This paper presents an electromagnetic analysis and experimental verification to optimize the noise, vibration, and harshness (NVH) characteristics of a permanent magnet synchronous generator (PMSG) for wave energy converters (WECs). WECs applicable to breakwater installed in island areas require a wider operating range and a robust design for maintenance compared with wind-turbine systems. Owing to the use of a permanent magnet with a high energy density, the PMSG has a higher power density than other types of generators; however, strong electromagnetic excitation forces that affect the NVH characteristics are generated. Therefore, in this study, the electromagnetic forces are analyzed through an electromagnetic-field analysis using a subdomain analytical method. Based on the analytical solution, electromagnetic forces were determined. Four electromagnetic excitation forces were classified, and the methods for reducing electromagnetic excitation forces are presented here. Finally, a method for evaluating the system resonance through electromechanical analysis is presented. The proposed analysis, optimization, and experimental study are validated through comparison with finite-element analysis and experimental results.