scholarly journals Comparison of ground-based and satellite measurements of water vapour vertical profiles over Ellesmere Island, Nunavut

2018 ◽  
Author(s):  
Dan Weaver ◽  
Kimberly Strong ◽  
Kaley A. Walker ◽  
Chris Sioris ◽  
Matthias Schneider ◽  
...  
Keyword(s):  
Water Vapour ◽  
Atmospheric Chemistry ◽  
Global Climate ◽  
Correlation Coefficients ◽  
High Arctic ◽  
Satellite Measurements ◽  
Solar Absorption ◽  
Comparison Results ◽  
Mean Differences ◽  
Dry Bias

Abstract. Improving measurements of water vapour in the lower stratosphere and upper troposphere (UTLS) is a priority for the atmospheric science community. In this work, UTLS water vapour profiles derived from Atmospheric Chemistry Experiment (ACE) satellite measurements are assessed with coincident ground-based measurements taken at a high Arctic observatory at Eureka, Nunavut, Canada. Additional comparisons to satellite measurements taken by AIRS, MIPAS, MLS, SCIAMACHY, and TES are included to put the ACE-FTS and ACE-MAESTRO results in context. Measurements of water vapour profiles at Eureka are made using a Bruker 125HR solar absorption Fourier transform infrared spectrometer at the Polar Environment Atmospheric Research Laboratory (PEARL) and radiosondes launched from the Eureka Weather Station. Radiosonde measurements used in this study have been processed with software developed by the Global Climate Observing System (GCOS) Reference Upper Air Network (GRUAN) to account for known biases and calculate uncertainties in a well-documented and consistent manner. ACE-FTS measurements were within 11 ppmv (13 %) of 125HR measurements between 6 and 14 km. Between 8 and 14 km ACE-FTS profiles showed a small wet bias of approximately 8 % relative to the 125HR. ACE-FTS water vapour profiles had mean differences of 13 ppmv (32 %) or better when compared to coincident radiosonde profiles at altitudes between 6 and 14 km; mean differences were within 6 ppmv (12 %) between 7 and 11 km. ACE-MAESTRO profiles showed a small dry bias relative to the 125HR of approximately 7 % between 6 and 9 km and 10 % between 10 and 14 km. ACE-MAESTRO profiles agreed within 30 ppmv (36 %) of the radiosondes between 7 and 14 km. ACE-FTS and ACE-MAESTRO comparison results show closer agreement with the radiosondes and PEARL 125HR overall than other satellite datasets – except AIRS. Close agreement was observed between AIRS and the 125HR and radiosonde measurements, with mean differences within 5 % and correlation coefficients above 0.83 in the troposphere between 1 and 7 km. Comparisons to MLS at altitudes around 10 km showed a dry bias, e.g., mean differences between MLS and radiosondes were −25.6 %. SCIAMACHY comparisons were very limited due to minimal overlap between the vertical extent of the measurements. TES had no temporal overlap with the radiosonde dataset used in this study. Comparisons between TES and the 125HR showed a wet bias of approximately 25 % in the UTLS and mean differences within 14 % below 5 km.

scholarly journals Comparison of ground-based and satellite measurements of water vapour vertical profiles over Ellesmere Island, Nunavut

2019 ◽  
Vol 12 (7) ◽  
pp. 4039-4063
Author(s):  
Dan Weaver ◽  
Kimberly Strong ◽  
Kaley A. Walker ◽  
Chris Sioris ◽  
Matthias Schneider ◽  
...  
Keyword(s):  
Fourier Transform ◽  
Water Vapour ◽  
Atmospheric Chemistry ◽  
Global Climate ◽  
Michelson Interferometer ◽  
Correlation Coefficients ◽  
Satellite Measurements ◽  
Comparison Results ◽  
Mean Differences ◽  
Dry Bias

Abstract. Improving measurements of water vapour in the upper troposphere and lower stratosphere (UTLS) is a priority for the atmospheric science community. In this work, UTLS water vapour profiles derived from Atmospheric Chemistry Experiment (ACE) satellite measurements are assessed with coincident ground-based measurements taken at a high Arctic observatory at Eureka, Nunavut, Canada. Additional comparisons to satellite measurements taken by the Atmospheric Infrared Sounder (AIRS), Michelson Interferometer for Passive Atmospheric Sounding (MIPAS), Microwave Limb Sounder (MLS), Scanning Imaging Absorption Spectrometer for Atmospheric CHartography (SCIAMACHY), and Tropospheric Emission Spectrometer (TES) are included to put the ACE Fourier transform spectrometer (ACE-FTS) and ACE Measurement of Aerosol Extinction in the Stratosphere and Troposphere Retrieved by Occultation (ACE-MAESTRO) results in context. Measurements of water vapour profiles at Eureka are made using a Bruker 125HR solar absorption Fourier transform infrared spectrometer at the Polar Environment Atmospheric Research Laboratory (PEARL) and radiosondes launched from the Eureka Weather Station. Radiosonde measurements used in this study were processed with software developed by the Global Climate Observing System (GCOS) Reference Upper-Air Network (GRUAN) to account for known biases and calculate uncertainties in a well-documented and consistent manner. ACE-FTS measurements were within 11 ppmv (parts per million by volume; 13 %) of 125HR measurements between 6 and 14 km. Between 8 and 14 km ACE-FTS profiles showed a small wet bias of approximately 8 % relative to the 125HR. ACE-FTS water vapour profiles had mean differences of 13 ppmv (32 %) or better when compared to coincident radiosonde profiles at altitudes between 6 and 14 km; mean differences were within 6 ppmv (12 %) between 7 and 11 km. ACE-MAESTRO profiles showed a small dry bias relative to the 125HR of approximately 7 % between 6 and 9 km and 10 % between 10 and 14 km. ACE-MAESTRO profiles agreed within 30 ppmv (36 %) of the radiosondes between 7 and 14 km. ACE-FTS and ACE-MAESTRO comparison results show closer agreement with the radiosondes and PEARL 125HR overall than other satellite datasets – except for AIRS. Close agreement was observed between AIRS and the 125HR and radiosonde measurements, with mean differences within 5 % and correlation coefficients above 0.83 in the troposphere between 1 and 7 km. Comparisons to MLS at altitudes around 10 km showed a dry bias, e.g. mean differences between MLS and radiosondes were −25.6 %. SCIAMACHY comparisons were very limited due to minimal overlap between the vertical extent of the measurements. TES had no temporal overlap with the radiosonde dataset used in this study. Comparisons between TES and the 125HR showed a wet bias of approximately 25 % in the UTLS and mean differences within 14 % below 5 km.

scholarly journals Intercomparison of atmospheric water vapour measurements at a Canadian High Arctic site

2017 ◽  
Vol 10 (8) ◽  
pp. 2851-2880 ◽  
Author(s):  
Dan Weaver ◽  
Kimberly Strong ◽  
Matthias Schneider ◽  
Penny M. Rowe ◽  
Chris Sioris ◽  
...  
Keyword(s):  
Water Vapour ◽  
Global Climate ◽  
Microwave Radiometer ◽  
Correlation Coefficients ◽  
High Arctic ◽  
Atmospheric Water ◽  
Canadian High Arctic ◽  
Solar Absorption ◽  
Atmospheric Water Vapour ◽  
Ftir Spectrometer

Abstract. Water vapour is a critical component of the Earth system. Techniques to acquire and improve measurements of atmospheric water vapour and its isotopes are under active development. This work presents a detailed intercomparison of water vapour total column measurements taken between 2006 and 2014 at a Canadian High Arctic research site (Eureka, Nunavut). Instruments include radiosondes, sun photometers, a microwave radiometer, and emission and solar absorption Fourier transform infrared (FTIR) spectrometers. Close agreement is observed between all combination of datasets, with mean differences  ≤  1.0 kg m−2 and correlation coefficients  ≥  0.98. The one exception in the observed high correlation is the comparison between the microwave radiometer and a radiosonde product, which had a correlation coefficient of 0.92.A variety of biases affecting Eureka instruments are revealed and discussed. A subset of Eureka radiosonde measurements was processed by the Global Climate Observing System (GCOS) Reference Upper Air Network (GRUAN) for this study. Comparisons reveal a small dry bias in the standard radiosonde measurement water vapour total columns of approximately 4 %. A recently produced solar absorption FTIR spectrometer dataset resulting from the MUSICA (MUlti-platform remote Sensing of Isotopologues for investigating the Cycle of Atmospheric water) retrieval technique is shown to offer accurate measurements of water vapour total columns (e.g. average agreement within −5.2 % of GRUAN and −6.5 % of a co-located emission FTIR spectrometer). However, comparisons show a small wet bias of approximately 6 % at the high-latitude Eureka site. In addition, a new dataset derived from Atmospheric Emitted Radiance Interferometer (AERI) measurements is shown to provide accurate water vapour measurements (e.g. average agreement was within 4 % of GRUAN), which usefully enables measurements to be taken during day and night (especially valuable during polar night).

scholarly journals Multi-year comparisons of ground-based and space-borne Fourier transform spectrometers in the high Arctic between 2006 and 2013

2017 ◽  
Vol 10 (9) ◽  
pp. 3273-3294 ◽  
Author(s):  
Debora Griffin ◽  
Kaley A. Walker ◽  
Stephanie Conway ◽  
Felicia Kolonjari ◽  
Kimberly Strong ◽  
...  
Keyword(s):  
Fourier Transform ◽  
Atmospheric Chemistry ◽  
Trace Gases ◽  
Correlation Coefficients ◽  
High Arctic ◽  
Atmospheric Research ◽  
Time Period ◽  
Experiment Validation ◽  
Mean Differences ◽  
Good Agreement

Abstract. This paper presents 8 years (2006–2013) of measurements obtained from Fourier transform spectrometers (FTSs) in the high Arctic at the Polar Environment Atmospheric Research Laboratory (PEARL; 80.05° N, 86.42° W). These measurements were taken as part of the Canadian Arctic ACE (Atmospheric Chemistry Experiment) validation campaigns that have been carried out since 2004 during the polar sunrise period (from mid-February to mid-April). Each spring, two ground-based FTSs were used to measure total and partial columns of HF, O3, and trace gases that impact O3 depletion, namely, HCl and HNO3. Additionally, some tropospheric greenhouse gases and pollutant species were measured, namely CH4, N2O, CO, and C2H6. During the same time period, the satellite-based ACE-FTS made measurements near Eureka and provided profiles of the same trace gases. Comparisons have been carried out between the measurements from the Portable Atmospheric Research Interferometric Spectrometer for the InfraRed (PARIS-IR) and the co-located high-resolution Bruker 125HR FTS, as well as with the latest version of the ACE-FTS retrievals (v3.5). The total column comparison between the two co-located ground-based FTSs, PARIS-IR and Bruker 125HR, found very good agreement for most of these species (except HF), with differences well below the estimated uncertainties ( ≤ 6  %) and with high correlations (R ≥ 0. 8). Partial columns have been used for the ground-based to space-borne comparison, with coincident measurements selected based on time, distance, and scaled potential vorticity (sPV). The comparisons of the ground-based measurements with ACE-FTS show good agreement in the partial columns for most species within 6  % (except for C2H6 and PARIS-IR HF), which is consistent with the total retrieval uncertainty of the ground-based instruments. The correlation coefficients (R) of the partial column comparisons for all eight species range from approximately 0.75 to 0.95. The comparisons show no notable increases of the mean differences over these 8 years, indicating the consistency of these datasets and suggesting that the space-borne ACE-FTS measurements have been stable over this period. In addition, changes in the amounts of these trace gases during springtime between 2006 and 2013 are presented and discussed. Increased O3 (0. 9  %  yr−1), HCl (1. 7  %  yr−1), HF (3. 8  %  yr−1), CH4 (0.5  % yr−1), and C2H6 (2. 3 % yr−1, 2009–2013) have been found with the PARIS-IR dataset, the longer of the two ground-based records.

scholarly journals Multi-year comparisons of ground-based and space-borne Fourier Transform Spectrometers in the high Arctic between 2006 and 2013

2016 ◽  
Author(s):  
Debora Griffin ◽  
Kaley A. Walker ◽  
Stephanie Conway ◽  
Felicia Kolonjari ◽  
Kimberly Strong ◽  
...  
Keyword(s):  
Fourier Transform ◽  
Atmospheric Chemistry ◽  
Trace Gases ◽  
Correlation Coefficients ◽  
High Arctic ◽  
Atmospheric Research ◽  
Time Period ◽  
Experiment Validation ◽  
Mean Differences ◽  
Good Agreement

Abstract. This paper presents eight years (2006–2013) of measurements obtained from Fourier Transform Spectrometers (FTSs) in the high Arctic at the Polar Environment Atmospheric Research Laboratory (PEARL, 80.05° N, 86.42° W). These measurements were taken as part of the Canadian Arctic ACE (Atmospheric Chemistry Experiment) Validation Campaigns that have been carried out since 2004 during the polar sunrise period (from mid-February to mid-April). Each spring, two ground-based FTSs were used to measure total and partial columns of HF, O3, and trace gases that impact O3 depletion, namely, HCl, and HNO3. Additionally, some tropospheric greenhouse gases and pollutant species were measured, namely CH4, N2O, CO, and C2H6. During the same time period, the satellite-based ACE-FTS made measurements near Eureka and provided profiles of the same trace gases. Comparisons have been carried out between the measurements from PARIS-IR and the co-located high-resolution Bruker 125HR FTS, as well as with the latest version of the ACE-FTS retrievals (v3.5). The total column comparison between the two co-located ground-based FTSs, PARIS-IR and Bruker 125HR, found very good agreement for most of these species (except HF), with differences well below the estimated uncertainties (~ 6 %) and with high correlations (R ≥ 0.8). Partial columns have been used for the ground-based to space-borne comparison, with coincident measurements selected based on time, distance and scaled potential vorticity (sPV). The comparisons of the ground-based measurements with ACE-FTS show good agreement in the partial columns for most species within 6 % (except for C2H6 and PARIS-IR HF), which are consistent with the total retrieval uncertainty of the ground-based instruments. The correlation coefficients (R) of the partial column comparisons for all eight species range from approximately 0.75 to 0.95. The comparisons show no significant increase in the mean differences over these eight years, indicating the consistency of these datasets and suggesting that the space-borne ACE-FTS measurements have been stable over this period. In addition, changes in the amounts of these trace gases during springtime between 2006 and 2013 are presented and discussed. Increased O3 (0.9 % yr−1), HCl (1.7 % yr−1), HF (3.8 % yr−1), CH4 (0.5 % yr−1) and C2H6 (2.3 % yr−1, 2009–2013) have been found near PEARL from the Portable Atmospheric Research Interferometric Spectrometer for the InfraRed (PARIS-IR) dataset.

scholarly journals Intercomparison of atmospheric water vapour measurements in the Canadian high Arctic

2016 ◽  
Author(s):  
Dan Weaver ◽  
Kimberly Strong ◽  
Matthias Schneider ◽  
Penny M. Rowe ◽  
Chris Sioris ◽  
...  
Keyword(s):  
Water Vapour ◽  
Microwave Radiometer ◽  
Correlation Coefficients ◽  
High Arctic ◽  
Atmospheric Water ◽  
Canadian High Arctic ◽  
Solar Absorption ◽  
Atmospheric Water Vapour ◽  
Retrieval Technique ◽  
Good Agreement

Abstract. Water vapour is a critical component of the Earth system. Techniques to acquire and improve measurements of atmospheric water vapour and its isotopes are under active development. This work presents a detailed intercomparison of water vapour total column measurements taken between 2006 and 2014 at a Canadian high Arctic research site. Instruments include radiosondes, sun photometers, a microwave radiometer, and emission and solar absorption Fourier transform spectrometers (FTSs). Good agreement is observed between all combination of datasets, with correlation coefficients ≥ 0.90 showing high correlations. A variety of biases and calibration issues are revealed and discussed for all instruments. A new FTS dataset, resulting from the MUSICA (Multi-platform remote Sensing of Isotopologues for investigating the Cycle of Atmospheric water) retrieval technique, is shown to offer accurate measurements of water vapour total columns; however, measurements show a small wet bias of approximately 6 %. A new dataset derived from Atmospheric Emitted Radiance Interferometer (AERI) measurements is also shown to provide accurate water vapour measurements, which usefully enables measurements to be taken during day and night (especially valuable during Polar Night). In addition, limited profile comparisons are conducted using radiosonde and ground-based FTS measurements. Results show MUSICA FTS profiles were within 15 % of radiosonde measurements throughout the troposphere.

scholarly journals Evaluation of MUSICA IASI tropospheric water vapour profiles using theoretical error assessments and comparisons to GRUAN Vaisala RS92 measurements

2018 ◽  
Vol 11 (9) ◽  
pp. 4981-5006 ◽  
Author(s):  
Christian Borger ◽  
Matthias Schneider ◽  
Benjamin Ertl ◽  
Frank Hase ◽  
Omaira E. García ◽  
...  
Keyword(s):  
Water Vapour ◽  
Degrees Of Freedom ◽  
Global Climate ◽  
Atmospheric Temperature ◽  
Systematic Difference ◽  
Polar Regions ◽  
Mixing Ratio ◽  
Random Errors ◽  
The Tropics ◽  
Dry Bias

Abstract. Volume mixing ratio water vapour profiles have been retrieved from IASI (Infrared Atmospheric Sounding Interferometer) spectra using the MUSICA (MUlti-platform remote Sensing of Isotopologues for investigating the Cycle of Atmospheric water) processor. The retrievals are done for IASI observations that coincide with Vaisala RS92 radiosonde measurements performed in the framework of the GCOS (Global Climate Observing System) Reference Upper-Air Network (GRUAN) in three different climate zones: the tropics (Manus Island, 2° S), mid-latitudes (Lindenberg, 52° N), and polar regions (Sodankylä, 67° N). The retrievals show good sensitivity with respect to the vertical H2O distribution between 1 km above ground and the upper troposphere. Typical DOFS (degrees of freedom for signal) values are about 5.6 for the tropics, 5.1 for summertime mid-latitudes, 3.8 for wintertime mid-latitudes, and 4.4 for summertime polar regions. The errors of the MUSICA IASI water vapour profiles have been theoretically estimated considering the contribution of many different uncertainty sources. For all three climate regions, unrecognized cirrus clouds and uncertainties in atmospheric temperature have been identified as the most important error sources and they can reach about 25 %. The MUSICA IASI water vapour profiles have been compared to 100 individual coincident GRUAN water vapour profiles. The systematic difference between the data is within 11 % below 12 km altitude; however, at higher altitudes the MUSICA IASI data show a dry bias with respect to the GRUAN data of up to 21 %. The scatter is largest close to the surface (30 %), but never exceeds 21 % above 1 km altitude. The comparison study documents that the MUSICA IASI retrieval processor provides H2O profiles that capture the large variations in H2O volume mixing ratio profiles well from 1 km above ground up to altitudes close to the tropopause. Above 5 km the observed scatter with respect to GRUAN data is in reasonable agreement with the combined MUSICA IASI and GRUAN random errors. The increased scatter at lower altitudes might be explained by surface emissivity uncertainties at the summertime continental sites of Lindenberg and Sodankylä, and the upper tropospheric dry bias might suggest deficits in correctly modelling the spectroscopic line shapes of water vapour.

scholarly journals The high Arctic in extreme winters: vortex, temperature, and MLS and ACE-FTS trace gas evolution

2008 ◽  
Vol 8 (3) ◽  
pp. 505-522 ◽  
Author(s):  
G. L. Manney ◽  
W. H. Daffer ◽  
K. B. Strawbridge ◽  
K. A. Walker ◽  
C. D. Boone ◽  
...  
Keyword(s):  
Atmospheric Chemistry ◽  
Lower Stratosphere ◽  
High Arctic ◽  
Trace Gas ◽  
Satellite Measurements ◽  
Broadband Emission ◽  
Gas Measurements ◽  
Chemistry Experiment ◽  
Very High ◽  
Good Agreement

Abstract. The first three Arctic winters of the ACE mission represented two extremes of winter variability: Stratospheric sudden warmings (SSWs) in 2004 and 2006 were among the strongest, most prolonged on record; 2005 was a record cold winter. Canadian Arctic Atmospheric Chemistry Experiment (ACE) Validation Campaigns were conducted at Eureka (80° N, 86° W) during each of these winters. New satellite measurements from ACE-Fourier Transform Spectrometer (ACE-FTS), Sounding of the Atmosphere using Broadband Emission Radiometry (SABER), and Aura Microwave Limb Sounder (MLS), along with meteorological analyses and Eureka lidar temperatures, are used to detail the meteorology in these winters, to demonstrate its influence on transport, and to provide a context for interpretation of ACE-FTS and validation campaign observations. During the 2004 and 2006 SSWs, the vortex broke down throughout the stratosphere, reformed quickly in the upper stratosphere, and remained weak in the middle and lower stratosphere. The stratopause reformed at very high altitude, near 75 km. ACE measurements covered both vortex and extra-vortex conditions in each winter, except in late-February through mid-March 2004 and 2006, when the strong, pole-centered vortex that reformed after the SSWs resulted in ACE sampling only inside the vortex in the middle through upper stratosphere. The 2004 and 2006 Eureka campaigns were during the recovery from the SSWs, with the redeveloping vortex over Eureka. 2005 was the coldest winter on record in the lower stratosphere, but with an early final warming in mid-March. The vortex was over Eureka at the start of the 2005 campaign, but moved away as it broke up. Disparate temperature profile structure and vortex evolution resulted in much lower (higher) temperatures in the upper (lower) stratosphere in 2004 and 2006 than in 2005. Satellite temperatures agree well with lidar data up to 50–60 km, and ACE-FTS, MLS and SABER show good agreement in high-latitude temperatures throughout the winters. Consistent with a strong, cold upper stratospheric vortex and enhanced radiative cooling after the SSWs, MLS and ACE-FTS trace gas measurements show strongly enhanced descent in the upper stratospheric vortex in late January through March 2006 compared to that in 2005.

scholarly journals Comparison Analysis of Total Precipitable Water of Satellite-Borne Microwave Radiometer Retrievals and Island Radiosondes

Atmosphere ◽  
2019 ◽  
Vol 10 (7) ◽  
pp. 390
Author(s):  
Ji-Ping Guan ◽  
Yan-Tong Yin ◽  
Li-Feng Zhang ◽  
Jing-Nan Wang ◽  
Ming-Yang Zhang
Keyword(s):  
Microwave Radiometer ◽  
Correlation Coefficients ◽  
Precipitable Water ◽  
Radiosonde Data ◽  
Mean Values ◽  
Total Precipitable Water ◽  
Comparison Results ◽  
Almost All ◽  
Mean Square Errors ◽  
Dry Bias

Total precipitable water (TPW) of satellite-borne microwave radiometer retrievals is compared with the data that were collected from 49 island radiosonde stations for the period 2007–2015. Great consistency was found between TPW measurements made by radiosonde and eight satellite-borne microwave radiometers, including SSMI-F13, SSMI-F14, SSMIS-F16, SSMIS-F17, AMSR-E, AMSR-2, GMI, and WindSat. Mean values of the TPW differences for eight satellites ranged from −0.51 to 0.38mm, both root mean square errors and standard deviations were around 3mm, and all of the correlation coefficients between satellite TPW retrievals and radiosonde TPW for each satellite can reach 0.99. Subsequently, an analysis of the comparison results was conducted, which revealed three problems in the satellite TPW retrieval and two problems in radiosonde data. For TPW retrievals of satellite, when the values are above 60 mm, the precision of TPW retrieval significantly decreases with a distinct dry bias, which can reach 4 mm; additionally, abias related to wind speed and the uncertainty with the TPW retrieval in the presence of rain, which is stronger than 1mm/h, was found. The TPW measurements of radiosonde made by the type of IM-MK3 from India were quite unreliable, and almost all of the radiosonde data during the daytime were plagued by a dry bias.

scholarly journals Methane cross-validation between three Fourier transform spectrometers: SCISAT ACE-FTS, GOSAT TANSO-FTS, and ground-based FTS measurements in the Canadian high Arctic

2016 ◽  
Vol 9 (5) ◽  
pp. 1961-1980 ◽  
Author(s):  
Gerrit Holl ◽  
Kaley A. Walker ◽  
Stephanie Conway ◽  
Naoko Saitoh ◽  
Chris D. Boone ◽  
...  
Keyword(s):  
Fourier Transform ◽  
Atmospheric Chemistry ◽  
Degrees Of Freedom ◽  
Near Infrared ◽  
Cross Validation ◽  
High Arctic ◽  
Canadian High Arctic ◽  
Infrared Band ◽  
Absolute Deviation ◽  
Solar Absorption

Abstract. We present cross-validation of remote sensing measurements of methane profiles in the Canadian high Arctic. Accurate and precise measurements of methane are essential to understand quantitatively its role in the climate system and in global change. Here, we show a cross-validation between three data sets: two from spaceborne instruments and one from a ground-based instrument. All are Fourier transform spectrometers (FTSs). We consider the Canadian SCISAT Atmospheric Chemistry Experiment (ACE)-FTS, a solar occultation infrared spectrometer operating since 2004, and the thermal infrared band of the Japanese Greenhouse Gases Observing Satellite (GOSAT) Thermal And Near infrared Sensor for carbon Observation (TANSO)-FTS, a nadir/off-nadir scanning FTS instrument operating at solar and terrestrial infrared wavelengths, since 2009. The ground-based instrument is a Bruker 125HR Fourier transform infrared (FTIR) spectrometer, measuring mid-infrared solar absorption spectra at the Polar Environment Atmospheric Research Laboratory (PEARL) Ridge Laboratory at Eureka, Nunavut (80° N, 86° W) since 2006. For each pair of instruments, measurements are collocated within 500 km and 24 h. An additional collocation criterion based on potential vorticity values was found not to significantly affect differences between measurements. Profiles are regridded to a common vertical grid for each comparison set. To account for differing vertical resolutions, ACE-FTS measurements are smoothed to the resolution of either PEARL-FTS or TANSO-FTS, and PEARL-FTS measurements are smoothed to the TANSO-FTS resolution. Differences for each pair are examined in terms of profile and partial columns. During the period considered, the number of collocations for each pair is large enough to obtain a good sample size (from several hundred to tens of thousands depending on pair and configuration). Considering full profiles, the degrees of freedom for signal (DOFS) are between 0.2 and 0.7 for TANSO-FTS and between 1.5 and 3 for PEARL-FTS, while ACE-FTS has considerably more information (roughly 1 DOFS per altitude level). We take partial columns between roughly 5 and 30 km for the ACE-FTS–PEARL-FTS comparison, and between 5 and 10 km for the other pairs. The DOFS for the partial columns are between 1.2 and 2 for PEARL-FTS collocated with ACE-FTS, between 0.1 and 0.5 for PEARL-FTS collocated with TANSO-FTS or for TANSO-FTS collocated with either other instrument, while ACE-FTS has much higher information content. For all pairs, the partial column differences are within ±3 × 1022 molecules cm−2. Expressed as median ± median absolute deviation (expressed in partial column units or as a percentage), these differences are 0.11 ± 9.60  × 1020 molecules cm−2 (0.012 ± 1.018 %) for TANSO-FTS–PEARL-FTS, −2.6 ± 2.6 × 1021  cm−2 (−1.6 ± 1.6 %) for ACE-FTS–PEARL-FTS, and 7.4 ± 6.0 × 1020 molecules cm−2 (0.78 ± 0.64 %) for TANSO-FTS–ACE-FTS. The differences for ACE-FTS–PEARL-FTS and TANSO-FTS–PEARL-FTS partial columns decrease significantly as a function of PEARL partial columns, whereas the range of partial column values for TANSO-FTS–ACE-FTS collocations is too small to draw any conclusion on its dependence on ACE-FTS partial columns.

scholarly journals Calibration and validation of water vapour lidar measurements from Eureka, Nunavut, using radiosondes and the Atmospheric Chemistry Experiment Fourier Transform Spectrometer

2013 ◽  
Vol 6 (3) ◽  
pp. 741-749 ◽  
Author(s):  
A. Moss ◽  
R. J. Sica ◽  
E. McCullough ◽  
K. Strawbridge ◽  
K. Walker ◽  
...  
Keyword(s):  
Fourier Transform ◽  
Water Vapour ◽  
Atmospheric Chemistry ◽  
High Arctic ◽  
Fourier Transform Spectrometer ◽  
Arctic Water ◽  
Lidar Measurements ◽  
Tropopause Region ◽  
Polar Day ◽  
Chemistry Experiment

Abstract. The Canadian Network for the Detection of Atmospheric Change and Environment Canada DIAL lidar located at the Polar Environment Atmospheric Research Laboratory (PEARL) in Eureka, Nunavut, has been upgraded to measure water vapour mixing ratio profiles. The lidar is capable of measuring water vapour in the dry Arctic atmosphere up to the tropopause region. Measurements were obtained in the February to March polar sunrise during 2007, 2008 and 2009 as part of the Canadian Arctic ACE (Atmospheric Chemistry Experiment) Validation Campaign. Before such measurements can be used to address important questions in understanding dynamics and chemistry, the lidar measurements must be calibrated against an independent determination of water vapour. Here, radiosonde measurements of relative humidity have been used to empirically calibrate the lidar measurements. It was found that the calibration varied significantly between each year's campaign. However, the calibration of the lidar during an individual polar sunrise campaign agrees on average with the local radiosonde measurements to better than 12%. To independently validate the calibration of the lidar derived from the radiosondes, comparisons are made between the calibrated lidar measurements and water vapour measurements from the ACE satellite-borne Fourier Transform Spectrometer (ACE-FTS). The comparisons between the lidar and satellite-borne spectrometer for both a campaign average and single overpasses show favourable agreement between the two instruments and help validate the lidar's calibration. The 39 nights of high-Arctic water vapour measurements obtained offer the most detailed high spatial-temporal resolution measurement set available for understanding this time of transition from the long polar night to polar day.

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