scholarly journals The impact of rainfall events, catchment characteristics and estuarine processes on the export of dissolved organic matter from two lowland rivers and their shared estuary

2020 ◽  
Vol 735 ◽  
pp. 139481 ◽  
Author(s):  
Anouska Panton ◽  
Fay Couceiro ◽  
Gary R. Fones ◽  
Duncan A. Purdie
Keyword(s):  
Organic Matter ◽  
Dissolved Organic Matter ◽  
Rainfall Events ◽  
Lowland Rivers ◽  
Catchment Characteristics ◽  
Estuarine Processes ◽  
The Impact

scholarly journals The impact of four decades of annual nitrogen addition on dissolved organic matter in a boreal forest soil

2013 ◽  
Vol 10 (3) ◽  
pp. 1365-1377 ◽  
Author(s):  
M. O. Rappe-George ◽  
A. I. Gärdenäs ◽  
D. B. Kleja
Keyword(s):  
Organic Matter ◽  
Dissolved Organic Matter ◽  
Soil Solution ◽  
Mineral Soil ◽  
Solution Concentration ◽  
Oxidative Enzymes ◽  
N Saturation ◽  
N Addition ◽  
Mineral N ◽  
The Impact

Abstract. Addition of mineral nitrogen (N) can alter the concentration and quality of dissolved organic matter (DOM) in forest soils. The aim of this study was to assess the effect of long-term mineral N addition on soil solution concentration of dissolved organic carbon (DOC) and dissolved organic nitrogen (DON) in Stråsan experimental forest (Norway spruce) in central Sweden. N was added yearly at two levels of intensity and duration: the N1 treatment represented a lower intensity but a longer duration (43 yr) of N addition than the shorter N2 treatment (24 yr). N additions were terminated in the N2 treatment in 1991. The N treatments began in 1967 when the spruce stands were 9 yr old. Soil solution in the forest floor O, and soil mineral B, horizons were sampled during the growing seasons of 1995 and 2009. Tension and non-tension lysimeters were installed in the O horizon (n = 6), and tension lysimeters were installed in the underlying B horizon (n = 4): soil solution was sampled at two-week intervals. Although tree growth and O horizon carbon (C) and N stock increased in treatments N1 and N2, the concentration of DOC in O horizon leachates was similar in both N treatments and control. This suggests an inhibitory direct effect of N addition on O horizon DOC. Elevated DON and nitrate in O horizon leachates in the ongoing N1 treatment indicated a move towards N saturation. In B horizon leachates, the N1 treatment approximately doubled leachate concentrations of DOC and DON. DON returned to control levels, but DOC remained elevated in B horizon leachates in N2 plots nineteen years after termination of N addition. We propose three possible explanations for the increased DOC in mineral soil: (i) the result of decomposition of a larger amount of root litter, either directly producing DOC or (ii) indirectly via priming of old SOM, and/or (iii) a suppression of extracellular oxidative enzymes.

Dissolved organic matter and metabolic dynamics in dryland lowland rivers

2020 ◽  
Vol 229 ◽  
pp. 117871 ◽  
Author(s):  
Aleicia Holland ◽  
Paul J. McInerney ◽  
Michael E. Shackleton ◽  
Gavin N. Rees ◽  
Nick R. Bond ◽  
...  
Keyword(s):  
Organic Matter ◽  
Dissolved Organic Matter ◽  
Lowland Rivers

The impact of land use on riparian soil dissolved organic matter and on streamwater quality on Chongming Island, China

2016 ◽  
Vol 16 (8) ◽  
pp. 2399-2408 ◽  
Author(s):  
Changming Yang ◽  
Yulai Wang ◽  
Yachao Jing ◽  
Jianhua Li
Keyword(s):  
Land Use ◽  
Organic Matter ◽  
Dissolved Organic Matter ◽  
Chongming Island ◽  
The Impact

Degradation of nanoplastics in aquatic environments: reactivity and impact on dissolved organic carbon

2020 ◽  
Author(s):  
Angelica Bianco ◽  
Fabrizio Sordello ◽  
Mikael Ehn ◽  
Davide Vione ◽  
Monica Passananti
Keyword(s):  
Organic Matter ◽  
Dissolved Organic Matter ◽  
Aqueous Phase ◽  
Surface Waters ◽  
High Resolution Mass Spectrometry ◽  
Degradation Products ◽  
Plastic Material ◽  
Environmental Models ◽  
Reactivity Constant ◽  
The Impact

<p>The large production of plastic material (PlasticsEurope, 2019), together with the mishandling of plastic waste, has resulted in ubiquitous plastic pollution, which now reaches even the most remote areas of the Earth (Allen et al., 2019; Bergmann et al., 2019). Plastics undergo a slow process of erosion in the environment that decreases their size: microplastics (MPs) and nanoplastics (NPs) have diameters between 1 µm and 5 mm and lower than 1 µm, respectively (Frias and Nash, 2019).</p><p>The occurrence, transformation and fate of MPs and NPs in the environment are still unclear. Therefore, the objective of this work is to better understand the reactivity of NPs using an aqueous suspension of polystyrene NPs (PS-NPs) as a proxy, in the presence of sunlight and chemicals oxidants. The results obtained are relevant to both the atmospheric aqueous phase, such as cloud and fog droplets, and surface waters. We investigated the reactivity of PS-NPs with light and with two important oxidants in the environment: ozone (O<sub>3</sub>) and hydroxyl radicals (<sup>•</sup>OH). The adsorption of ozone (O<sub>3</sub>) on PS-NPs is investigated, showing a significant O<sub>3</sub> uptake. Moreover, for the first time, a reactivity constant with <sup>•</sup>OH is determined. We found a linear correlation between the kinetic constants measured for three different sizes of PS-NPs and the surface exposed by the particles. Degradation products (short chain carboxylic acids and aromatic compounds), obtained by direct and <sup>•</sup>OH-mediated photolysis of PS-NPs suspensions, are identified by high-resolution mass spectrometry. Irradiation of a PS-NPs suspension under natural sunlight for 1 year has shown the formation of formic acid and organic compounds similar to those found in riverine and cloud dissolved organic matter.</p><p>This work is crucial to assess the impact of NPs abiotic degradation in atmospheric and surface waters; indeed, the reactivity constant and the degradation products can be implemented in environmental models to estimate the contribution of NPs degradation to the natural dissolved organic matter in the aqueous phase. A preliminary simulation using APEX (Aqueous Photochemistry of Environmentally occurring Xenobiotics) (Bodrato and Vione, 2014) model shows that in NPs-polluted environments (10<sup>9</sup> particles mL<sup>-1</sup>) there is potential for NPs to significantly scavenge <sup>•</sup>OH, if the content of natural organic matter is not too high, as observed for surface and cloud water.</p><p>Allen, S., et al., 2019.  Nat. Geosci. 12, 339–344. https://doi.org/10.1038/s41561-019-0335-5<br>Bergmann, et al., 2019.  Sci. Adv. 5, eaax1157. https://doi.org/10.1126/sciadv.aax1157<br>Bodrato, M., Vione, D., 2014. Environ. Sci.: Processes Impacts 16, 732–740. https://doi.org/10.1039/C3EM00541K<br>Frias, J., Nash, R., 2019. Mar. Pollut. Bull. 138, 145–147. https://doi.org/10.1016/j.marpolbul.2018.11.022</p>

scholarly journals The impact of climate change on the treatability of dissolved organic matter (DOM) in upland water supplies: A UK perspective

2014 ◽  
Vol 473-474 ◽  
pp. 714-730 ◽  
Author(s):  
J.P. Ritson ◽  
N.J.D. Graham ◽  
M.R. Templeton ◽  
J.M. Clark ◽  
R. Gough ◽  
...  
Keyword(s):  
Climate Change ◽  
Organic Matter ◽  
Dissolved Organic Matter ◽  
Water Supplies ◽  
Impact Of Climate Change ◽  
The Impact

scholarly journals Dissolved organic matter concentration changes in river waters of Latvia

2011 ◽  
Vol 65 (1-2) ◽  
pp. 40-47
Author(s):  
Māris Kļaviņš ◽  
Ilga Kokorīte ◽  
Valērijs Rodinovs
Keyword(s):  
Land Use ◽  
Organic Matter ◽  
Dissolved Organic Matter ◽  
Water Bodies ◽  
Biological Processes ◽  
River Waters ◽  
Organic Matter Concentration ◽  
Concentration Changes ◽  
The Impact ◽  
Matter Concentration

Dissolved organic matter concentration changes in river waters of Latvia Amounts of natural organic matter in surface waters reflect the character and intensity of biological processes in water bodies, human impact and depend on the physico-geographical environment and land-use in the catchments. Thus, analysis of the concentrations and loadings of organic substances to adjacent water bodies can be used to indicate environmental change and human impacts. This study revealed significant increasing trends of total organic carbon (TOC) and water colour in most of the studied Latvian rivers during the last decade. However, over longer time periods, there have been pronounced oscillations of TOC concentrations, stressing the importance of long-term changes of river discharge. On a yearly basis, there was a positive correlation between parameters of organic matter concentration and discharge in all selected rivers. The impact of discharge on concentrations of organic matter can be masked by other factors, such as changes in precipitation, biological processes, soil types and land-use.

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