise an empirical linear relationship between the surface reflectances in the AVHRR channels at wavelengths of 3.75 μm and 2.1 μm, which has been identified in the Moderate Resolution Imaging Spectroradiometer (MODIS) data. Following the MODIS dark target approach, this relationship is used to obtain the surface reflectance at 0.64 μm. The comparison of the estimated surface reflectances with MODIS reflectance products (MOD09) shows a strong correlation. Once this was established, the MODIS "dark-target" aerosol retrieval method was adapted to AVHRR data. A simplified look-up table (LUT) method, adopted from the Bremen AErosol Retrieval (BAER) algorithm, was used in the retrieval. The aerosol optical depth (AOD) values retrieved from AVHRR with this method compare favourably with ground-based measurements, with 71.8% of the points located within ±(0.1 + 0.15τ) (τ is the AOD) of the identity line. This method can be easily applied to other satellite instruments which do not have a 2.1 μm channel, such as those currently planned to be used on geostationary satellites.


2018 ◽  
Author(s):  
Pawan Gupta ◽  
Lorraine A. Remer ◽  
Robert C. Levy ◽  
Shana Mattoo

Abstract. The two MODerate Resolution Imaging Spectroradiometer (MODIS) sensors, aboard Earth Observing Satellites (EOS) Terra and Aqua, have been making aerosol observations for more than 15 years. From these observations, the MODIS dark target (DT) aerosol retrieval algorithm provides aerosol optical depth (AOD) products, globally over both land and ocean. In addition to the standard resolution product (10 × 10 km2), the MODIS collection 6 (C006) data release included a higher resolution (3 × 3 km2). Other than accommodations for the two different resolutions, the 10 km, and 3 km DT algorithms are basically the same. In this study, we perform global validation of the higher resolution AOD over global land by comparing against AERONET measurements. The MODIS-AERONET collocated data sets consist of 161,410 high-confidence AOD pairs from 2000 to 2015 for MODIS Terra and 2003 to 2015 for MODIS-Aqua. We find that 62.5 % and 68.4 % of AODs retrieved from MODIS-Terra and MODIS-Aqua, respectively, fall within previously published expected error bounds of ±(0.05 + 0.2*AOD), with a high correlation (R = 0.87). The scatter is not random but exhibits a mean positive bias of ~ 0.06 for Terra and ~ 0.03 for Aqua. These biases for the 3 km product are approximately 0.03 larger than the biases found in similar validations of the 10 km product. The validation results for the 3 km product did not have a relationship to aerosol loading (i.e. true AOD) but did exhibit dependence on quality flags, region, viewing geometry, and aerosol spatial variability. Time series of global MODIS-AERONET differences show that validation is not static, but has changed over the course of both sensors' lifetimes, with MODIS-Terra showing more change over time. The likely cause of the change of validation over time is sensor degradation, but changes in the distribution of AERONET stations and differences in the global aerosol system itself could be contributing to the temporal variability of validation.


2013 ◽  
Vol 13 (12) ◽  
pp. 32269-32289
Author(s):  
T. Logan ◽  
B. Xi ◽  
X. Dong

Abstract. Biomass burning aerosols can have a large impact on atmospheric processes as well as human health. During the 2012 warm season, a large outbreak of wildfires originating from the intermountain and Pacific states provided many opportunities to observe the physical and chemical properties of biomass smoke aerosols. Six biomass burning smoke plumes (26 June–15 September) have been observed by the newly installed Grand Forks, North Dakota, AERONET site (47.91° N, 97.32° W) and are selected for this study. To identify the source regions, HYSPLIT backward trajectory model data and satellite imagery are used to track these events. The volume size distribution and spectral aerosol optical depth (AOD) dependence showed the relative influences of fine and coarse mode particles. Case II (4 July) had the strongest fine mode influence as evidenced by a strong spectral AOD dependence while Case VI (15 September) had the strongest coarse mode influence with the weakest spectral dependence. The spectral dependences of absorption aerosol optical depth (AAOD) and single scattering co-albedo (ωoabs) illustrated the varying absorption of the smoke plumes by inferring the relative contributions of strongly and weakly absorbing carbonaceous species. More specifically, the AAOD parameter is primarily influenced by aerosol particle size while ωoabs is more dependent on aerosol composition. The AAOD spectral dependences for Cases I (26 June), III (31 July), and VI were weaker than those from Cases II, IV (28 August), and V (30 August). However, the spectral ωoabs dependences were different in that the smoke particles in Cases III and VI had the strongest absorption while Cases I, II, IV, and V had moderate to weakly absorbing particles. In addition, a weak correlation was found between plume transport time and particle absorption where strongly absorbing carbon was converted to weakly absorbing carbon.


2011 ◽  
Vol 4 (2) ◽  
pp. 131-141 ◽  
Author(s):  
C. Kittaka ◽  
D. M. Winker ◽  
M. A. Vaughan ◽  
A. Omar ◽  
L. A. Remer

Abstract. The Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) is carried on the CALIPSO satellite and has acquired global aerosol profiles since June 2006. CALIPSO is flown in formation with the Aqua satellite as part of the A-train satellite constellation, so that a large number of coincident aerosol observations are available from CALIOP and the MODIS-Aqua instrument. This study compares column aerosol optical depth at 0.532 μm derived from CALIOP aerosol profiles with MODIS-Aqua 0.55 μm aerosol optical depth over the period June 2006 through August 2008. The study is based on the CALIOP Version 2 Aerosol Layer Product and MODIS Collection 5. While CALIOP is first and foremost a profiling instrument, this comparison of column aerosol optical depth provides insight into quality of CALIOP aerosol data. It is found that daytime aerosol optical depth from the CALIOP Version 2 product has only a small global mean bias relative to MODIS Collection 5. Regional biases, of both signs, are larger and biases are seen to vary somewhat with season. Good agreement between the two sensors in ocean regions with low cloudiness suggests that the selection of lidar ratios used in the CALIOP aerosol retrieval is sufficient to provide a regional mean AOD consistent with that retrieved from MODIS. Although differences over land are observed to be larger than over ocean, the bias between CALIOP and MODIS AOD on a regional-seasonal basis is found to be roughly within the envelope of the MODIS expected uncertainty over land and ocean. This work forms a basis for further comparisons using the recently released CALIOP Version 3 data.


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