scholarly journals Stratospheric aerosol extinction profiles from SCIAMACHY solar occultation

2020 ◽  
Vol 13 (10) ◽  
pp. 5643-5666
Author(s):  
Stefan Noël ◽  
Klaus Bramstedt ◽  
Alexei Rozanov ◽  
Elizaveta Malinina ◽  
Heinrich Bovensmann ◽  
...  
Keyword(s):  
Time Series ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Optical Absorption Spectroscopy ◽  
Atmospheric Effects ◽  
Aerosol Extinction ◽  
Radiometric Calibration ◽  
Quasi Biennial Oscillation ◽  
Solar Occultation ◽  
Occultation Data

Abstract. The Scanning Imaging Absorption spectroMeter for Atmospheric CHartographY (SCIAMACHY) instrument on Envisat provided, between August 2002 and April 2012, measurements of solar and Earthshine spectra from the UV to the shortwave infrared spectral region in multiple viewing geometries. We present a new approach to derive stratospheric aerosol extinction profiles from SCIAMACHY solar occultation measurements based on an onion-peeling method similar to the onion-peeling differential optical absorption spectroscopy (DOAS) retrieval, which has already been successfully used for the derivation of greenhouse gas profiles. Since the retrieval of aerosol extinction requires as input measured transmissions in absolute units, an improved radiometric calibration of the SCIAMACHY solar occultation measurements has been developed, which considers various instrumental and atmospheric effects specific to solar occultation. The aerosol extinction retrieval can in principle be applied to all wavelengths measured by SCIAMACHY. As a first application, we show results for 452, 525 and 750 nm. The SCIAMACHY solar occultation time series has been processed, covering a latitudinal range of about 50–70∘ N. Reasonable aerosol extinctions are derived between about 15 and 30 km with typically larger uncertainties at higher altitudes due to decreasing aerosol extinction. Comparisons with collocated Stratospheric Aerosol and Gas Experiment II (SAGE-II) and SCIAMACHY limb aerosol data products revealed good agreement with essentially no mean bias. However, dependent on altitude, differences of up to ±20 %–30% to SAGE-II at 452 and 525 nm are observed. Similar results are obtained from comparisons with SAGE-III. SCIAMACHY solar occultation data at 750 nm have been compared with corresponding SAGE-III, Optical Spectrograph and InfraRed Imager System (OSIRIS) and SCIAMACHY limb results. The agreement with SCIAMACHY limb data at 750 nm is within 5 %–20 % between 17 and 27 km. SAGE-III and OSIRIS show at this wavelength and altitude range on average about 40 % and 25 % smaller values, with some additional 10 %–20 % modulation with altitude. The altitude variations in the differences are mainly caused by systematic vertical oscillations in the SCIAMACHY occultation data of up to 30 % below about 25 km. These oscillations decrease to amplitudes below 10 % with increasing number of collocations and are no longer visible in monthly anomalies. Major volcanic eruptions as well as occurrences of polar stratospheric clouds (PSCs) can be identified in the time series of aerosol extinction data and related anomalies. The influence of the quasi-biennial oscillation (QBO) is visible above 25 km.

scholarly journals Stratospheric Extinction Profiles from SCIAMACHY Solar Occultation

2020 ◽  
Author(s):  
Stefan Noël ◽  
Klaus Bramstedt ◽  
Alexei Rozanov ◽  
Elizaveta Malinina ◽  
Heinrich Bovensmann ◽  
...  
Keyword(s):  
Time Series ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Optical Absorption Spectroscopy ◽  
Atmospheric Effects ◽  
Aerosol Extinction ◽  
Radiometric Calibration ◽  
Quasi Biennial Oscillation ◽  
Solar Occultation ◽  
Scanning Imaging

Abstract. The SCIAMACHY (Scanning Imaging Absorption Spectrometer for Atmospheric CHartographY) instrument on ENVISAT provided between August 2002 and April 2012 measurements of solar and Earthshine spectra from the UV to the SWIR spectral region in multiple viewing geometries. We present a new approach to derive stratospheric aerosol extinction profiles from SCIAMACHY solar occultation measurements based on an onion peeling method similar to the Onion Peeling DOAS (Differential Optical Absorption Spectroscopy) retrieval, which has already been successfully used for the derivation of greenhouse gas profiles. Since the retrieval of aerosol extinction requires as input measured transmissions in absolute units, an improved radiometric calibration of the SCIAMACHY solar occultation measurements has been developed, which considers various instrumental and atmospheric effects specific to solar occultation. The extinction retrieval can in principle be applied to all wavelengths measured by SCIAMACHY. As a first application, we show results for 452 nm, 525 nm and 750 nm. The whole SCIAMACHY solar occultation time series has been processed, covering a latitudinal range of about 50–70° N. Reasonable extinctions are derived between about 15 and 30 km with typically larger uncertainties at higher altitudes due to decreasing extinction. Comparisons with collocated SAGE~II and SCIAMACHY limb aerosol data products revealed a good agreement with essentially no mean bias. However, depending on altitude differences of up to ± 20–30 % to SAGE II at 452 nm and 525 nm are observed. These differences are mainly caused by systematic vertical oscillations in the SCIAMACHY occultation data. The agreement with SCIAMACHY limb data is even better (typically within 5–10 % between 17 and 27 km). Major volcanic eruptions as well as occurrences of PSCs can be identified in the time series of extinction data and related anomalies. Influence of the Quasi-Biennial-Oscillation (QBO) are visible above 25 km. Estimated linear changes of extinction between 2003 and 2011 reach 20–30 % per year at 15 km, mainly because all relevant volcanic eruptions (above 50° N) occurred after 2006.

scholarly journals Improved stratospheric aerosol extinction profiles from SCIAMACHY: validation and sample results

2015 ◽  
Vol 8 (12) ◽  
pp. 5223-5235 ◽  
Author(s):  
C. von Savigny ◽  
F. Ernst ◽  
A. Rozanov ◽  
R. Hommel ◽  
K.-U. Eichmann ◽  
...  
Keyword(s):  
Solar Radiation ◽  
Optical Depth ◽  
Temporal Variability ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Aerosol Extinction ◽  
Data Set ◽  
Solar Occultation ◽  
Mission Period ◽  
Relative Differences

Abstract. Stratospheric aerosol extinction profiles have been retrieved from SCIAMACHY/Envisat measurements of limb-scattered solar radiation. The retrieval is an improved version of an algorithm presented earlier. The retrieved aerosol extinction profiles are compared to co-located aerosol profile measurements from the SAGE II solar occultation instrument at a wavelength of 525 nm. Comparisons were carried out with two versions of the SAGE II data set (version 6.2 and the new version 7.0). In a global average sense the SCIAMACHY and the SAGE II version 7.0 extinction profiles agree to within about 10 % for altitudes above 15 km. Larger relative differences (up to 40 %) are observed at specific latitudes and altitudes. We also find differences between the two SAGE II data versions of up to 40 % for specific latitudes and altitudes, consistent with earlier reports. Sample results on the latitudinal and temporal variability of stratospheric aerosol extinction and optical depth during the SCIAMACHY mission period are presented. The results confirm earlier reports that a series of volcanic eruptions is responsible for the increase in stratospheric aerosol optical depth from 2002 to 2012. Above about an altitude of 28 km, volcanic eruptions are found to have negligible impact in the period 2002–2012.

scholarly journals Stratospheric aerosol evolution after Pinatubo simulated with a coupled size-resolved aerosol–chemistry–climate model, SOCOL-AERv1.0

2018 ◽  
Vol 11 (7) ◽  
pp. 2633-2647 ◽  
Author(s):  
Timofei Sukhodolov ◽  
Jian-Xiong Sheng ◽  
Aryeh Feinberg ◽  
Bei-Ping Luo ◽  
Thomas Peter ◽  
...  
Keyword(s):  
Climate Model ◽  
Reference Model ◽  
Volcanic Eruptions ◽  
Global Scale ◽  
Stratospheric Aerosol ◽  
Atmospheric Effects ◽  
Aerosol Layer ◽  
Aerosol Chemistry ◽  
Quasi Biennial Oscillation ◽  
Aerosol Parameters

Abstract. We evaluate how the coupled aerosol–chemistry–climate model SOCOL-AERv1.0 represents the influence of the 1991 eruption of Mt. Pinatubo on stratospheric aerosol properties and atmospheric state. The aerosol module is coupled to the radiative and chemical modules and includes comprehensive sulfur chemistry and microphysics, in which the particle size distribution is represented by 40 size bins with radii spanning from 0.39 nm to 3.2 µm. SOCOL-AER simulations are compared with satellite and in situ measurements of aerosol parameters, temperature reanalyses, and ozone observations. In addition to the reference model configuration, we performed series of sensitivity experiments looking at different processes affecting the aerosol layer. An accurate sedimentation scheme is found to be essential to prevent particles from diffusing too rapidly to high and low altitudes. The aerosol radiative feedback and the use of a nudged quasi-biennial oscillation help to keep aerosol in the tropics and significantly affect the evolution of the stratospheric aerosol burden, which improves the agreement with observed aerosol mass distributions. The inclusion of van der Waals forces in the particle coagulation scheme suggests improvements in particle effective radius, although other parameters (such as aerosol longevity) deteriorate. Modification of the Pinatubo sulfur emission rate also improves some aerosol parameters, while it worsens others compared to observations. Observations themselves are highly uncertain and render it difficult to conclusively judge the necessity of further model reconfiguration. The model revealed problems in reproducing aerosol sizes above 25 km and also in capturing certain features of the ozone response. Besides this, our results show that SOCOL-AER is capable of predicting the most important global-scale atmospheric effects following volcanic eruptions, which is also a prerequisite for an improved understanding of solar geoengineering effects from sulfur injections to the stratosphere.

scholarly journals Improved stratospheric aerosol extinction profiles from SCIAMACHY: validation and sample results

2015 ◽  
Vol 8 (8) ◽  
pp. 8353-8383 ◽  
Author(s):  
C. von Savigny ◽  
F. Ernst ◽  
A. Rozanov ◽  
R. Hommel ◽  
K.-U. Eichmann ◽  
...  
Keyword(s):  
Solar Radiation ◽  
Optical Depth ◽  
Temporal Variability ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Aerosol Extinction ◽  
Data Set ◽  
Solar Occultation ◽  
Mission Period ◽  
Relative Differences

Abstract. Stratospheric aerosol extinction profiles have been retrieved from SCIAMACHY/Envisat measurements of limb-scattered solar radiation. The retrieval is an improved version of an algorithm presented earlier. The retrieved aerosol extinction profiles are compared to co-located aerosol profile measurements with the SAGE II solar occultation instrument at a wavelength of 525 nm. Comparisons were carried out with two versions of the SAGE II data set (version 6.2 and the new version 7.0). In a global average sense the SCIAMACHY and the SAGE II version 7.0 extinction profiles agree to within about 10 % for altitudes above 15 km. Larger relative differences (up to 40 %) are observed at specific latitudes and altitudes. We also find differences between the two SAGE II data versions of up to 40 % for specific latitudes and altitudes. Sample results on the latitudinal and temporal variability of stratospheric aerosol extinction and optical depth during the SCIAMACHY mission period are presented. The results indicate that a series of volcanic eruptions is responsible for the increase in stratospheric aerosol optical depth from 2002 to 2012. Above about 28 km altitude volcanic eruptions are found to have negligible impact in the period 2002 to 2012.

scholarly journals Effect of volcanic aerosol on stratospheric NO<sub>2</sub> and N<sub>2</sub>O<sub>5</sub> from 2002–2014 as measured by Odin-OSIRIS and Envisat-MIPAS

2016 ◽  
Author(s):  
Cristen Adams ◽  
Adam E. Bourassa ◽  
Chris A. McLinden ◽  
Chris E. Sioris ◽  
Thomas von Clarmann ◽  
...  
Keyword(s):  
Infrared Imaging ◽  
Pearson Correlation ◽  
Michelson Interferometer ◽  
Correlation Coefficients ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Volcanic Aerosol ◽  
Quasi Biennial Oscillation ◽  
El Chichón ◽  
El Chichon

Abstract. Following the large volcanic eruptions of Pinatubo in 1991 and El Chichón in 1982, decreases in stratospheric NO2 associated with enhanced aerosol were observed. The Optical Spectrograph and InfraRed Imaging Spectrometer (OSIRIS) likewise measured widespread enhancements of stratospheric aerosol following seven volcanic eruptions between 2002 and 2014, although the magnitudes of these eruptions were all much smaller than the Pinatubo and El Chichón eruptions. In order to isolate and quantify the relationship between volcanic aerosol and NO2, NO2 anomalies were calculated using measurements from OSIRIS and the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS). In the tropics, variability due to the quasi-biennial oscillation was subtracted from the timeseries. OSIRIS profile measurements indicate that the strongest relationships between NO2 and volcanic aerosol extinction were for the layer ~ 3–7 km above the tropopause, where OSIRIS stratospheric NO2 partial columns for ~ 3–7 km above the tropopause were found to be smaller than baseline levels during these aerosol enhancements by up to ~ 60 % with typical Pearson correlation coefficients of R ~ −0.7. MIPAS also observed decreases in NO2 partial columns during periods of affected by volcanic aerosol, with percent differences of up to ~ 25 %. An even stronger relationship was observed between OSIRIS aerosol optical depth and MIPAS N2O5 partial columns, with R ~ −0.9, although no link with MIPAS HNO3 was observed. The variation of OSIRIS NO2 with increasing aerosol was found to be quantitatively consistent with simulations from a photochemical box model in terms of both magnitude and degree of non-linearity.

scholarly journals Evidence for the predictability of changes in the stratospheric aerosol size following volcanic eruptions of diverse magnitudes using space-based instruments

2020 ◽  
Author(s):  
Larry W. Thomason ◽  
Mahesh Kovilakam ◽  
Anja Schmidt ◽  
Christian von Savigny ◽  
Travis Knepp ◽  
...  
Keyword(s):  
Size Distribution ◽  
Extinction Coefficient ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Global Climate Models ◽  
Aerosol Size Distribution ◽  
Aerosol Layer ◽  
Aerosol Extinction ◽  
Volcanic Event ◽  
Aerosol Extinction Coefficient

Abstract. An analysis of multiwavelength stratospheric aerosol extinction coefficient data from the Stratospheric Aerosol and Gas Experiment II and III/ISS instruments is used to demonstrate a coherent relationship between the perturbation in extinction coefficient in an eruption's main aerosol layer and an apparent change in aerosol size distribution that spans multiple orders of magnitude in the stratospheric impact of a volcanic event. The relationship is measurement-based and does not rely on assumptions about the aerosol size distribution. We note limitations on this analysis including that the presence of significant amounts of ash in the main aerosol layer may significantly modulate these results. Despite this limitation, these findings represent a unique opportunity to verify the performance of interactive aerosol models used in Global Climate Models and Earth System Model and may suggest an avenue for improving aerosol extinction coefficient measurements from single channel observations such the Optical Spectrograph and Infrared Imager System as they rely on a priori assumptions about particle size.

scholarly journals Evidence for the predictability of changes in the stratospheric aerosol size following volcanic eruptions of diverse magnitudes using space-based instruments

2021 ◽  
Vol 21 (2) ◽  
pp. 1143-1158 ◽  
Author(s):  
Larry W. Thomason ◽  
Mahesh Kovilakam ◽  
Anja Schmidt ◽  
Christian von Savigny ◽  
Travis Knepp ◽  
...  
Keyword(s):  
Extinction Coefficient ◽  
Climate Models ◽  
Single Channel ◽  
Volcanic Eruptions ◽  
Stratospheric Aerosol ◽  
Global Climate Models ◽  
Aerosol Size Distribution ◽  
Aerosol Layer ◽  
Aerosol Extinction ◽  
Aerosol Extinction Coefficient

Abstract. An analysis of multiwavelength stratospheric aerosol extinction coefficient data from the Stratospheric Aerosol and Gas Experiment II and III/ISS instruments is used to demonstrate a coherent relationship between the perturbation in extinction coefficient in an eruption's main aerosol layer and the wavelength dependence of that perturbation. This relationship spans multiple orders of magnitude in the aerosol extinction coefficient of stratospheric impact of volcanic events. The relationship is measurement-based and does not rely on assumptions about the aerosol size distribution. We note limitations on this analysis including that the presence of significant amounts of ash in the main sulfuric acid aerosol layer and other factors may significantly modulate these results. Despite these limitations, the findings suggest an avenue for improving aerosol extinction coefficient measurements from single-channel observations such as the Optical Spectrograph and Infrared Imager System as they rely on a prior assumptions about particle size. They may also represent a distinct avenue for the comparison of observations with interactive aerosol models used in global climate models and Earth system models.

scholarly journals Surface temperature response to the major volcanic eruptions in multiple reanalysis data sets

2019 ◽  
Author(s):  
Masatomo Fujiwara ◽  
Patrick Martineau ◽  
Jonathon S. Wright
Keyword(s):  
Time Series ◽  
Surface Temperature ◽  
Volcanic Eruptions ◽  
Reanalysis Data ◽  
Data Sets ◽  
Hemispheric Differences ◽  
Quasi Biennial Oscillation ◽  
Cooling Period ◽  
El Chichón ◽  
El Chichon

Abstract. The global response of air temperature at 2 metre above the surface to the eruptions of Mount Agung in March 1963, El Chichón in April 1982, and Mount Pinatubo in June 1991 is investigated using 11 global atmospheric reanalysis data sets (JRA-55, JRA-25, MERRA-2, MERRA, ERA-Interim, ERA-40, CFSR, NCEP-NCAR R-1, 20CR version 2c, ERA-20C, and CERA-20C). Multiple linear regression (MLR) is applied to the monthly mean time series of temperature for two periods, 1980–2010 (for 10 reanalyses) and 1958–2001 (for six reanalyses), by considering explanatory factors of seasonal harmonics, linear trends, Quasi-Biennial Oscillation (QBO), solar cycle, tropical sea surface temperature (SST) variations in the Pacific, Indian, and Atlantic Oceans, and Arctic SST variations. Empirical orthogonal function (EOF) analysis is applied to these climatic indices to obtain a set of orthogonal indices to be used for the MLR. The residuals of the MLR are used to define the volcanic signals for the three eruptions separately. First, latitudinally averaged time series of the residuals are investigated and compared with the results from previous studies. Then, the geographical distribution of the response during the peak cooling period after each eruption is investigated. In general, different reanalyses show similar geographical patterns of the response, but with the largest differences in the polar regions. The Pinatubo response shows largest average cooling in the 60° N–60° S region among the three eruptions, with a peak cooling of 0.10–0.15 K. The El Chichón response shows slightly larger cooling in the NH than in the Southern Hemisphere (SH), while the Agung response shows larger cooling in the SH. These hemispheric differences are consistent with the distribution of stratospheric aerosol optical depth after these eruptions; however, the peak cooling after these two eruptions is comparable in magnitude to unexplained cooling events in other periods without volcanic influence. Other methods in which the MLR model is used with different sets of indices are also tested, and it is found that careful treatment of tropical SST variability is necessary to evaluate the surface response to volcanic eruptions in observations and reanalyses.

scholarly journals Surface temperature response to the major volcanic eruptions in multiple reanalysis data sets

2020 ◽  
Vol 20 (1) ◽  
pp. 345-374
Author(s):  
Masatomo Fujiwara ◽  
Patrick Martineau ◽  
Jonathon S. Wright
Keyword(s):  
Time Series ◽  
Surface Temperature ◽  
Volcanic Eruptions ◽  
Reanalysis Data ◽  
Data Sets ◽  
Hemispheric Differences ◽  
Quasi Biennial Oscillation ◽  
Cooling Period ◽  
El Chichón ◽  
El Chichon

Abstract. The global response of air temperature at 2 m above the surface to the eruptions of Mount Agung in March 1963, El Chichón in April 1982, and Mount Pinatubo in June 1991 is investigated using 11 global atmospheric reanalysis data sets (JRA-55, JRA-25, MERRA-2, MERRA, ERA-Interim, ERA-40, CFSR, NCEP-NCAR R-1, 20CR version 2c, ERA-20C, and CERA-20C). Multiple linear regression (MLR) is applied to the monthly mean time series of temperature for two periods – 1980–2010 (for 10 reanalyses) and 1958–2001 (for 6 reanalyses) – by considering explanatory factors of seasonal harmonics, linear trends, quasi-biennial oscillation (QBO), solar cycle, tropical sea surface temperature (SST) variations in the Pacific, Indian, and Atlantic Oceans, and Arctic SST variations. Empirical orthogonal function (EOF) analysis is applied to these climatic indices to obtain a set of orthogonal indices to be used for the MLR. The residuals of the MLR are used to define the volcanic signals for the three eruptions separately. First, area-averaged time series of the residuals are investigated and compared with the results from previous studies. Then, the geographical distribution of the response during the peak cooling period after each eruption is investigated. In general, different reanalyses show similar geographical patterns of the response, but with the largest differences in the polar regions. The Pinatubo response shows the largest average cooling in the 60∘ N–60∘ S region among the three eruptions, with a peak cooling of 0.10–0.15 K. The El Chichón response shows slightly larger cooling in the NH than in the Southern Hemisphere (SH), while the Agung response shows larger cooling in the SH. These hemispheric differences are consistent with the distribution of stratospheric aerosol optical depth after these eruptions; however, the peak cooling after these two eruptions is comparable in magnitude to unexplained cooling events in other periods without volcanic influence. Other methods in which the MLR model is used with different sets of indices are also tested, and it is found that careful treatment of tropical SST variability is necessary to evaluate the surface response to volcanic eruptions in observations and reanalyses.

scholarly journals Characterization of Polar Stratospheric Clouds with spaceborne lidar: CALIPSO and the 2006 Antarctic season

2007 ◽  
Vol 7 (19) ◽  
pp. 5207-5228 ◽  
Author(s):  
M. C. Pitts ◽  
L. W. Thomason ◽  
L. R. Poole ◽  
D. M. Winker
Keyword(s):  
Time Series ◽  
Winter Season ◽  
Temporal Distribution ◽  
Detection Algorithm ◽  
Polar Stratospheric Clouds ◽  
Satellite Mission ◽  
Spatial And Temporal Scales ◽  
Solar Occultation ◽  
Occultation Data ◽  
Stratospheric Clouds

Abstract. The role of polar stratospheric clouds in polar ozone loss has been well documented. The CALIPSO satellite mission offers a new opportunity to characterize PSCs on spatial and temporal scales previously impossible. A PSC detection algorithm based on a single wavelength threshold approach has been developed for CALIPSO. The method appears to accurately detect PSCs of all opacities, including tenuous clouds, with a very low rate of false positives and few missed clouds. We applied the algorithm to CALIOP data acquired during the 2006 Antarctic winter season from 13 June through 31 October. The spatial and temporal distribution of CALIPSO PSC observations is illustrated with weekly maps of PSC occurrence. The evolution of the 2006 PSC season is depicted by time series of daily PSC frequency as a function of altitude. Comparisons with "virtual" solar occultation data indicate that CALIPSO provides a different view of the PSC season than attained with previous solar occultation satellites. Measurement-based time series of PSC areal coverage and vertically-integrated PSC volume are computed from the CALIOP data. The observed area covered with PSCs is significantly smaller than would be inferred from the commonly used temperature-based proxy TNAT but is similar in magnitude to that inferred from TSTS. The potential of CALIOP measurements for investigating PSC composition is illustrated using combinations of lidar backscatter and volume depolarization for two CALIPSO PSC scenes.

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