Simple interferometric setup enabling sub-Fourier-scale ultra-short laser pulses

In this work, we describe an interferometric method to generate ultra-short pulses below the Fourier limit. It is done by extending concepts first developed in the spatial domain to achieve sub-diffractive beams through the addition of a spatial chirp in one of the arms of a Michelson interferometer using a spherical mirror. To experimentally synthesize sub-Fourier pulses, we replace the spherical mirror with a water cell, since it produces chirp in the temporal domain. We also present an alternative procedure, based on asymmetrical interference between the widened pulse and the original pulse where the peaks of both pulses exhibit a temporal delay achieving the narrowing of ultra-short pulses with sub-Fourier scales. To characterize the performance of the system, we performed a preliminary assessment considering the percentage of FWHM shrinking obtained for each scheme. By means of a symmetrical configuration 7 and 12 \% pulse reductions were verified, both experimentally and analytically, while for the non-symmetrical configuration 10 and 24\% reductions were achieved corresponding to main lobe to side-lobes ratios of 10 and 30\% . The experimental setup scheme is simple, versatile and able to work with high-power laser sources and ultra-short pulses with a broad bandwidth at any central wavelength. The results presented in this work are promising and help to enlighten new routes and strategies in the design of coherent control systems. We envision that they will become broadly useful in different areas from strong field domain to quantum information.

The interferometric measurement of thermal lens effect in a LD pumped Tm-doped bulk laser

Directly measuring thermal focal length is important for designing and optimizing the mode locking oscillator, especially for a 2-μm mode-locking laser. In this paper, we propose a novel interferometric method for measuring the thermal focal length in a 2-μm mode-locking laser. This method could give a precise measurement of the thermal focal length inside a long-folded oscillator in both lasing and non-lasing operation. We also theoretically calculate the thermal focal length based on the temperature distribution inside the laser crystal, which matches well with the experimental result

Effect of Relative Humidity on the Thickness of Assembled Silica Colloidal Crystal Films

In order for the colloidal crystal films to be better applied, the influence of relative humidity on the preparation of silica colloidal crystal (SCC) films was systematically studied to solve the problem of different thicknesses of SCC films prepared by different batches under the conditions with the same temperature, concentration of suspension and diameter of the particles. SCC films with 190 nm particles were prepared by static vertical deposition method under different humidity regulated by saturated salt solutions, and the thickness of the films was obtained by an interferometric method. The results showed that the increase in humidity would reduce the thickness of the prepared films, which was believed to be caused by the decrease in evaporation rate after the wetting film absorbs water vapor. A new formula for calculating film thickness was proposed and verified from a series of experiments. With the control of humidity, high-quality SCC films with controlled thickness can be repeatedly prepared.

Photoelastic Properties of Trigonal Crystals

All possible experimental geometries of the piezo-optic effect in crystals of trigonal symmetry are studied in detail through the interferometric technique, and the corresponding expressions for the calculation of piezo-optic coefficients (POCs) πim and some sums of πim based on experimental data obtained from the samples of direct and X/45°-cuts are given. The reliability of the values of POCs is proven by the convergence of πim obtained from different experimental geometries as well as by the convergence of some sums of POCs. Because both the signs and the absolute values of POCs π14 and π41 are defined by the choice of the right crystal-physics coordinate system, we here use the system whereby the condition S14 > 0 is fulfilled (S14 is an elastic compliance coefficient). The absolute value and the sign of S14 are determined by piezo-optic interferometric method from two experimental geometries. The errors of POCs are calculated as mean square values of the errors of the half-wave stresses and the elastic term. All components of the matrix of elasto-optic coefficients pin are calculated based on POCs and elastic stiffness coefficients. The technique is tested on LiTaO3 crystal. The obtained results are compared with the corresponding data for trigonal LiNbO3 and Ca3TaGa3Si2O14 crystals.

Label-free SARS-CoV-2 detection and classification using phase imaging with computational specificity

Efforts to mitigate the COVID-19 crisis revealed that fast, accurate, and scalable testing is crucial for curbing the current impact and that of future pandemics. We propose an optical method for directly imaging unlabeled viral particles and using deep learning for detection and classification. An ultrasensitive interferometric method was used to image four virus types with nanoscale optical path-length sensitivity. Pairing these data with fluorescence images for ground truth, we trained semantic segmentation models based on U-Net, a particular type of convolutional neural network. The trained network was applied to classify the viruses from the interferometric images only, containing simultaneously SARS-CoV-2, H1N1 (influenza-A virus), HAdV (adenovirus), and ZIKV (Zika virus). Remarkably, due to the nanoscale sensitivity in the input data, the neural network was able to identify SARS-CoV-2 vs. the other viruses with 96% accuracy. The inference time for each image is 60 ms, on a common graphic-processing unit. This approach of directly imaging unlabeled viral particles may provide an extremely fast test, of less than a minute per patient. As the imaging instrument operates on regular glass slides, we envision this method as potentially testing on patient breath condensates. The necessary high throughput can be achieved by translating concepts from digital pathology, where a microscope can scan hundreds of slides automatically.

The Influence of Battery Acid on the Destruction of Acrylic Coatings of Car Bodies

Renovation coatings of car bodies undergo destruction under the influence of operational factors. Like ultraviolet radiation, erosion, and aggressive media (among others, battery acid). This article concerns the evaluation of the influence of battery acid on the destruction of acrylic coatings previously non-aged, as well as aged climatically for 2 years. Ageing of the coatings with battery acid contributed to a degradation increase of their chemical structure. It was supported by a considerable increase in the polar component of surface free energy (SFE) of the coatings. In the case of prior climate ageing, the increase in the polar component was even higher. Moreover, the coating’s ability to absorb battery acid increased, which induced blistering. The DSC method revealed that the action of battery acid caused more intense oxidation of coating material, and as a result, the brittleness increased, leading to chipping of the coating surface layers. This led to the increase in surface roughness, measured using an interferometric method. The coatings previously climatically aged for 2 years presented higher values of surface roughness parameters than the non-aged ones. The increase in the surface roughness contributed to a substantial decrease in the gloss of coatings. A sharp difference in colour escalating with the lengthening of the ageing period was also observed using the spectrophotometric method.

Reconstruction of attosecond beating by interference of two-photon transitions in the bulk of solids

The reconstruction of attosecond beating by interference of two-photon transitions (RABBIT) is one of the most widely used techniques for resolving ultrafast electronic dynamics in atomic and molecular systems. As it relies on the interference of photo-electrons in vacuum, similar interference has never been contemplated in the bulk of crystals. Using accurate numerical simulations in a realistic system, here we show that the interference of two-photon transitions can be recorded directly in the bulk of solids and read out with standard angle-resolved photo-emission spectroscopy. The phase of the RABBIT beating in the photoelectron spectra coming from the bulk of solids is sensitive to the relative phase of the Berry connection between bands and it experiences a shift of π as one of the quantum paths crosses a band. For resonant interband transitions, the amplitude of the RABBIT oscillation decays as the pump and probe pulses are separated in time due to electronic decoherence, providing a simple interferometric method to extract dephasing times.