scholarly journals Biomass Burning Over the United States East Coast and Western North Atlantic Ocean: Implications for Clouds and Air Quality

2021 ◽  
Author(s):  
Ali Hossein Mardi ◽  
Hossein Dadashazar ◽  
David Painemal ◽  
Taylor Shingler ◽  
Shane T. Seaman ◽  
...  
Keyword(s):  
United States ◽  
Air Quality ◽  
Atlantic Ocean ◽  
Biomass Burning ◽  
North Atlantic ◽  
East Coast ◽  
North Atlantic Ocean ◽  
The United States

scholarly journals Natural and Anthropogenic Aerosol Trends from Satellite and Surface Observations and Model Simulations over the North Atlantic Ocean from 2002 to 2012

2016 ◽  
Vol 73 (11) ◽  
pp. 4469-4485 ◽  
Author(s):  
Andrew R. Jongeward ◽  
Zhanqing Li ◽  
Hao He ◽  
Xiaoxiong Xiong
Keyword(s):  
United States ◽  
Atlantic Ocean ◽  
North Atlantic ◽  
North Atlantic Ocean ◽  
The United States ◽  
Transport Processes ◽  
Negative Trend ◽  
Seasonal Trends ◽  
The North ◽  
The North Atlantic

Abstract Aerosols contribute to Earth’s radiative budget both directly and indirectly, and large uncertainties remain in quantifying aerosol effects on climate. Variability in aerosol distribution and properties, as might result from changing emissions and transport processes, must be characterized. In this study, variations in aerosol loading across the eastern seaboard of the United States and the North Atlantic Ocean during 2002 to 2012 are analyzed to examine the impacts of anthropogenic emission control measures using monthly mean data from MODIS, AERONET, and IMPROVE observations and Goddard Chemistry Aerosol Radiation and Transport (GOCART) model simulation. MODIS observes a statistically significant negative trend in aerosol optical depth (AOD) over the midlatitudes (−0.030 decade−1). Correlation analyses with surface AOD from AERONET sites in the upwind region combined with trend analysis from GOCART component AOD confirm that the observed decrease in the midlatitudes is chiefly associated with anthropogenic aerosols that exhibit significant negative trends from the eastern U.S. coast extending over the western North Atlantic. Additional analysis of IMPROVE surface PM2.5 observations demonstrates statistically significant negative trends in the anthropogenic components with decreasing mass concentrations over the eastern United States. Finally, a seasonal analysis of observational datasets is performed. The negative trend seen by MODIS is strongest during spring (MAM) and summer (JJA) months. This is supported by AERONET seasonal trends and is identified from IMPROVE seasonal trends as resulting from ammonium sulfate decreases during these seasons.

scholarly journals Long-term trends in aerosol and precipitation composition over the western North Atlantic Ocean at Bermuda

2014 ◽  
Vol 14 (5) ◽  
pp. 7025-7066 ◽  
Author(s):  
W. C. Keene ◽  
J. L. Moody ◽  
J. N. Galloway ◽  
J. M. Prospero ◽  
O. R. Cooper ◽  
...  
Keyword(s):  
Atlantic Ocean ◽  
North Atlantic ◽  
North Atlantic Ocean ◽  
Flow Regimes ◽  
The United States ◽  
Open Ocean ◽  
Anthropogenic Sources ◽  
Trade Wind ◽  
Chemical Compositions ◽  
Near Surface

Abstract. Since the 1980s, emissions of SO2 and NOx (NO + NO2) from anthropogenic sources in the United States (US) and Europe have decreased significantly suggesting that the export of oxidized S and N compounds from surrounding continents to the atmosphere overlying North Atlantic Ocean (NAO) has also decreased. The chemical compositions of aerosols and precipitation sampled daily on Bermuda (32.27° N, 64.87° W) from 1989 to 1997 and from 2006 to 2009 were evaluated to quantify the magnitudes, significance, and implications of associated tends in atmospheric composition. The chemical data were stratified based on FLEXPART retroplumes into four discrete transport regimes: westerly flow from the eastern North America (NEUS/SEUS); easterly trade-wind flow from northern Africa and the subtropical NAO (Africa); long, open-ocean, anticyclonic flow around the Bermuda High (Oceanic); and transitional flow from the relatively clean open ocean to the polluted northeastern US (North). Based on all data, annual average concentrations of non-sea-salt (nss) SO42- associated with aerosols and annual VWA concentrations in precipitation decreased significantly (by 22 and 49%, respectively) whereas annual VWA concentrations of NH4+ in precipitation increased significantly (by 70%). Corresponding trends in aerosol and precipitation NO3- and of aerosol NH4+ were insignificant. Nss SO42- in precipitation under NEUS/SEUS and Oceanic flow decreased significantly (61% each) whereas corresponding trends in particulate nss SO42- under both flow regimes were insignificant. Trends for precipitation were driven in part by decreasing emissions of SO2 over upwind continents and associated decreases in anthropogenic contributions to nss SO42- concentrations. Under NEUS/SEUS and Oceanic flow, the ratio of anthropogenic to biogenic contributions to to nss SO42- in the column scavenged by precipitation were relatively greater than those in near surface aerosol, which implies that, for these flow regimes, precipitation is a better indicator of overall anthropogenic impacts on the lower troposphere. Particulate nss SO42- under African flow also decreased significantly (34%) whereas the corresponding decrease in nss SO42- associated with precipitation was marginally insignificant. We infer that these trends were driven in part by reductions in the emissions and transport of oxidized S compounds from Europe. The lack of significant trends in NO3- associated with aerosols and precipitation under NEUS/SEUS flow is notable in light of the large decrease (39%) in NOx emissions in the US over the period of record. Rapid chemical processing of oxidized N in marine air contributed to this lack of correspondence. Decreasing ratios of nss SO42- to NH4+ and the significant decreasing trend in precipitation acidity (37%) indicate that the total amount of acidity in the multiphase gas-aerosol system in the western NAO troposphere decreased over the period of record. Decreasing aerosol acidities would have shifted the phase partitioning of total NH3 (NH3 + particulate NH4+) towards the gas phase thereby decreasing the atmospheric lifetime of total NH3 against wet plus dry deposition. The trend of increasing NH4+ in precipitation at Bermuda over the period of record suggests that NH3 emissions from surrounding continents also increased. Decreasing particulate nss SO42- in near-surface air under NEUS/SEUS flow over the period of record suggests a lower limit for net warming in the range of 0.1–0.3 W m-2 resulting from the decreased shortwave scattering and absorption by nss SO42- and associated aerosol constituents.

scholarly journals Hurricane Katrina (2005). Part II: Evolution and Hemispheric Impacts of a Diabatically Generated Warm Pool

2007 ◽  
Vol 135 (12) ◽  
pp. 3927-3949 ◽  
Author(s):  
Ron McTaggart-Cowan ◽  
Lance F. Bosart ◽  
John R. Gyakum ◽  
Eyad H. Atallah
Keyword(s):  
United States ◽  
Hurricane Katrina ◽  
North Atlantic ◽  
North Atlantic Ocean ◽  
Flow Analysis ◽  
Warm Pool ◽  
The United States ◽  
The North ◽  
The North Atlantic ◽  
Upper Level

Abstract The landfall of Hurricane Katrina (2005) near New Orleans, Louisiana, on 29 August 2005 will be remembered as one of the worst natural disasters in the history of the United States. By comparison, the extratropical transition (ET) of the system as it accelerates poleward over the following days is innocuous and the system weakens until its eventual demise off the coast of Greenland. The extent of Katrina’s perturbation of the midlatitude flow would appear to be limited given the lack of reintensification or downstream development during ET. However, the slow progression of a strong upper-tropospheric warm pool across the North Atlantic Ocean in the week following Katrina’s landfall prompts the question of whether even a nonreintensifying ET event can lead to significant modification of the midlatitude flow. Analysis of Hurricane Katrina’s outflow layer after landfall suggests that it does not itself make up the long-lived midlatitude warm pool. However, the interaction between Katrina’s anticyclonic outflow and an approaching baroclinic trough is shown to establish an anomalous southwesterly conduit or “freeway” that injects a preexisting tropospheric warm pool over the southwestern United States into the midlatitudes. This warm pool reduces predictability in medium-range forecasts over the North Atlantic and Europe while simultaneously aiding in the development of Hurricanes Maria and Nate. The origin of the warm pool is shown to be the combination of anticyclonic upper-level features generated by eastern Pacific Hurricane Hilary and the south Asian anticyclone (SAA). The hemispheric nature of the connections involved with the development of the warm pool and its injection into the extratropics has an impact on forecasting, since the predictability issue associated with ET in this case involves far more than the potential reintensification of the transitioning system itself.

scholarly journals Synoptic influences on springtime tropospheric O<sub>3</sub> and CO over the North American export region observed by TES

2009 ◽  
Vol 9 (11) ◽  
pp. 3755-3776 ◽  
Author(s):  
J. Hegarty ◽  
H. Mao ◽  
R. Talbot
Keyword(s):  
Atlantic Ocean ◽  
North Atlantic ◽  
North American ◽  
East Coast ◽  
North Atlantic Ocean ◽  
Free Troposphere ◽  
The North ◽  
Circulation Patterns ◽  
The Us ◽  
Us East Coast

Abstract. The relationship between synoptic circulation patterns over the western North Atlantic Ocean in spring (March, April, and May) and tropospheric O3 and CO was investigated using retrievals from the Tropospheric Emission Spectrometer (TES) for 2005 and 2006. Seasonal composites of TES retrievals reprocessed to remove the artificial geographic structure added from the a priori revealed a channel of slightly elevated O3 (>55 ppbv) and CO (>115 ppbv) at the 681 hPa retrieval level between 30° N and 45° N extending from North America out over the Atlantic Ocean. Ozone and CO in this region were correlated at r=0.22 with a slope value of 0.13 mol mol−1 indicative of the overall impact of photochemical chemical processes in North American continental export. Composites of TES retrievals for the six predominant circulation patterns identified as map types from sea level pressure fields of the NCEP FNL analyses showed large variability in the distribution of tropospheric O3. Map types MAM2 and MAM3 featuring cyclones near the US east coast produced the greatest export to the lower free troposphere with O3>65 ppbv and a relatively well-defined O3-CO correlation (slope values near 0.20 mol mol−1). The ensembles of HYSPLIT backward trajectories indicated that the high O3 levels were possibly a result of pollutants lofted to the free troposphere by the warm conveyor belt (WCB) of a cyclone. An important finding was that pollutant export occurred in the main WCB branch to the east of the cyclone and in a secondary branch circling to the back of the cyclone center. Conversely, a map type featuring a large anticyclone dominating the flow over the US east coast (MAM6) restricted export with O3 levels generally <55 ppbv and CO levels generally <110 ppbv. There was also evidence of stratospheric intrusions particularly to the north of 45° N in the 316 hPa composites predominately for MAM1 which featured a large cyclone near Newfoundland. However, the concurrence of these intrusions with pollutant export, specifically in the southwestern North Atlantic Ocean, made it difficult to delineate their respective contributions to the 681 hPa O3 composites.

Biomass Burning Smoke Climatology of the United States: Implications for Particulate Matter Air Quality

2017 ◽  
Vol 51 (20) ◽  
pp. 11731-11741 ◽  
Author(s):  
Aaron S. Kaulfus ◽  
Udaysankar Nair ◽  
Daniel Jaffe ◽  
Sundar A. Christopher ◽  
Scott Goodrick
Keyword(s):  
United States ◽  
Particulate Matter ◽  
Air Quality ◽  
Biomass Burning ◽  
The United States

Stock identification of the sciaenid fish Micropogonias undulatus in the western North Atlantic Ocean using parasites as biological tags

2007 ◽  
Vol 81 (2) ◽  
pp. 155-167 ◽  
Author(s):  
Tiffany G. Baker ◽  
Serge Morand ◽  
Charles A. Wenner ◽  
William A. Roumillat ◽  
Isaure de Buron
Keyword(s):  
Atlantic Ocean ◽  
North Atlantic ◽  
North Atlantic Ocean ◽  
The United States ◽  
Atlantic Croaker ◽  
South Atlantic Bight ◽  
Stock Structure ◽  
Micropogonias Undulatus ◽  
Cape Hatteras ◽  
Biological Tags

AbstractProper fisheries management of the Atlantic croaker Micropogonias undulatus is necessary in the United States due to the commercial and recreational importance of this fish species. Croaker stock structure in the western North Atlantic has been investigated in the past by various authors, with inconclusive results. In this study, macroparasites were used as biological tags to identify putative croaker stocks in the area between New Jersey and Florida, which encompasses the Mid Atlantic Bight and the South Atlantic Bight separated at Cape Hatteras, North Carolina. The macroparasite community of the fish was identified, showing the presence of 30 species in four phyla, of which several were new host records, and one species, a monogenean, was new to science. A canonical correspondence analysis was applied to determine the variables responsible for parasite species composition, to resolve the question of croaker stock structure in the western North Atlantic Ocean. This analysis showed that latitude was the deciding variable delineating the parasite community composition of the Atlantic croaker. Among the 30 parasites, 15 were identified as putative tags according to qualitative criteria, and then 10 out of those 15 were selected as being appropriate tags using quantitative criteria. These parasite tags support the presence of two stocks roughly separated at the known biogeographical barrier at Cape Hatteras.

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