scholarly journals Aerosol profiling during the large scale field campaign CINDI-2

2018 ◽  
Vol 176 ◽  
pp. 10005
Author(s):  
Arnoud Apituley ◽  
Michel Van Roozendael ◽  
Andreas Richter ◽  
Thomas Wagner ◽  
Udo Friess ◽  
...  

For the validation of space borne observations of NO2 and other trace gases from hyperspectral imagers, ground based instruments based on the MAXDOAS technique are an excellent choice, since they rely on similar retrieval techniques as the observations from orbit. To ensure proper traceability of the MAXDOAS observations, a thorough validation and intercomparison is mandatory. Advanced MAXDOAS observation and retrieval techniques enable inferring vertical structure of trace gases and aerosols. These techniques and their results need validation by e.g. lidar techniques. For the proper understanding of the results from passive remote sensing techniques, independent observations are needed that include parameters needed to understand the light paths, i.e. in-situ aerosol observations of optical and microphysical properties, and essential are in particular the vertical profiles of aerosol optical properties by (Raman) lidar. The approach used in the CINDI-2 campaign held in Cabauw in 2016 is presented in this paper and the results will be discussed in the presentation at the conference.

1999 ◽  
Vol 104 (D10) ◽  
pp. 12221-12226 ◽  
Author(s):  
Johan Ström ◽  
Horst Fischer ◽  
Jos Lelieveld ◽  
Franz Schröder

2017 ◽  
Vol 58 ◽  
pp. 10.1-10.21 ◽  
Author(s):  
J. Bühl ◽  
S. Alexander ◽  
S. Crewell ◽  
A. Heymsfield ◽  
H. Kalesse ◽  
...  

Abstract State-of-the-art remote sensing techniques applicable to the investigation of ice formation and evolution are described. Ground-based and spaceborne measurements with lidar, radar, and radiometric techniques are discussed together with a global view on past and ongoing remote sensing measurement campaigns concerned with the study of ice formation and evolution. This chapter has the intention of a literature study and should illustrate the major efforts that are currently taken in the field of remote sensing of atmospheric ice. Since other chapters of this monograph mainly focus on aircraft in situ measurements, special emphasis is put on active remote sensing instruments and synergies between aircraft in situ measurements and passive remote sensing methods. The chapter concentrates on homogeneous and heterogeneous ice formation in the troposphere because this is a major topic of this monograph. Furthermore, methods that deliver direct, process-level information about ice formation are elaborated with a special emphasis on active remote sensing methods. Passive remote sensing methods are also dealt with but only in the context of synergy with aircraft in situ measurements.


2012 ◽  
Vol 5 (1) ◽  
pp. 589-625
Author(s):  
R. E. Mamouri ◽  
A. Papayannis ◽  
V. Amiridis ◽  
D. Müller ◽  
P. Kokkalis ◽  
...  

Abstract. A novel procedure has been developed to retrieve, simultaneously, the optical, microphysical and chemical properties of tropospheric aerosols with a multi-wavelength Raman lidar system in the troposphere over an urban site (Athens, Greece: 37.9° N, 23.6° E, 200 m a.s.l.) using data obtained during the European Space Agency (ESA) THERMOPOLIS project which took place between 15–31 July 2009 over the Greater Athens Area (GAA). We selected to apply our procedure for a case study of intense aerosol layers occurred on 20–21 July 2009. The National Technical University of Athens (NTUA) EOLE 6-wavelength Raman lidar system has been used to provide the vertical profiles of the optical properties of aerosols (extinction and backscatter coefficients, lidar ratio) and the water vapor mixing ratio. An inversion algorithm was used to derive the mean aerosol microphysical properties (mean effective radius – reff), single-scattering albedo (ω) and mean complex refractive index (m) at selected heights in the 2–3 km height region. We found that reff was 0.3–0.4 μm, ω at 532 nm ranged from 0.63 to 0.88 and m ranged from 1.45 + 0.015i to 1.56 + 0.05i, in good accordance with in situ aircraft measurements. The final data set of the aerosol microphysical properties along with the water vapor and temperature profiles were incorporated into the ISORROPIA model to infer an in situ aerosol composition consistent with the retrieved m and ω values. The retrieved aerosol chemical composition in the 2–3 km height region gave a variable range of sulfate (0–60%) and organic carbon (OC) content (0–50%), although the OC content increased (up to 50%) and the sulfate content dropped (up to 30%) around 3 km height; in connection with the retrieved low ω value (0.63), indicates the presence of absorbing biomass burning smoke mixed with urban haze. Finally, the retrieved aerosol microphysical properties were compared with column-integrated sunphotometer data.


1981 ◽  
Vol 103 (2) ◽  
pp. 110-118 ◽  
Author(s):  
T. F. Adams ◽  
S. C. Schmidt ◽  
W. J. Carter

In-situ recovery methods for many of our hydrocarbon and mineral resources depend on the ability to create or enhance permeability in the resource bed to allow uniform and predictable flow. To meet this need, a new branch of geomechanics devoted to computer prediction of explosive rock breakage and permeability enhancement has developed. The computer is used to solve the nonlinear equations of compressible flow, with the explosive behavior and constitutive properties of the medium providing the initial/boundary conditions and material response. Once the resulting computational tool has been verified and calibrated with appropriate large-scale field tests, it can be used to develop and optimize commercially used explosive techniques for in-situ resource recovery.


2008 ◽  
Vol 8 (1) ◽  
pp. 403-452
Author(s):  
M. Salzmann ◽  
M. G. Lawrence ◽  
V. T. J. Phillips ◽  
L. J. Donner

Abstract. A cloud system resolving model including photo-chemistry (CSRMC) has been developed based on a prototype version of the Weather Research and Forecasting (WRF) model and is used to study influences of deep convection on chemistry in the TOGA COARE/CEPEX region. Lateral boundary conditions for trace gases are prescribed from global chemistry-transport simulations, and the vertical advection of trace gases by large scale dynamics, which is not reproduced in a limited area cloud system resolving model, is taken into account. The influences of in situ lightning and other processes on NOx, O3, and HOx(=HO2+OH), in the vicinity of the deep convective systems are investigated in a 7-day 3-D 248×248 km2 horizontal domain simulation and several 2-D sensitivity runs with a 500 km horizontal domain. The fraction of NOx chemically lost within the domain varies between 20 and 24% in the 2-D runs, but is negligible in the 3-D run, in agreement with a lower average NOx concentration in the 3-D run despite a greater number of flashes. In all runs, in situ lightning is found to have only minor impacts on the local O3 budget. Mid-tropospheric entrainment is more important on average for the upward transport of O3 in the 3-D run than in the 2-D runs, but at the same time undiluted O3-poor air from the marine boundary layer reaches the upper troposphere more frequently in the 3-D run than in the 2-D runs, indicating the presence of undiluted convective cores. Near zero O3 volume mixing ratios due to the reaction with lightning-produced NO are only simulated in a 2-D sensitivity run with an extremely high number of NO molecules per flash, which is outside the range of current estimates. Stratosphere to troposphere transport of O3 is simulated to occur episodically in thin filaments, but on average net upward transport of O3 from below ~16 km is simulated in association with mean large scale ascent in the region. Ozone profiles in the TOGA COARE/CEPEX region are suggested to be strongly influenced by the intra-seasonal (Madden-Julian) oscillation.


2012 ◽  
Vol 12 (10) ◽  
pp. 28033-28068
Author(s):  
I. Pisso ◽  
K. S. Law ◽  
F. Fierli ◽  
P. H. Haynes ◽  
P. Hoor ◽  
...  

Abstract. In-situ observations of atmospheric tracers from multiple measurement campaigns over the period 1994–2007 were combined to investigate the Extra-tropical Transition Layer (ExTL) region and the properties of large scale meridional transport. We used potential temperature, equivalent latitude and distance relative to the local dynamical tropopause as vertical coordinates to highlight the behaviour of trace gases in the tropopause region. Vertical coordinates based on constant PV surfaces allowed us to relate the dynamical definition of the tropopause with trace gases distributions and vertical gradients and hence analyse its latitudinal dependence and seasonal variability. Analysis of the available data provides a working definition of the upper limit of the ExTL based on the upper limit of the region of high vertical CO gradient in PV relative coordinates. A secondary local maximum in vertical O3 gradient can be used a proxy for the lower limit, although it is less clearly defined than that of CO. The sloping isopleths of CO and O3 mixing ratios and the CO mixing ratio gradient are consistent with isopleths in purely dynamical diagnostics such as χ30 d, the proportion of air masses in contact with the PBL within one month and underline the differences between the PV based and chemical tropopauses. The use of tropopause relative coordinates allows different seasons to be analysed together to produce climatological means. The weak dependence of dynamical diagnostics of transport on the absolute values of tracer concentrations makes them a suitable process-oriented tool to evaluate global chemical models and make Lagrangian comparisons.


2015 ◽  
Vol 8 (9) ◽  
pp. 9289-9338 ◽  
Author(s):  
M. J. Granados-Muñoz ◽  
J. A. Bravo-Aranda ◽  
D. Baumgardner ◽  
J. L. Guerrero-Rascado ◽  
D. Pérez-Ramírez ◽  
...  

Abstract. In this work we present an analysis of mineral dust optical and microphysical properties obtained from different retrieval techniques applied to active and passive remote sensing measurements, including a comparison with simultaneous in-situ aircraft measurements. Data were collected in a field campaign performed during a mineral dust outbreak a Granada, Spain, experimental site (37.16° N, 3.61° W, 680 m a.s.l.) on the 27 June 2011. Column-integrated properties are provided by sun- and star-photometry which allows a continuous evaluation of the mineral dust optical properties during both day and night-time. Both the Linear Estimation and AERONET (Aerosol Robotic Network) inversion algorithms are applied for the retrieval of the column-integrated microphysical particle properties. In addition, vertically-resolved microphysical properties are obtained from a multi-wavelength Raman lidar system included in EARLINET (European Aerosol Research Lidar Network), by using both LIRIC (Lidar Radiometer Inversion Code) algorithm during daytime and an algorithm applied to the Raman measurements based on the regularization technique during night-time. LIRIC retrievals reveal several dust layers between 3 and 5 km a.s.l. with volume concentrations of the coarse spheroid mode up to 60 μm3 cm−3. The combined use of the regularization and LIRIC methods reveals the night-to-day evolution of the vertical structure of the mineral dust microphysical properties and offers complementary information to that from column-integrated variables retrieved from passive remote sensing. Additionally, lidar depolarization profiles and LIRIC retrieved volume concentration are compared with aircraft in-situ measurements. This study presents for the first time a comparison of both volume concentration and dust particle polarization ratios measured with in-situ and remote sensing techniques. Results for the depolarization measurements in the dust layer indicate reasonable agreement within the estimated uncertainties. The differences in the volume concentration profiles, although somewhat larger, are still within the expected uncertainties.


2012 ◽  
Vol 5 (7) ◽  
pp. 1793-1808 ◽  
Author(s):  
R. E. Mamouri ◽  
A. Papayannis ◽  
V. Amiridis ◽  
D. Müller ◽  
P. Kokkalis ◽  
...  

Abstract. A novel procedure has been developed to retrieve, simultaneously, the optical, microphysical and chemical properties of tropospheric aerosols with a multi-wavelength Raman lidar system in the troposphere over an urban site (Athens, Greece: 37.9° N, 23.6° E, 200 m a.s.l.) using data obtained during the European Space Agency (ESA) THERMOPOLIS project, which took place between 15–31 July 2009 over the Greater Athens Area (GAA). We selected to apply our procedure for a case study of intense aerosol layers that occurred on 20–21 July 2009. The National Technical University of Athens (NTUA) EOLE 6-wavelength Raman lidar system has been used to provide the vertical profiles of the optical properties of aerosols (extinction and backscatter coefficients, lidar ratio) and the water vapor mixing ratio. An inversion algorithm was used to derive the mean aerosol microphysical properties (mean effective radius (reff), single-scattering albedo ω) and mean complex refractive index (m)) at selected heights in the 2–3 km height region. We found that reff was 0.14–0.4 (±0.14) μm, ω was 0.63–0.88 (±0.08) (at 532 nm) and m ranged from 1.44 (±0.10) + 0.01 (±0.01)i to 1.55 (±0.12) + 0.06 (±0.02)i, in good agreement (only for the reff values) with in situ aircraft measurements. The water vapor and temperature profiles were incorporated into the ISORROPIA II model to propose a possible in situ aerosol composition consistent with the retrieved m and ω values. The retrieved aerosol chemical composition in the 2–3 km height region gave a variable range of sulfate (0–60%) and organic carbon (OC) content (0–50%), although the OC content increased (up to 50%) and the sulfate content dropped (up to 30%) around 3 km height; the retrieved low ω value (0.63), indicates the presence of absorbing biomass burning smoke mixed with urban haze. Finally, the retrieved aerosol microphysical properties were compared with column-integrated sun photometer CIMEL data.


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