Influences of Recent Particle Formation on Southern Ocean Aerosol Variability and Low Cloud Properties

2021 ◽  
Author(s):  
Isabel L. McCoy ◽  
Christopher S. Bretherton ◽  
Robert Wood ◽  
Cynthia H. Twohy ◽  
Andrew Gettelman ◽  
...  
Keyword(s):  
Southern Ocean ◽  
Particle Formation ◽  
Cloud Properties ◽  
Low Cloud

Influences of Recent Particle Formation on Southern Ocean Aerosol Variability and Low Cloud Properties

2021 ◽  
Author(s):  
Isabel L. McCoy ◽  
Christopher S. Bretherton ◽  
Robert Wood ◽  
Cynthia H. Twohy ◽  
Andrew Gettelman ◽  
...  
Keyword(s):  
Southern Ocean ◽  
Particle Formation ◽  
Cloud Properties ◽  
Low Cloud

scholarly journals Instantaneous Linkages between Clouds and Large-Scale Meteorology over the Southern Ocean in Observations and a Climate Model

2017 ◽  
Vol 30 (23) ◽  
pp. 9455-9474 ◽  
Author(s):  
Casey J. Wall ◽  
Dennis L. Hartmann ◽  
Po-Lun Ma
Keyword(s):  
Southern Ocean ◽  
Large Scale ◽  
Climate Models ◽  
Climate Model ◽  
Austral Summer ◽  
Vertical Motion ◽  
Cloud Properties ◽  
Low Clouds ◽  
Community Atmosphere Model ◽  
Low Cloud

Instantaneous, coincident, footprint-level satellite observations of cloud properties and radiation taken during austral summer over the Southern Ocean are used to study relationships between clouds and large-scale meteorology. Cloud properties are very sensitive to the strength of vertical motion in the midtroposphere, and low-cloud properties are sensitive to estimated inversion strength, low-level temperature advection, and sea surface temperature. These relationships are quantified. An index for the meteorological anomalies associated with midlatitude cyclones is presented, and it is used to reveal the sensitivity of clouds to the meteorology within the warm and cold sectors of cyclones. The observed relationships between clouds and meteorology are compared to those in the Community Atmosphere Model, version 5 (CAM5), using satellite simulators. Low clouds simulated by CAM5 are too few, are too bright, and contain too much ice. In the cold sector of cyclones, the low clouds are also too sensitive to variations in the meteorology. When CAM5 is coupled with an updated boundary layer parameterization known as Cloud Layers Unified by Binormals (CLUBB), bias in the ice content of low clouds is dramatically reduced. More generally, this study demonstrates that examining the instantaneous time scale is a powerful approach to understanding the physical processes that control clouds and how they are represented in climate models. Such an evaluation goes beyond the cloud climatology and exposes model bias under various meteorological conditions.

scholarly journals Iodine observed in new particle formation events in the Arctic atmosphere during ACCACIA

2014 ◽  
Vol 14 (21) ◽  
pp. 28949-28972 ◽  
Author(s):  
J. D. Allan ◽  
P. I. Williams ◽  
J. Najera ◽  
J. D. Whitehead ◽  
M. J. Flynn ◽  
...  
Keyword(s):  
Sea Ice ◽  
Molecular Iodine ◽  
Particle Formation ◽  
The Arctic ◽  
New Particle Formation ◽  
Sulphur Compounds ◽  
Cloud Properties ◽  
Coastal Sea ◽  
Arctic Atmosphere ◽  
Initial Source

Abstract. Accurately accounting for new particle formation (NPF) is crucial to our ability to predict aerosol number concentrations and thus cloud properties, which is in turn vital in simulating radiative transfer and climate. Here we present an analysis of NPF events observed in the Greenland Sea during the summertime as part of the Aerosol-Cloud Coupling And Climate Interactions in the Arctic (ACCACIA) project. While NPF events have been reported in the Arctic before, we were able, for the first time, to detect iodine in the growing particles using an Aerosol Mass Spectrometer (AMS) during a persistent event in the region of the coastal sea ice near Greenland. Given the potency of iodine as a nucleation precursor, the results imply that iodine was responsible for the initial NPF, a phenomenon that has been reported at lower latitudes and associated with molecular iodine emissions from coastal macroalgae. The initial source of iodine in this instance is not clear, but it was associated with air originating approximately 1 day previously over melting coastal sea ice. These results show that atmospheric models must consider iodine as a source of new particles in addition to established precursors such as sulphur compounds.

International Satellite Cloud Climatology Project: Extending the Record

2021 ◽  
pp. 1-62
Author(s):  
William B. Rossow ◽  
Kenneth R. Knapp ◽  
Alisa H Young
Keyword(s):  
Product Design ◽  
Cloud Amount ◽  
Cloud Microphysics ◽  
Temperature Threshold ◽  
Ancillary Data ◽  
Total Cloud Amount ◽  
High Cloud ◽  
Enso Events ◽  
Cloud Properties ◽  
Low Cloud

AbstractISCCP continues to quantify the global distribution and diurnal-to-interannual variations of cloud properties in a revised version. This paper summarizes assessments of the previous version, describes refinements of the analysis and enhanced features of the product design, discusses the few notable changes in the results, and illustrates the long-term variations of global mean cloud properties and differing high cloud changes associated with ENSO. The new product design includes a global, pixel-level product on a 0.1°?grid, all other gridded products at 1.0°-equivalent equal-area, separate-satellite products with ancillary data for regional studies, more detailed, embedded quality information, and all gridded products in netCDF format. All the data products including all input data), expanded documentation, the processing code and an Operations Guide are available online. Notable changes are: (1) a lowered ice-liquid temperature threshold, (2) a treatment of the radiative effects of aerosols and surface temperature inversions, (3) refined specification of the assumed cloud microphysics, and (4) interpolation of the main daytime cloud information overnight. The changes very slightly increase the global monthly mean cloud amount with a little more high and a little less middle and low cloud. Over the whole period, total cloud amount slowly decreases caused by decreases in cumulus/altocumulus; consequently, average cloud top temperature and optical thickness have increased. The diurnal and seasonal cloud variations are very similar to earlier versions. Analysis of the whole record shows that high cloud variations, but not low clouds, exhibit different patterns in different ENSO events.

Observed Southern Ocean Cloud Properties and Shortwave Reflection. Part I: Calculation of SW Flux from Observed Cloud Properties*

2014 ◽  
Vol 27 (23) ◽  
pp. 8836-8857 ◽  
Author(s):  
Daniel T. McCoy ◽  
Dennis L. Hartmann ◽  
Daniel P. Grosvenor
Keyword(s):  
Seasonal Variation ◽  
Solar Radiation ◽  
Southern Ocean ◽  
Water Content ◽  
Liquid Water ◽  
Effective Radius ◽  
Shortwave Radiation ◽  
Liquid Water Path ◽  
Cloud Liquid Water ◽  
Cloud Properties

Abstract The sensitivity of the reflection of shortwave radiation over the Southern Ocean to the cloud properties there is estimated using observations from a suite of passive and active satellite instruments in combination with radiative transfer modeling. A composite cloud property observational data description is constructed that consistently incorporates mean cloud liquid water content, ice water content, liquid and ice particle radius information, vertical structure, vertical overlap, and spatial aggregation of cloud water as measured by optical depth versus cloud-top pressure histograms. The observational datasets used are Moderate Resolution Imaging Spectroradiometer (MODIS) effective radius filtered to mitigate solar zenith angle bias, the Multiangle Imaging Spectroradiometer (MISR) cloud-top height–optical depth (CTH–OD) histogram, the liquid water path from the University of Wisconsin dataset, and ice cloud properties from CloudSat. This cloud database is used to compute reflected shortwave radiation as a function of month and location over the ocean from 40° to 60°S, which compares well with observations of reflected shortwave radiation. This calculation is then used to test the sensitivity of the seasonal variation of shortwave reflection to the observed seasonal variation of cloud properties. Effective radius decreases during the summer season, which results in an increase in reflected solar radiation of 4–8 W m−2 during summer compared to what would be reflected if the effective radius remained constant at its annual-mean value. Summertime increases in low cloud fraction similarly increase the summertime reflection of solar radiation by 9–11 W m−2. In-cloud liquid water path is less in summertime, causing the reflected solar radiation to be 1–4 W m−2 less.

scholarly journals Evaluation of Southern Ocean cloud in the HadGEM3 general circulation model and MERRA-2 reanalysis using ship-based observations

2020 ◽  
Vol 20 (11) ◽  
pp. 6607-6630 ◽  
Author(s):  
Peter Kuma ◽  
Adrian J. McDonald ◽  
Olaf Morgenstern ◽  
Simon P. Alexander ◽  
John J. Cassano ◽  
...  
Keyword(s):  
Boundary Layer ◽  
Southern Ocean ◽  
General Circulation ◽  
Cloud Cover ◽  
Atmospheric Stability ◽  
Austral Summer ◽  
Circulation Model ◽  
Radiation Budget ◽  
Cloud Albedo ◽  
Low Cloud

Abstract. Southern Ocean (SO) shortwave (SW) radiation biases are a common problem in contemporary general circulation models (GCMs), with most models exhibiting a tendency to absorb too much incoming SW radiation. These biases have been attributed to deficiencies in the representation of clouds during the austral summer months, either due to cloud cover or cloud albedo being too low. The problem has been the focus of many studies, most of which utilised satellite datasets for model evaluation. We use multi-year ship-based observations and the CERES spaceborne radiation budget measurements to contrast cloud representation and SW radiation in the atmospheric component Global Atmosphere (GA) version 7.1 of the HadGEM3 GCM and the MERRA-2 reanalysis. We find that the prevailing bias is negative in GA7.1 and positive in MERRA-2. GA7.1 performs better than MERRA-2 in terms of absolute SW bias. Significant errors of up to 21 W m−2 (GA7.1) and 39 W m−2 (MERRA-2) are present in both models in the austral summer. Using ship-based ceilometer observations, we find low cloud below 2 km to be predominant in the Ross Sea and the Indian Ocean sectors of the SO. Utilising a novel surface lidar simulator developed for this study, derived from an existing Cloud Feedback Model Intercomparison Project (CFMIP) Observation Simulator Package (COSP) – active remote sensing simulator (ACTSIM) spaceborne lidar simulator, we find that GA7.1 and MERRA-2 both underestimate low cloud and fog occurrence relative to the ship observations on average by 4 %–9 % (GA7.1) and 18 % (MERRA-2). Based on radiosonde observations, we also find the low cloud to be strongly linked to boundary layer atmospheric stability and the sea surface temperature. GA7.1 and MERRA-2 do not represent the observed relationship between boundary layer stability and clouds well. We find that MERRA-2 has a much greater proportion of cloud liquid water in the SO in austral summer than GA7.1, a likely key contributor to the difference in the SW radiation bias. Our results suggest that subgrid-scale processes (cloud and boundary layer parameterisations) are responsible for the bias and that in GA7.1 a major part of the SW radiation bias can be explained by cloud cover underestimation, relative to underestimation of cloud albedo.

scholarly journals Subseasonal variability of low cloud radiative properties over the southeast Pacific Ocean

2010 ◽  
Vol 10 (8) ◽  
pp. 4047-4063 ◽  
Author(s):  
R. C. George ◽  
R. Wood
Keyword(s):  
Large Scale ◽  
Cloud Fraction ◽  
Radiative Properties ◽  
Pressure System ◽  
Cloud Albedo ◽  
Cloud Properties ◽  
Droplet Concentration ◽  
Subseasonal Variability ◽  
Low Cloud ◽  
Macrophysical Properties

Abstract. Subseasonal variability of cloud radiative properties in the persistent southeast Pacific stratocumulus deck is investigated using MODIS satellite observations and NCEP reanalysis data. A once-daily albedo proxy is derived based on the fractional coverage of low cloud (a macrophysical field) and the cloud albedo, with the latter broken down into contributions from microphysics (cloud droplet concentration) and macrophysics (liquid water path). Subseasonal albedo variability is dominated by the contribution of low cloud fraction variability, except within 10–15° of the South American coast, where cloud albedo variability contributes significantly. Covariance between cloud fraction and cloud albedo also contributes significantly and positively to the variance in albedo, which highlights how complex and inseparable the factors controlling albedo are. Droplet concentration variability contributes only weakly to the subseasonal variability of albedo, which emphasizes that attributing albedo variability to the indirect effects of aerosols against the backdrop of natural meteorological variability is extremely challenging. The dominant large scale meteorological variability is associated with the subtropical high pressure system. Two indices representing changes in the subtropical high strength and extent explain 80–90% of this variability, and significantly modulate the cloud microphysical, macrophysical, and radiative cloud properties. Variations in droplet concentration of up to 50% of the mean are associated with the meteorological driving. We hypothesize that these fluctuations in droplet concentration are a result of the large scale meteorology and their correlation with cloud macrophysical properties should not be used as evidence of aerosol effects. Mechanisms by which large scale meteorology affects cloud properties are explored. Our results support existing hypotheses linking cloud cover variability to changes in cold advection, subsidence, and lower tropospheric stability. Within 10° of the coast interactions between variability in the surface high pressure system and the orography appear to modulate both cloud macrophysical properties and aerosol transport through suppression of the marine boundary layer depth near the coast. This suggests one possible way in which cloud macrophysical properties and droplet concentration may be correlated independently of the second aerosol indirect effect. The results provide variability constraints for models that strive to represent both meteorological and aerosol impacts on stratocumulus clouds.

Evaluation of ACCESS model cloud properties over the Southern Ocean area using multiple-satellite products

2015 ◽  
Vol 142 (694) ◽  
pp. 160-171 ◽  
Author(s):  
San Luo ◽  
Zhian Sun ◽  
Xiaogu Zheng ◽  
Lawrie Rikus ◽  
Charmaine Franklin
Keyword(s):  
Southern Ocean ◽  
Ocean Area ◽  
Cloud Properties ◽  
Model Cloud ◽  
Access Model

The Southern Ocean Cloud project

2021 ◽  
Author(s):  
Tom Lachlan-Cope ◽  
Amelie Kirchgaessner ◽  
Anna Jones ◽  
Jo Browse ◽  
David Topping ◽  
...  
Keyword(s):  
Southern Ocean ◽  
Production Control ◽  
Size Spectrum ◽  
Climate Modelling ◽  
Oceanic Circulation ◽  
Aerosol Composition ◽  
Atlantic Sector ◽  
Cloud Properties ◽  
Cloud Development ◽  
The Uk

<p>The Southern Ocean Cloud (SOC) project is funded by the UK Natural Environment Research Council to investigate clouds, particularly mixed-phase, in the Atlantic sector of the Southern Ocean and how aerosol sources and production control clouds properties. Here we aim to introduce the community to the project and any associated opportunities that might be available. At high Southern latitudes models are relatively poor at representing clouds and this has an impact on the energy balance and hence atmospheric and oceanic circulation both locally and globally. This project will investigate those processes that control cloud development and will concentrate on the aerosol that act as cloud nuclei, the source of these nuclei and how aerosol and microphysical processes are modelled.</p><p> </p><p>It is planned to deploy instruments to the British Antarctic Survey (BAS) research stations Rothera and Bird Island research stations as well as on the BAS research vessel. These instruments will measure the aerosol size spectrum at all stations and in addition CCN and INP numbers, cloud properties (with a polarized lidar) and aerosol composition at Rothera. The instruments will be deployed for at least 3 years, although some instruments may be moved from Rothera to the ship for special observing periods.</p><p> </p><p>In addition to the long-term measurements there will be two special observing periods (SOPs), the first in the 2022/23 Antarctic season will consist of a dedicated ship cruise and an airborne campaign using the BAS instrumented twin otter aircraft along with enhanced observations at the surface stations. The second SOP will also have enhanced observations at the surface stations along with an airborne campaign.</p><p> </p><p>The observations will be backed up with a programme of aerosol, weather and climate modelling. The combination of modelling and observations should enable us to identify the major sources of cloud nuclei over the Southern Ocean, examine their role in cloud development, and improve the representation of these processes in models.</p><p> </p>

scholarly journals Iodine observed in new particle formation events in the Arctic atmosphere during ACCACIA

2015 ◽  
Vol 15 (10) ◽  
pp. 5599-5609 ◽  
Author(s):  
J. D. Allan ◽  
P. I. Williams ◽  
J. Najera ◽  
J. D. Whitehead ◽  
M. J. Flynn ◽  
...  
Keyword(s):  
Sea Ice ◽  
Molecular Iodine ◽  
Particle Formation ◽  
The Arctic ◽  
New Particle Formation ◽  
Cloud Properties ◽  
Aerosol Mass ◽  
Coastal Sea ◽  
Arctic Atmosphere ◽  
Initial Source

Abstract. Accurately accounting for new particle formation (NPF) is crucial to our ability to predict aerosol number concentrations in many environments and thus cloud properties, which is in turn vital in simulating radiative transfer and climate. Here we present an analysis of NPF events observed in the Greenland Sea during the summertime as part of the Aerosol-Cloud Coupling And Climate Interactions in the Arctic (ACCACIA) project. While NPF events have been reported in the Arctic before, we were able, for the first time, to detect iodine in the growing particles using an Aerosol Mass Spectrometer (AMS) during a persistent event in the region of the coastal sea-ice near Greenland. Given the potency of iodine as a nucleation precursor, the results imply that iodine was responsible for the initial NPF, a phenomenon that has been reported at lower latitudes and associated with molecular iodine emissions from coastal macroalgae. The initial source of iodine in this instance is not clear, but it was associated with air originating approximately 1 day previously over melting coastal sea-ice. These results show that atmospheric models must consider iodine as a source of new particles in addition to established precursors such as sulfur compounds.

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