Impact of Short-Term Emission Control Measures on Air Quality in Nanjing During the Jiangsu Development Summit

This study analyzed the effectiveness of temporary emission control measures on air quality of Nanjing, China during the Jiangsu Development Summit (JDS). We employed a regional chemistry model WRF-Chem to simulate air pollutants in Nanjing and compared the results to surface observations and satellite retrievals. During the JDS, air pollutant emissions from industry and transportation sectors largely decreased by 50–67% due to the short-term emission control measures such as reducing coal combustions, shutting down factories, and partially limiting traffic. Benefiting from the emission control, the simulated concentrations of PM2.5, NO2, SO2, CO and VOCs in Nanjing decreased by 17%, 20%, 20%, 19%, and 15% respectively, consistent with the surface and satellite observations. However, both the observed and simulated O3 increased by 3–48% during the JDS, which was mainly due to the remarkable NOx emission reduction (26%) in the downtown of Nanjing where the O3 production regime was mainly VOC-controlled. In addition, the atmospheric oxidation capacity and further the sulfur oxidation ratio, were facilitated by the elevated O3, which led to variable mitigation efficiencies of different secondary PM2.5 compositions. Our study offers an opportunity for understanding the coordinated control of PM2.5 and O3 in typical city clusters, and can provide implications for future mitigation actions.

Reduced light absorption of black carbon (BC) and its influence on BC-boundary-layer interactions during “APEC Blue”

Light absorption and radiative forcing of black carbon (BC) is influenced by both BC itself and its interactions with other aerosol chemical compositions. Although the changes in BC concentrations in response to emission reduction measures have been well documented, the influence of emission reductions on the light absorption properties of BC and its influence on BC-boundary-layer interactions has been less explored. In this study, we used the online coupled WRF-Chem model to examine how emission control measures during the Asia-Pacific Economic Cooperation (APEC) summit affect the mixing state and light absorption of BC, and the associated implications for BC-PBL interactions. We found that both the mass concentration of BC and the BC coating materials declined during the APEC week, which reduced the light absorption and light absorption enhancement (Eab) of BC. The reduced absorption aerosol optical depth (AAOD) during APEC was caused by both the decline in the mass concentration of BC itself (52.0 %), and the lensing effect of BC (48.0 %). The reduction in coating materials (39.4 %) contributed the most to the influence of the lensing effect, and the reduced light absorption capability (Eab) contributed 3.2 % to the total reduction in AAOD. Reduced light absorption of BC due to emission control during APEC enhanced planetary boundary layer height (PBLH) by 8.2 m. PM2.5 and O3 were found to have different responses to the changes in the light absorption of BC. Reduced light absorption of BC due to emission reductions decreased near-surface PM2.5 concentrations but near-surface O3 concentrations were enhanced in the North China Plain. These results suggest that current measures to control SO2, NOx, etc. would be effective in reducing the absorption enhancement of BC and in inhibiting the feedback of BC on the boundary layer. However, enhanced ground O3 might be a side effect of current emission control strategies. How to control emissions to offset this side effect of current emission control measures on O3 should be an area of further focus.

Reduced light absorption of black carbon (BC) and its influence on BC-boundary-layer interactions during APEC Blue

Light absorption and radiative forcing of black carbon (BC) is influenced by both BC itself and its interactions with other aerosol chemical compositions. Although the changes in BC concentrations in response to emission reduction measures have been well documented, the influence of emission reductions on the light absorption properties of BC and its influence on BC-boundary-layer interactions has been less explored. In this study, we used the online coupled WRF-Chem model to examine how emission control measures during APEC affect the mixing state/light absorption of BC, and the associated implications for BC-PBL interactions. We found that both the mass concentration of BC and the BC coating materials declined during the APEC week, which reduced the light absorption and light absorption enhancement (Eab) of BC. The reduced absorption aerosol optical depth (AAOD) during APEC were caused by both the declines in mass concentration of BC itself (52.0 %), and the lensing effect of BC (48.0 %). The reductions in coating materials (39.4 %) dominated the influence of lensing effect, and the reduced light absorption capability (Eab) contributed 3.2 % to the total reductions in AAOD. Reduced light absorption of BC due to emission control during APEC enhanced planetary boundary layer height (PBLH) by 8.2 m. Different responses of PM2.5 and O3 were found to the changes in light absorption of BC. Reduced light absorption of BC due to emission reductions decreased near surface PM2.5 concentrations but enhanced near surface O3 concentrations in the North China Plain. These results suggest that current measures to control SO2, NOx, etc. would be efficient to reduce the absorption enhancement of BC, and to inhibit the feedback of BC on boundary layer. Yet enhanced ground O3 might be a side effect of current emission control strategies. How to control emissions to offset this side effect of current emission control measures on O3 should be an area of further focus.

Significant wintertime PM_2.5 mitigation in the Yangtze River Delta, China, from 2016 to 2019: observational constraints on anthropogenic emission controls

Ambient fine particulate matter (PM2.5) mitigation relies strongly on anthropogenic emission control measures, the actual effectiveness of which is challenging to pinpoint owing to the complex synergies between anthropogenic emissions and meteorology. Here, observational constraints on model simulations allow us to derive not only reliable PM2.5 evolution but also accurate meteorological fields. On this basis, we isolate meteorological factors to achieve reliable estimates of surface PM2.5 responses to both long-term and emergency emission control measures from 2016 to 2019 over the Yangtze River Delta (YRD), China. The results show that long-term emission control strategies play a crucial role in curbing PM2.5 levels, especially in the megacities and other areas with abundant anthropogenic emissions. The G20 summit hosted in Hangzhou in 2016 provides a unique and ideal opportunity involving the most stringent, even unsustainable, emergency emission control measures. These emergency measures lead to the largest decrease (∼ 35 µg m−3, ∼ 59 %) in PM2.5 concentrations in Hangzhou. The hotspots also emerge in megacities, especially in Shanghai (32 µg m−3, 51 %), Nanjing (27 µg m−3, 55 %), and Hefei (24 µg m−3, 44 %) because of the emergency measures. Compared to the long-term policies from 2016 to 2019, the emergency emission control measures implemented during the G20 Summit achieve more significant decreases in PM2.5 concentrations (17 µg m−3 and 41 %) over most of the whole domain, especially in Hangzhou (24 µg m−3, 48 %) and Shanghai (21 µg m−3, 45 %). By extrapolation, we derive insight into the magnitude and spatial distribution of PM2.5 mitigation potential across the YRD, revealing significantly additional room for curbing PM2.5 levels.

Significant wintertime PM_2.5 mitigation in the Yangtze River Delta, China from 2016 to 2019: observational constraints on anthropogenic emission controls

Ambient fine particulate matter (PM2.5) mitigation relies strongly on anthropogenic emission control measures, the actual effectiveness of which is challenging to pinpoint owing to the complex synergies between anthropogenic emissions and meteorology. Here, observational constraints on model simulations allow us to derive not only reliable PM2.5 evolution but also accurate meteorological fields. In this study, we isolate meteorological factors to achieve reliable estimates of surface PM2.5 responses to both long-term and emergency emission control measures from 2016 to 2019 over the Yangtze River Delta (YRD), China. The results show that long-term emission control strategies play a crucial role in curbing PM2.5 levels (> 14 μg/m3, 19 %), especially in the megacities and other areas with abundant anthropogenic emissions. The G20 summit hosted in Hangzhou in 2016 provides a unique and ideal opportunity involving the most stringent, even unsustainable, emergency emission control measures. For the winter time periods from 2016 to 2019, the most substantial declines in PM2.5 concentrations (~ 35 μg/m3, ~ 59 %) are thus achieved in Hangzhou and its surrounding areas. The following hotspots also emerge in megacities, especially in Shanghai (32 μg/m3, 51 %), Nanjing (27 μg/m3, 55 %), and Hefei (24 μg/m3, 44 %). Compared to the long-term policies from 2016 to 2019, the emergency emission control measures implemented during the G20 Summit achieve more significant decreases in PM2.5 concentrations (17 μg/m3 and 41 %) over most of the whole domain, especially in Hangzhou (24 μg/m3, 48 %) and Shanghai (21 μg/m3, 45 %). By extrapolation, we derive insight into the magnitude and spatial distributions of PM2.5 mitigation potentials across the YRD, revealing significantly additional rooms for curbing PM2.5 levels.

China’s emission control strategies have suppressed unfavorable influences of climate on wintertime PM2.5 concentrations in Beijing since 2002

<p>Severe wintertime PM2.5 pollution in Beijing has been receiving increasing worldwide attention, yet the decadal variations remain relatively unexplored. Combining field measurements and model simulations, we quantified the relative influences of anthropogenic emissions and meteorological conditions on PM2.5 concentrations in Beijing overwinters of 2002-2016. Between the winters of 2011 and 2016, stringent emission control measures resulted in a 21% decrease in mean mass concentrations of PM2.5 in Beijing, with 7 fewer haze days per winter on average. Given the overestimation of PM2.5 by model, the effectiveness of stringent emission control measures might have been slightly overstated. With fixed emissions, meteorological conditions over the study period would have led to an increase of haze in Beijing, but the strict emission control measures have suppressed the unfavorable influences of recent climate. The unfavorable meteorological conditions are attributed to the weakening of the East Asia Winter Monsoon associated particularly with an increase in pressure associated with the Aleutian low.</p>

China's emission control strategies have suppressed unfavorable influences of climate on wintertime PM_2.5 concentrations in Beijing since 2002

Severe wintertime PM2.5 pollution in Beijing has been receiving increasing worldwide attention, yet the decadal variations remain relatively unexplored. Combining field measurements and model simulations, we quantified the relative influences of anthropogenic emissions and meteorological conditions on PM2.5 concentrations in Beijing over the winters of 2002–2016. Between the winters of 2011 and 2016, stringent emission control measures resulted in a 21 % decrease in mean mass concentrations of PM2.5 in Beijing, with 7 fewer haze days per winter on average. Given the overestimation of PM2.5 by the model, the effectiveness of stringent emission control measures might have been slightly overstated. With fixed emissions, meteorological conditions over the study period would have led to an increase in haze in Beijing, but the strict emission control measures have suppressed the unfavorable influences of the recent climate. The unfavorable meteorological conditions are attributed to the weakening of the East Asia winter monsoon associated particularly with an increase in pressure associated with the Aleutian Low.