scholarly journals Large area perovskite light-emitting diodes by gas-assisted crystallization

2019 ◽  
Vol 7 (13) ◽  
pp. 3795-3801 ◽  
Author(s):  
Vittal Prakasam ◽  
Daniel Tordera ◽  
Francesco Di Giacomo ◽  
Robert Abbel ◽  
Arjan Langen ◽  
...  

An anti-solvent free facile solution processing technique for fabricating perovskite light emitting diodes (PeLEDs), and scaling it up to large areas by slot-die coating.

2015 ◽  
Vol 26 ◽  
pp. 66-74 ◽  
Author(s):  
Kwang-Jun Choi ◽  
Jin-Young Lee ◽  
Jongwoon Park ◽  
Yu-Seok Seo

Micromachines ◽  
2019 ◽  
Vol 10 (1) ◽  
pp. 53 ◽  
Author(s):  
Amruth C ◽  
Marco Colella ◽  
Jonathan Griffin ◽  
James Kingsley ◽  
Nicholas Scarratt ◽  
...  

This study presents the slot-die coating process of two layers of organic materials for the fabrication of organic light emitting diodes (OLEDs). Poly(3,4-ethylenedioxythiophene) polystyrene sulfonate (PEDOT:PSS), which is commonly used in OLEDs and in organic photovoltaic devices as the hole injection layer (HIL), has been deposited via slot-die coating. Uniform films of PEDOT:PSS were obtained after optimizing the slot-die processing parameters: substrate temperature, coating speed, and ink flow rate. The film quality was examined using optical microscopy, profilometry, and atomic force microscopy. Further, poly(9,9-dioctylfluorene) (F8) and poly(9,9-dioctylfluorene-alt-benzothiadiazole) (F8BT), a well know polymer blend F8:F8BT, which is used as an emissive layer in OLEDs, has been slot-die coated. The optoelectronic properties of the slot-die coated F8:F8BT films were examined by means of photoluminescence (PL) and electroluminescence (EL) studies. The fabricated OLEDs, consisting of slot-die coated PEDOT:PSS and F8:F8BT films, were characterized to record the brightness and current efficiency.


2020 ◽  
Author(s):  
Haoran Wang ◽  
Xiwen Gong ◽  
Dewei Zhao ◽  
Yong-Biao Zhao ◽  
Sheng Wang ◽  
...  

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Peipei Du ◽  
Jinghui Li ◽  
Liang Wang ◽  
Liang Sun ◽  
Xi Wang ◽  
...  

AbstractWith rapid advances of perovskite light-emitting diodes (PeLEDs), the large-scale fabrication of patterned PeLEDs towards display panels is of increasing importance. However, most state-of-the-art PeLEDs are fabricated by solution-processed techniques, which are difficult to simultaneously achieve high-resolution pixels and large-scale production. To this end, we construct efficient CsPbBr3 PeLEDs employing a vacuum deposition technique, which has been demonstrated as the most successful route for commercial organic LED displays. By carefully controlling the strength of the spatial confinement in CsPbBr3 film, its radiative recombination is greatly enhanced while the nonradiative recombination is suppressed. As a result, the external quantum efficiency (EQE) of thermally evaporated PeLED reaches 8.0%, a record for vacuum processed PeLEDs. Benefitting from the excellent uniformity and scalability of the thermal evaporation, we demonstrate PeLED with a functional area up to 40.2 cm2 and a peak EQE of 7.1%, representing one of the most efficient large-area PeLEDs. We further achieve high-resolution patterned perovskite film with 100 μm pixels using fine metal masks, laying the foundation for potential display applications. We believe the strategy of confinement strength regulation in thermally evaporated perovskites provides an effective way to process high-efficiency and large-area PeLEDs towards commercial display panels.


2013 ◽  
Vol 14 (8) ◽  
pp. 1939-1945 ◽  
Author(s):  
Philipp Schwamb ◽  
Thilo C.G. Reusch ◽  
Christoph J. Brabec

2017 ◽  
Vol E100.C (2) ◽  
pp. 161-165 ◽  
Author(s):  
Jitsuo OHTA ◽  
Jeong Woo SHON ◽  
Kohei UENO ◽  
Atsushi KOBAYASHI ◽  
Hiroshi FUJIOKA

2021 ◽  
Vol 12 (1) ◽  
Author(s):  
Changjiu Sun ◽  
Yuanzhi Jiang ◽  
Minghuan Cui ◽  
Lu Qiao ◽  
Junli Wei ◽  
...  

AbstractSerious performance decline arose for perovskite light-emitting diodes (PeLEDs) once the active area was enlarged. Here we investigate the failure mechanism of the widespread active film fabrication method; and ascribe severe phase-segregation to be the reason. We thereby introduce L-Norvaline to construct a COO−-coordinated intermediate phase with low formation enthalpy. The new intermediate phase changes the crystallization pathway, thereby suppressing the phase-segregation. Accordingly, high-quality large-area quasi-2D films with desirable properties are obtained. Based on this, we further rationally adjusted films’ recombination kinetics. We reported a series of highly-efficient green quasi-2D PeLEDs with active areas of 9.0 cm2. The peak EQE of 16.4% is achieved in <n > = 3, represent the most efficient large-area PeLEDs yet. Meanwhile, high brightness device with luminance up to 9.1 × 104 cd m−2 has achieved in <n> = 10 film.


2021 ◽  
Vol 314 ◽  
pp. 3-8
Author(s):  
Noel Giebink

Organic optoelectronic devices such as light-emitting diodes and solar cells present unique challenges for surface cleaning and preparation because of their large area and the ‘soft’, thin film nature of the materials involved. This paper gives an introduction to this class of semiconductor devices and covers a recent example of how surface cleaning impacts the long-term reliability of organic light-emitting diodes being commercialized for solid-state lighting.


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