<p>Surface seawater carbon dioxide was observed from 3 &#176;S to 27 &#176;S along 67 &#176;E of the Indian Ocean in April 2018 and 2019. Partial pressure of CO<sub>2</sub>(pCO<sub>2</sub>) in the surface seawater and the atmosphere were observed every two minutes using an underway CO2 measurement system (General Oceanics Model 8050) installed on R/V Isabu. Surface water temperature and salinity were measured as well. The pCO<sub>2</sub> was measured using Li-7000 NDIR. Standard gases were measured every 8 hours in five classes with concentrations of 0 &#181;atm, 202 &#181;atm, 350 &#181;atm, 447 &#181;atm, and 359.87 &#181;atm. The fCO<sub>2</sub> of atmosphere remained nearly constant at 387 &#177; 2 &#181;atm, but the surface seawater fCO<sub>2</sub> peaked at about 3 &#176;S and tended to decrease toward the north and south. The distribution of fCO<sub>2</sub> in surface seawater according to latitude tends to be very similar to that of sea surface temperature. In order to investigate the factors that control the distribution of fCO<sub>2</sub> in surface seawater, we analyzed the sea surface temperature, sea surface salinity, and other factors. The effects of salinity are insignificant, and the surface fCO<sub>2</sub> distribution is mainly controlled by sea surface temperature and other factors that can be represented mainly by biological activity and mixing.</p>