Pressure-dependent topological superconductivity on the surface of FeTe0.5Se0.5

FeTe1-xSex is a family of iron-based superconductors with its critical temperature (Tc) dependent on the composition of Se. A well-known Tc is 14.5 K for x = 0.45, which exhibits an s-wave superconducting gap between the topological superconducting surfaces states. Exchange interaction between the electrons has been proposed as the mechanism behind the formation of Cooper pairs for the sample of FeTe0.5Se0.5. In this article we provide further proof that exchange interaction, and hence the associated Tc, depends on the applied pressure on FeTe0.5Se0.5. Using density functional calculations for electrons and phonons and the Bardeen-Cooper-Schrieffer (BCS) theory for superconductivity, we found that Tc and superconducting gap for FeTe0.5Se0.5 soars under increasing compression, consistent with the results of experiment.

Cooper pairs spotted above critical temperature for superconductivity

Researchers have detected Cooper pairs above the critical temperature in a superconductor despite it not having a pseudogap.

Cooper-pair distribution function $$D_{cp}(\omega ,T_c)$$ for superconducting $$\hbox {D}_3\hbox {S}$$ and $$\hbox {H}_3\hbox {S}$$

Cooper-pair distribution function, $$D_{cp}(\omega ,T_c)$$ D cp ( ω , T c ) , is a recent theoretical proposal that reveals information about the superconductor state through the determination of the spectral regions where Cooper pairs are formed. This is built from the well-established Eliashberg spectral function and phonon density of states, calculated by first-principles. From this function is possible to obtain the $$N_{cp}$$ N cp parameter, which is proportional to the total number of Cooper pairs formed at a critical temperature $$T_c$$ T c . Herein, we reported $$D_{cp}(\omega ,T_c)$$ D cp ( ω , T c ) function of the compressed $$D_3S$$ D 3 S and $$H_3S$$ H 3 S high-$$T_c$$ T c conventional superconductors, including the effect of stable sulfur isotopes in $$H_3S$$ H 3 S . $$D_{cp}(\omega ,T_c)$$ D cp ( ω , T c ) suggests that the vibration energy range of 10–70 meV is where the Cooper pairs are possible for these superconductors, pointing out the possible importance of the low-energy region on the electron–phonon superconductivity. This has been confirmed by the fact that a simple variation in the low-frequency region induced for the substitution of S atoms in $$H_3S$$ H 3 S by its stable isotopes can lead to important changes in $$T_c$$ T c . The results also show proportionality between $$N_{cp}$$ N cp parameter and experimental or theoretical $$T_c$$ T c values.

Current Fluctuations in Hybrid-Superconductor Normal Structures with Quantum Dots

<p>Nanostructures with quantum dots in proximity to superconducting electrodes are an ideal tool to study superconducting correlations in systems with few degrees of freedom that exhibit strong Coulomb-interaction effects. Such hybrid superconductor-normal structures show rich physics due to the interplay of superconductivity, Coulomb interaction and non-equilibrium. Superconducting correlations are established on the quantum dot when it is coupled to a superconductor even in the presence of strong Coulomb repulsion and Cooper pairs can tunnel coherently between the quantum dot and the superconductor. In this thesis, we investigate theoretically electronic transport through an interacting quantum dot coupled to normal and superconducting leads. The presence of the proximity effect can be detected by the dot's current, namely the Andreev current. However, current fluctuations might reveal information on the electronic transport and the internal structure of the system which is not visible in the mean value of the current. For this reason, we study the current fluctuations through the proximized quantum dot to get access to the properties of such a hybrid quantum-dot system. In particular, we are interested in the finite-frequency fluctuations to unveil the coherent dynamics underlying the proximity effect in the quantum dot and its internal time scales. At first, we present a study of the frequency-dependent current noise for subgap transport through an interacting single-level quantum dot tunnel-coupled to normal and superconducting leads. For this purpose, we employ a non-equilibrium diagrammatic real-time approach to calculate the finite-frequency current noise. The finite-frequency noise spectrum shows a sharp dip at a frequency corresponding to the energy splitting of the Andreev bound states which is a signature of the coherent exchange of Cooper pairs between the quantum dot and the superconductor. Furthermore, in the high frequency regime, the so called quantum noise regime, the noise spectrum exhibits steps at frequencies equal to the excitation energies. These steps can be related to the effective coupling strength of the excitations. However, the statistical description of the electron transport does not stop with the noise. Current cumulants of arbitrary order can be obtained by means of full counting statistics (FCS). We set up a theory based on the diagrammatic real-time approach to calculate the finite-time FCS for quantum transport with a non-Markovian master equation that captures the initial correlations between system and reservoir. This allows us to fully describe the current fluctuations of the hybrid quantum-dot system, that is the noise and all higher order current cumulants.</p>

Current Fluctuations in Hybrid-Superconductor Normal Structures with Quantum Dots

<p>Nanostructures with quantum dots in proximity to superconducting electrodes are an ideal tool to study superconducting correlations in systems with few degrees of freedom that exhibit strong Coulomb-interaction effects. Such hybrid superconductor-normal structures show rich physics due to the interplay of superconductivity, Coulomb interaction and non-equilibrium. Superconducting correlations are established on the quantum dot when it is coupled to a superconductor even in the presence of strong Coulomb repulsion and Cooper pairs can tunnel coherently between the quantum dot and the superconductor. In this thesis, we investigate theoretically electronic transport through an interacting quantum dot coupled to normal and superconducting leads. The presence of the proximity effect can be detected by the dot's current, namely the Andreev current. However, current fluctuations might reveal information on the electronic transport and the internal structure of the system which is not visible in the mean value of the current. For this reason, we study the current fluctuations through the proximized quantum dot to get access to the properties of such a hybrid quantum-dot system. In particular, we are interested in the finite-frequency fluctuations to unveil the coherent dynamics underlying the proximity effect in the quantum dot and its internal time scales. At first, we present a study of the frequency-dependent current noise for subgap transport through an interacting single-level quantum dot tunnel-coupled to normal and superconducting leads. For this purpose, we employ a non-equilibrium diagrammatic real-time approach to calculate the finite-frequency current noise. The finite-frequency noise spectrum shows a sharp dip at a frequency corresponding to the energy splitting of the Andreev bound states which is a signature of the coherent exchange of Cooper pairs between the quantum dot and the superconductor. Furthermore, in the high frequency regime, the so called quantum noise regime, the noise spectrum exhibits steps at frequencies equal to the excitation energies. These steps can be related to the effective coupling strength of the excitations. However, the statistical description of the electron transport does not stop with the noise. Current cumulants of arbitrary order can be obtained by means of full counting statistics (FCS). We set up a theory based on the diagrammatic real-time approach to calculate the finite-time FCS for quantum transport with a non-Markovian master equation that captures the initial correlations between system and reservoir. This allows us to fully describe the current fluctuations of the hybrid quantum-dot system, that is the noise and all higher order current cumulants.</p>

Real-time observation of Cooper pair splitting showing strong non-local correlations

Controlled generation and detection of quantum entanglement between spatially separated particles constitute an essential prerequisite both for testing the foundations of quantum mechanics and for realizing future quantum technologies. Splitting of Cooper pairs from a superconductor provides entangled electrons at separate locations. However, experimentally accessing the individual split Cooper pairs constitutes a major unresolved issue as they mix together with electrons from competing processes. Here, we overcome this challenge with the first real-time observation of the splitting of individual Cooper pairs, enabling direct access to the time-resolved statistics of Cooper pair splitting. We determine the correlation statistics arising from two-electron processes and find a pronounced peak that is two orders of magnitude larger than the background. Our experiment thereby allows to unambiguously pinpoint and select split Cooper pairs with 99% fidelity. These results open up an avenue for performing experiments that tap into the spin-entanglement of split Cooper pairs.