scholarly journals Comparison of ground-based and satellite measurements of water vapour vertical profiles over Ellesmere Island, Nunavut

2019 ◽  
Vol 12 (7) ◽  
pp. 4039-4063
Author(s):  
Dan Weaver ◽  
Kimberly Strong ◽  
Kaley A. Walker ◽  
Chris Sioris ◽  
Matthias Schneider ◽  
...  

Abstract. Improving measurements of water vapour in the upper troposphere and lower stratosphere (UTLS) is a priority for the atmospheric science community. In this work, UTLS water vapour profiles derived from Atmospheric Chemistry Experiment (ACE) satellite measurements are assessed with coincident ground-based measurements taken at a high Arctic observatory at Eureka, Nunavut, Canada. Additional comparisons to satellite measurements taken by the Atmospheric Infrared Sounder (AIRS), Michelson Interferometer for Passive Atmospheric Sounding (MIPAS), Microwave Limb Sounder (MLS), Scanning Imaging Absorption Spectrometer for Atmospheric CHartography (SCIAMACHY), and Tropospheric Emission Spectrometer (TES) are included to put the ACE Fourier transform spectrometer (ACE-FTS) and ACE Measurement of Aerosol Extinction in the Stratosphere and Troposphere Retrieved by Occultation (ACE-MAESTRO) results in context. Measurements of water vapour profiles at Eureka are made using a Bruker 125HR solar absorption Fourier transform infrared spectrometer at the Polar Environment Atmospheric Research Laboratory (PEARL) and radiosondes launched from the Eureka Weather Station. Radiosonde measurements used in this study were processed with software developed by the Global Climate Observing System (GCOS) Reference Upper-Air Network (GRUAN) to account for known biases and calculate uncertainties in a well-documented and consistent manner. ACE-FTS measurements were within 11 ppmv (parts per million by volume; 13 %) of 125HR measurements between 6 and 14 km. Between 8 and 14 km ACE-FTS profiles showed a small wet bias of approximately 8 % relative to the 125HR. ACE-FTS water vapour profiles had mean differences of 13 ppmv (32 %) or better when compared to coincident radiosonde profiles at altitudes between 6 and 14 km; mean differences were within 6 ppmv (12 %) between 7 and 11 km. ACE-MAESTRO profiles showed a small dry bias relative to the 125HR of approximately 7 % between 6 and 9 km and 10 % between 10 and 14 km. ACE-MAESTRO profiles agreed within 30 ppmv (36 %) of the radiosondes between 7 and 14 km. ACE-FTS and ACE-MAESTRO comparison results show closer agreement with the radiosondes and PEARL 125HR overall than other satellite datasets – except for AIRS. Close agreement was observed between AIRS and the 125HR and radiosonde measurements, with mean differences within 5 % and correlation coefficients above 0.83 in the troposphere between 1 and 7 km. Comparisons to MLS at altitudes around 10 km showed a dry bias, e.g. mean differences between MLS and radiosondes were −25.6 %. SCIAMACHY comparisons were very limited due to minimal overlap between the vertical extent of the measurements. TES had no temporal overlap with the radiosonde dataset used in this study. Comparisons between TES and the 125HR showed a wet bias of approximately 25 % in the UTLS and mean differences within 14 % below 5 km.

2018 ◽  
Author(s):  
Dan Weaver ◽  
Kimberly Strong ◽  
Kaley A. Walker ◽  
Chris Sioris ◽  
Matthias Schneider ◽  
...  

Abstract. Improving measurements of water vapour in the lower stratosphere and upper troposphere (UTLS) is a priority for the atmospheric science community. In this work, UTLS water vapour profiles derived from Atmospheric Chemistry Experiment (ACE) satellite measurements are assessed with coincident ground-based measurements taken at a high Arctic observatory at Eureka, Nunavut, Canada. Additional comparisons to satellite measurements taken by AIRS, MIPAS, MLS, SCIAMACHY, and TES are included to put the ACE-FTS and ACE-MAESTRO results in context. Measurements of water vapour profiles at Eureka are made using a Bruker 125HR solar absorption Fourier transform infrared spectrometer at the Polar Environment Atmospheric Research Laboratory (PEARL) and radiosondes launched from the Eureka Weather Station. Radiosonde measurements used in this study have been processed with software developed by the Global Climate Observing System (GCOS) Reference Upper Air Network (GRUAN) to account for known biases and calculate uncertainties in a well-documented and consistent manner. ACE-FTS measurements were within 11 ppmv (13 %) of 125HR measurements between 6 and 14 km. Between 8 and 14 km ACE-FTS profiles showed a small wet bias of approximately 8 % relative to the 125HR. ACE-FTS water vapour profiles had mean differences of 13 ppmv (32 %) or better when compared to coincident radiosonde profiles at altitudes between 6 and 14 km; mean differences were within 6 ppmv (12 %) between 7 and 11 km. ACE-MAESTRO profiles showed a small dry bias relative to the 125HR of approximately 7 % between 6 and 9 km and 10 % between 10 and 14 km. ACE-MAESTRO profiles agreed within 30 ppmv (36 %) of the radiosondes between 7 and 14 km. ACE-FTS and ACE-MAESTRO comparison results show closer agreement with the radiosondes and PEARL 125HR overall than other satellite datasets – except AIRS. Close agreement was observed between AIRS and the 125HR and radiosonde measurements, with mean differences within 5 % and correlation coefficients above 0.83 in the troposphere between 1 and 7 km. Comparisons to MLS at altitudes around 10 km showed a dry bias, e.g., mean differences between MLS and radiosondes were −25.6 %. SCIAMACHY comparisons were very limited due to minimal overlap between the vertical extent of the measurements. TES had no temporal overlap with the radiosonde dataset used in this study. Comparisons between TES and the 125HR showed a wet bias of approximately 25 % in the UTLS and mean differences within 14 % below 5 km.


2017 ◽  
Vol 10 (9) ◽  
pp. 3273-3294 ◽  
Author(s):  
Debora Griffin ◽  
Kaley A. Walker ◽  
Stephanie Conway ◽  
Felicia Kolonjari ◽  
Kimberly Strong ◽  
...  

Abstract. This paper presents 8 years (2006–2013) of measurements obtained from Fourier transform spectrometers (FTSs) in the high Arctic at the Polar Environment Atmospheric Research Laboratory (PEARL; 80.05° N, 86.42° W). These measurements were taken as part of the Canadian Arctic ACE (Atmospheric Chemistry Experiment) validation campaigns that have been carried out since 2004 during the polar sunrise period (from mid-February to mid-April). Each spring, two ground-based FTSs were used to measure total and partial columns of HF, O3, and trace gases that impact O3 depletion, namely, HCl and HNO3. Additionally, some tropospheric greenhouse gases and pollutant species were measured, namely CH4, N2O, CO, and C2H6. During the same time period, the satellite-based ACE-FTS made measurements near Eureka and provided profiles of the same trace gases. Comparisons have been carried out between the measurements from the Portable Atmospheric Research Interferometric Spectrometer for the InfraRed (PARIS-IR) and the co-located high-resolution Bruker 125HR FTS, as well as with the latest version of the ACE-FTS retrievals (v3.5). The total column comparison between the two co-located ground-based FTSs, PARIS-IR and Bruker 125HR, found very good agreement for most of these species (except HF), with differences well below the estimated uncertainties ( ≤ 6  %) and with high correlations (R ≥ 0. 8). Partial columns have been used for the ground-based to space-borne comparison, with coincident measurements selected based on time, distance, and scaled potential vorticity (sPV). The comparisons of the ground-based measurements with ACE-FTS show good agreement in the partial columns for most species within 6  % (except for C2H6 and PARIS-IR HF), which is consistent with the total retrieval uncertainty of the ground-based instruments. The correlation coefficients (R) of the partial column comparisons for all eight species range from approximately 0.75 to 0.95. The comparisons show no notable increases of the mean differences over these 8 years, indicating the consistency of these datasets and suggesting that the space-borne ACE-FTS measurements have been stable over this period. In addition, changes in the amounts of these trace gases during springtime between 2006 and 2013 are presented and discussed. Increased O3 (0. 9  %  yr−1), HCl (1. 7  %  yr−1), HF (3. 8  %  yr−1), CH4 (0.5  % yr−1), and C2H6 (2. 3 % yr−1, 2009–2013) have been found with the PARIS-IR dataset, the longer of the two ground-based records.


2016 ◽  
Author(s):  
Debora Griffin ◽  
Kaley A. Walker ◽  
Stephanie Conway ◽  
Felicia Kolonjari ◽  
Kimberly Strong ◽  
...  

Abstract. This paper presents eight years (2006–2013) of measurements obtained from Fourier Transform Spectrometers (FTSs) in the high Arctic at the Polar Environment Atmospheric Research Laboratory (PEARL, 80.05° N, 86.42° W). These measurements were taken as part of the Canadian Arctic ACE (Atmospheric Chemistry Experiment) Validation Campaigns that have been carried out since 2004 during the polar sunrise period (from mid-February to mid-April). Each spring, two ground-based FTSs were used to measure total and partial columns of HF, O3, and trace gases that impact O3 depletion, namely, HCl, and HNO3. Additionally, some tropospheric greenhouse gases and pollutant species were measured, namely CH4, N2O, CO, and C2H6. During the same time period, the satellite-based ACE-FTS made measurements near Eureka and provided profiles of the same trace gases. Comparisons have been carried out between the measurements from PARIS-IR and the co-located high-resolution Bruker 125HR FTS, as well as with the latest version of the ACE-FTS retrievals (v3.5). The total column comparison between the two co-located ground-based FTSs, PARIS-IR and Bruker 125HR, found very good agreement for most of these species (except HF), with differences well below the estimated uncertainties (~ 6 %) and with high correlations (R ≥ 0.8). Partial columns have been used for the ground-based to space-borne comparison, with coincident measurements selected based on time, distance and scaled potential vorticity (sPV). The comparisons of the ground-based measurements with ACE-FTS show good agreement in the partial columns for most species within 6 % (except for C2H6 and PARIS-IR HF), which are consistent with the total retrieval uncertainty of the ground-based instruments. The correlation coefficients (R) of the partial column comparisons for all eight species range from approximately 0.75 to 0.95. The comparisons show no significant increase in the mean differences over these eight years, indicating the consistency of these datasets and suggesting that the space-borne ACE-FTS measurements have been stable over this period. In addition, changes in the amounts of these trace gases during springtime between 2006 and 2013 are presented and discussed. Increased O3 (0.9 % yr−1), HCl (1.7 % yr−1), HF (3.8 % yr−1), CH4 (0.5 % yr−1) and C2H6 (2.3 % yr−1, 2009–2013) have been found near PEARL from the Portable Atmospheric Research Interferometric Spectrometer for the InfraRed (PARIS-IR) dataset.


2019 ◽  
Vol 12 (6) ◽  
pp. 3111-3121 ◽  
Author(s):  
Mark E. Hervig ◽  
Benjamin T. Marshall ◽  
Scott M. Bailey ◽  
David E. Siskind ◽  
James M. Russell III ◽  
...  

Abstract. Nitric oxide (NO) measurements from the Solar Occultation for Ice Experiment (SOFIE) are validated through detailed uncertainty analysis and comparisons with independent observations. SOFIE was compared with coincident satellite measurements from the Atmospheric Chemistry Experiment (ACE) – Fourier Transform Spectrometer (FTS) instrument and the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) instrument. The comparisons indicate mean differences of less than ∼50 % for altitudes from roughly 50 to 105 km for SOFIE spacecraft sunrise and 50 to 140 km for SOFIE sunsets. Comparisons of NO time series show a high degree of correlation between SOFIE and both ACE and MIPAS for altitudes below ∼130 km, indicating that measured NO variability in time is robust. SOFIE uncertainties increase below ∼80 km due to interfering H2O absorption and signal correction uncertainties, which are larger for spacecraft sunrise compared to sunset. These errors are sufficiently large in sunrises that reliable NO measurements are infrequent below ∼80 km.


2019 ◽  
Author(s):  
Mark E. Hervig ◽  
Benjamin T. Marshall ◽  
Scott M. Bailey ◽  
David E. Siskind ◽  
James M. Russell III ◽  
...  

Abstract. Nitric oxide (NO) measurements from the Solar Occultation for Ice Experiment (SOFIE) are validated through detailed uncertainty analysis and comparisons with independent observations. SOFIE was compared with coincident satellite measurements from the Atmospheric Chemistry Experiment (ACE) – Fourier Transform Spectrometer (FTS) instrument, and the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) instrument. The comparisons indicate mean differences of less than ~ 50 % for altitudes from roughly 50 to 105 km for SOFIE spacecraft sunrise, and 50 to 140 km for SOFIE sunsets. Comparisons of NO time series show a high degree of correlation between SOFIE and both ACE and MIPAS for altitudes below ~ 130 km, indicating that measured NO variability in time is robust. SOFIE uncertainties increase below ~ 80 km due to interfering H2O absorption, and from signal correction uncertainties which are larger for spacecraft sunrise compared to sunset. These errors are sufficiently large in sunrises that reliable NO measurements are infrequent below ~ 80 km.


2018 ◽  
Vol 11 (9) ◽  
pp. 4981-5006 ◽  
Author(s):  
Christian Borger ◽  
Matthias Schneider ◽  
Benjamin Ertl ◽  
Frank Hase ◽  
Omaira E. García ◽  
...  

Abstract. Volume mixing ratio water vapour profiles have been retrieved from IASI (Infrared Atmospheric Sounding Interferometer) spectra using the MUSICA (MUlti-platform remote Sensing of Isotopologues for investigating the Cycle of Atmospheric water) processor. The retrievals are done for IASI observations that coincide with Vaisala RS92 radiosonde measurements performed in the framework of the GCOS (Global Climate Observing System) Reference Upper-Air Network (GRUAN) in three different climate zones: the tropics (Manus Island, 2° S), mid-latitudes (Lindenberg, 52° N), and polar regions (Sodankylä, 67° N). The retrievals show good sensitivity with respect to the vertical H2O distribution between 1 km above ground and the upper troposphere. Typical DOFS (degrees of freedom for signal) values are about 5.6 for the tropics, 5.1 for summertime mid-latitudes, 3.8 for wintertime mid-latitudes, and 4.4 for summertime polar regions. The errors of the MUSICA IASI water vapour profiles have been theoretically estimated considering the contribution of many different uncertainty sources. For all three climate regions, unrecognized cirrus clouds and uncertainties in atmospheric temperature have been identified as the most important error sources and they can reach about 25 %. The MUSICA IASI water vapour profiles have been compared to 100 individual coincident GRUAN water vapour profiles. The systematic difference between the data is within 11 % below 12 km altitude; however, at higher altitudes the MUSICA IASI data show a dry bias with respect to the GRUAN data of up to 21 %. The scatter is largest close to the surface (30 %), but never exceeds 21 % above 1 km altitude. The comparison study documents that the MUSICA IASI retrieval processor provides H2O profiles that capture the large variations in H2O volume mixing ratio profiles well from 1 km above ground up to altitudes close to the tropopause. Above 5 km the observed scatter with respect to GRUAN data is in reasonable agreement with the combined MUSICA IASI and GRUAN random errors. The increased scatter at lower altitudes might be explained by surface emissivity uncertainties at the summertime continental sites of Lindenberg and Sodankylä, and the upper tropospheric dry bias might suggest deficits in correctly modelling the spectroscopic line shapes of water vapour.


2017 ◽  
Vol 17 (18) ◽  
pp. 11521-11539 ◽  
Author(s):  
Stefan Lossow ◽  
Hella Garny ◽  
Patrick Jöckel

Abstract. The amplitude of the annual variation in water vapour exhibits a distinct isolated maximum in the middle and upper stratosphere in the southern tropics and subtropics, peaking typically around 15° S in latitude and close to 3 hPa (∼  40.5 km) in altitude. This enhanced annual variation is primarily related to the Brewer–Dobson circulation and hence also visible in other trace gases. So far this feature has not gained much attention in the literature and the present work aims to add more prominence. Using Envisat/MIPAS (Environmental Satellite/Michelson Interferometer for Passive Atmospheric Sounding) observations and ECHAM/MESSy (European Centre for Medium-Range Weather Forecasts Hamburg/Modular Earth Submodel System) Atmospheric Chemistry (EMAC) simulations we provide a dedicated illustration and a full account of the reasons for this enhanced annual variation.


2018 ◽  
Author(s):  
Charlotta Högberg ◽  
Stefan Lossow ◽  
Ralf Bauer ◽  
Kaley A. Walker ◽  
Patrick Eriksson ◽  
...  

Abstract. Within the framework of the second SPARC (Stratosphere-troposphere Processes And their Role in Climate) water vapour assessment (WAVAS-II), we have evaluated five data sets of δD(H2O) obtained from observations of Odin/SMR (Sub-Millimetre Radiometer), Envisat/MIPAS (Environmental Satellite/Michelson Interferometer for Passive Atmospheric Sounding) and SCISAT/ACE-FTS (Science Satellite/Atmospheric Chemistry Experiment-Fourier Transform Spectrometer) using profile-to-profile and climatological comparisons. Our focus is on stratospheric altitudes, but results from the upper troposphere to the lower mesosphere are provided. There are clear quantitative differences in the measurements of the isotopic ratio, which primarily concerns the comparisons to the SMR data set. In the lower stratosphere, this data set shows a higher depletion than the MIPAS and ACE-FTS data sets. The differences maximise close to 50 hPa and exceed 200 per mille. With increasing altitude, the biases typically decrease. Above 4 hPa, the SMR data set shows a lower depletion than the MIPAS data sets, on occasion exceeding 100 per mille. Overall, the δD biases of the SMR data set are driven by HDO biases in the lower stratosphere and by H2O biases in the upper stratosphere and lower mesosphere. In between, in the middle stratosphere, the biases in δD are a combination of deviations in both HDO and H2O. These biases are attributed to issues with the calibration, in particular in terms of the sideband filtering for H2O, and uncertainties in spectroscopic parameters. The MIPAS and ACE-FTS data sets agree rather well between about 100 hPa and 10 hPa. The MIPAS data sets show less depletion below about 15 hPa (up to about 30 per mille), due to differences in both HDO and H2O. Higher up the picture is reversed, and towards the upper stratosphere the biases typically increase. This is driven by increasing biases in H2O and on occasion the differences in δD exceed 80 per mille. Below 100 hPa, the differences between the MIPAS and ACE-FTS data sets are even larger. In the climatological comparisons, the MIPAS data sets continue to show less depletion than the ACE-FTS data sets below 15 hPa during all seasons, with some variations in magnitude. The differences between the MIPAS and ACE-FTS data come from different aspects, such as differences in the temporal and spatial sampling (except for the profile-to-profile comparisons), cloud influence, vertical resolution, and the microwindows and spectroscopic database chosen. Differences between data sets from the same instrument are typically small in the stratosphere.


2019 ◽  
Vol 19 (4) ◽  
pp. 2497-2526 ◽  
Author(s):  
Charlotta Högberg ◽  
Stefan Lossow ◽  
Farahnaz Khosrawi ◽  
Ralf Bauer ◽  
Kaley A. Walker ◽  
...  

Abstract. Within the framework of the second SPARC (Stratosphere-troposphere Processes And their Role in Climate) water vapour assessment (WAVAS-II), we evaluated five data sets of δD(H2O) obtained from observations by Odin/SMR (Sub-Millimetre Radiometer), Envisat/MIPAS (Environmental Satellite/Michelson Interferometer for Passive Atmospheric Sounding), and SCISAT/ACE-FTS (Science Satellite/Atmospheric Chemistry Experiment – Fourier Transform Spectrometer) using profile-to-profile and climatological comparisons. These comparisons aimed to provide a comprehensive overview of typical uncertainties in the observational database that could be considered in the future in observational and modelling studies. Our primary focus is on stratospheric altitudes, but results for the upper troposphere and lower mesosphere are also shown. There are clear quantitative differences in the measurements of the isotopic ratio, mainly with regard to comparisons between the SMR data set and both the MIPAS and ACE-FTS data sets. In the lower stratosphere, the SMR data set shows a higher depletion in δD than the MIPAS and ACE-FTS data sets. The differences maximise close to 50 hPa and exceed 200 ‰. With increasing altitude, the biases decrease. Above 4 hPa, the SMR data set shows a lower δD depletion than the MIPAS data sets, occasionally exceeding 100 ‰. Overall, the δD biases of the SMR data set are driven by HDO biases in the lower stratosphere and by H2O biases in the upper stratosphere and lower mesosphere. In between, in the middle stratosphere, the biases in δD are the result of deviations in both HDO and H2O. These biases are attributed to issues with the calibration, in particular in terms of the sideband filtering, and uncertainties in spectroscopic parameters. The MIPAS and ACE-FTS data sets agree rather well between about 100 and 10 hPa. The MIPAS data sets show less depletion below approximately 15 hPa (up to about 30 ‰), due to differences in both HDO and H2O. Higher up this behaviour is reversed, and towards the upper stratosphere the biases increase. This is driven by increasing biases in H2O, and on occasion the differences in δD exceed 80 ‰. Below 100 hPa, the differences between the MIPAS and ACE-FTS data sets are even larger. In the climatological comparisons, the MIPAS data sets continue to show less depletion in δD than the ACE-FTS data sets below 15 hPa during all seasons, with some variations in magnitude. The differences between the MIPAS and ACE-FTS data have multiple causes, such as differences in the temporal and spatial sampling (except for the profile-to-profile comparisons), cloud influence, vertical resolution, and the microwindows and spectroscopic database chosen. Differences between data sets from the same instrument are typically small in the stratosphere. Overall, if the data sets are considered together, the differences in δD among them in key areas of scientific interest (e.g. tropical and polar lower stratosphere, lower mesosphere, and upper troposphere) are too large to draw robust conclusions on atmospheric processes affecting the water vapour budget and distribution, e.g. the relative importance of different mechanisms transporting water vapour into the stratosphere.


Atmosphere ◽  
2019 ◽  
Vol 10 (7) ◽  
pp. 390
Author(s):  
Ji-Ping Guan ◽  
Yan-Tong Yin ◽  
Li-Feng Zhang ◽  
Jing-Nan Wang ◽  
Ming-Yang Zhang

Total precipitable water (TPW) of satellite-borne microwave radiometer retrievals is compared with the data that were collected from 49 island radiosonde stations for the period 2007–2015. Great consistency was found between TPW measurements made by radiosonde and eight satellite-borne microwave radiometers, including SSMI-F13, SSMI-F14, SSMIS-F16, SSMIS-F17, AMSR-E, AMSR-2, GMI, and WindSat. Mean values of the TPW differences for eight satellites ranged from −0.51 to 0.38mm, both root mean square errors and standard deviations were around 3mm, and all of the correlation coefficients between satellite TPW retrievals and radiosonde TPW for each satellite can reach 0.99. Subsequently, an analysis of the comparison results was conducted, which revealed three problems in the satellite TPW retrieval and two problems in radiosonde data. For TPW retrievals of satellite, when the values are above 60 mm, the precision of TPW retrieval significantly decreases with a distinct dry bias, which can reach 4 mm; additionally, abias related to wind speed and the uncertainty with the TPW retrieval in the presence of rain, which is stronger than 1mm/h, was found. The TPW measurements of radiosonde made by the type of IM-MK3 from India were quite unreliable, and almost all of the radiosonde data during the daytime were plagued by a dry bias.


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