scholarly journals Current Fluctuations in Hybrid-Superconductor Normal Structures with Quantum Dots

2021 ◽  
Author(s):  
◽  
Stephanie Droste

<p>Nanostructures with quantum dots in proximity to superconducting electrodes are an ideal tool to study superconducting correlations in systems with few degrees of freedom that exhibit strong Coulomb-interaction effects. Such hybrid superconductor-normal structures show rich physics due to the interplay of superconductivity, Coulomb interaction and non-equilibrium. Superconducting correlations are established on the quantum dot when it is coupled to a superconductor even in the presence of strong Coulomb repulsion and Cooper pairs can tunnel coherently between the quantum dot and the superconductor.  In this thesis, we investigate theoretically electronic transport through an interacting quantum dot coupled to normal and superconducting leads. The presence of the proximity effect can be detected by the dot's current, namely the Andreev current. However, current fluctuations might reveal information on the electronic transport and the internal structure of the system which is not visible in the mean value of the current. For this reason, we study the current fluctuations through the proximized quantum dot to get access to the properties of such a hybrid quantum-dot system. In particular, we are interested in the finite-frequency fluctuations to unveil the coherent dynamics underlying the proximity effect in the quantum dot and its internal time scales.  At first, we present a study of the frequency-dependent current noise for subgap transport through an interacting single-level quantum dot tunnel-coupled to normal and superconducting leads. For this purpose, we employ a non-equilibrium diagrammatic real-time approach to calculate the finite-frequency current noise. The finite-frequency noise spectrum shows a sharp dip at a frequency corresponding to the energy splitting of the Andreev bound states which is a signature of the coherent exchange of Cooper pairs between the quantum dot and the superconductor. Furthermore, in the high frequency regime, the so called quantum noise regime, the noise spectrum exhibits steps at frequencies equal to the excitation energies. These steps can be related to the effective coupling strength of the excitations.  However, the statistical description of the electron transport does not stop with the noise. Current cumulants of arbitrary order can be obtained by means of full counting statistics (FCS). We set up a theory based on the diagrammatic real-time approach to calculate the finite-time FCS for quantum transport with a non-Markovian master equation that captures the initial correlations between system and reservoir. This allows us to fully describe the current fluctuations of the hybrid quantum-dot system, that is the noise and all higher order current cumulants.</p>

2021 ◽  
Author(s):  
◽  
Stephanie Droste

<p>Nanostructures with quantum dots in proximity to superconducting electrodes are an ideal tool to study superconducting correlations in systems with few degrees of freedom that exhibit strong Coulomb-interaction effects. Such hybrid superconductor-normal structures show rich physics due to the interplay of superconductivity, Coulomb interaction and non-equilibrium. Superconducting correlations are established on the quantum dot when it is coupled to a superconductor even in the presence of strong Coulomb repulsion and Cooper pairs can tunnel coherently between the quantum dot and the superconductor.  In this thesis, we investigate theoretically electronic transport through an interacting quantum dot coupled to normal and superconducting leads. The presence of the proximity effect can be detected by the dot's current, namely the Andreev current. However, current fluctuations might reveal information on the electronic transport and the internal structure of the system which is not visible in the mean value of the current. For this reason, we study the current fluctuations through the proximized quantum dot to get access to the properties of such a hybrid quantum-dot system. In particular, we are interested in the finite-frequency fluctuations to unveil the coherent dynamics underlying the proximity effect in the quantum dot and its internal time scales.  At first, we present a study of the frequency-dependent current noise for subgap transport through an interacting single-level quantum dot tunnel-coupled to normal and superconducting leads. For this purpose, we employ a non-equilibrium diagrammatic real-time approach to calculate the finite-frequency current noise. The finite-frequency noise spectrum shows a sharp dip at a frequency corresponding to the energy splitting of the Andreev bound states which is a signature of the coherent exchange of Cooper pairs between the quantum dot and the superconductor. Furthermore, in the high frequency regime, the so called quantum noise regime, the noise spectrum exhibits steps at frequencies equal to the excitation energies. These steps can be related to the effective coupling strength of the excitations.  However, the statistical description of the electron transport does not stop with the noise. Current cumulants of arbitrary order can be obtained by means of full counting statistics (FCS). We set up a theory based on the diagrammatic real-time approach to calculate the finite-time FCS for quantum transport with a non-Markovian master equation that captures the initial correlations between system and reservoir. This allows us to fully describe the current fluctuations of the hybrid quantum-dot system, that is the noise and all higher order current cumulants.</p>


2006 ◽  
Vol 6 (11) ◽  
pp. 3329-3332 ◽  
Author(s):  
Heejun Jeong

We have measured the electronic transport properties of the coupled quantum dot devices at low temperatures. The interplay between the strong many body spin interaction and the molecular states are probed in linear and non-linear transport regime. We observe the formation of strong coherent molecular states clearly visible in the double dot conductance phase diagram. In our study, the spin configuration in multiply coupled quantum dots could be identified using Kondo phenomenon. In addition, the characteristics of the spin dependent molecular states and phase dependant tunneling have been also observed using non-linear conductance measurement of the double dots. The results suggest the importance of the diverse spin related physical issues in artificial quantum dot devices.


2020 ◽  
Vol 32 (16) ◽  
pp. 165601
Author(s):  
Denis Zhuravel ◽  
Dmitry V Anchishkin ◽  
Roland Hayn ◽  
Pierre Lombardo ◽  
Steffen Schäfer

2021 ◽  
Author(s):  
Xu Dan ◽  
Ruiyi Li ◽  
Qinsheng Wang ◽  
Yongqiang Yang ◽  
Haiyan Zhu ◽  
...  

The paper reports the synthesis of nickel-silver-graphene quantum dot-graphene hybrid. Histidine-functionalized graphene quantum dots (His-GQDs) were bonded to graphene oxide (GO) and then combined with Ni2+ and Ag+ to form...


Molecules ◽  
2021 ◽  
Vol 26 (15) ◽  
pp. 4439
Author(s):  
Shui-Yang Lien ◽  
Yu-Hao Chen ◽  
Wen-Ray Chen ◽  
Chuan-Hsi Liu ◽  
Chien-Jung Huang

In this study, adding CsPbI3 quantum dots to organic perovskite methylamine lead triiodide (CH3NH3PbI3) to form a doped perovskite film filmed by different temperatures was found to effectively reduce the formation of unsaturated metal Pb. Doping a small amount of CsPbI3 quantum dots could enhance thermal stability and improve surface defects. The electron mobility of the doped film was 2.5 times higher than the pristine film. This was a major breakthrough for inorganic quantum dot doped organic perovskite thin films.


2021 ◽  
Author(s):  
Xianfeng Zhang ◽  
Zongqun Li ◽  
Shaowen Xu ◽  
Yaowen Ruan

TiO2/CQD composites were synthesized through carbon quantum dots covalently attached to the surface of hollow TiO2 spheres for visible light photocatalytic degradation of organics.


2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Long Hu ◽  
Qian Zhao ◽  
Shujuan Huang ◽  
Jianghui Zheng ◽  
Xinwei Guan ◽  
...  

AbstractAll-inorganic CsPbI3 perovskite quantum dots have received substantial research interest for photovoltaic applications because of higher efficiency compared to solar cells using other quantum dots materials and the various exciting properties that perovskites have to offer. These quantum dot devices also exhibit good mechanical stability amongst various thin-film photovoltaic technologies. We demonstrate higher mechanical endurance of quantum dot films compared to bulk thin film and highlight the importance of further research on high-performance and flexible optoelectronic devices using nanoscale grains as an advantage. Specifically, we develop a hybrid interfacial architecture consisting of CsPbI3 quantum dot/PCBM heterojunction, enabling an energy cascade for efficient charge transfer and mechanical adhesion. The champion CsPbI3 quantum dot solar cell has an efficiency of 15.1% (stabilized power output of 14.61%), which is among the highest report to date. Building on this strategy, we further demonstrate a highest efficiency of 12.3% in flexible quantum dot photovoltaics.


2021 ◽  
Vol 52 (1) ◽  
pp. 953-956
Author(s):  
Tatsuya Ryowa ◽  
Yusuke Sakakibara ◽  
Tadashi Kobashi ◽  
Keisuke Kitano ◽  
Masaya Ueda ◽  
...  

2008 ◽  
Vol 20 (14) ◽  
pp. 1240-1242 ◽  
Author(s):  
Chi-Che Tseng ◽  
Shu-Ting Chou ◽  
Yi-Hao Chen ◽  
Cheng-Nan Chen ◽  
Wei-Hsun Lin ◽  
...  

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