scholarly journals Operation of the boreal peatland methane cycle across the past 16 k.y.

Geology ◽  
2019 ◽  
Vol 48 (1) ◽  
pp. 82-86 ◽  
Author(s):  
Yanhong Zheng ◽  
Zhengkun Fang ◽  
Tongyu Fan ◽  
Zhao Liu ◽  
Zhangzhang Wang ◽  
...  

Abstract The role of boreal wetlands in driving variations in atmospheric methane (CH4) concentrations across the last deglaciation (20–10 ka) and the Holocene is debated. Most studies infer the sources of atmospheric methane via ice-core records of methane concentration and its light stable isotopic composition. However, direct evidence for variations in the methane cycle from the wetlands themselves is relatively limited. Here, we used a suite of biomarker proxies to reconstruct the methane cycle in the Chinese Hani peat across the past 16 k.y. We found two periods of enhanced methanogenesis, at ca. 15–11 ka and ca. 10–6 ka, whereas weak methanogenesis characterized the late Holocene. These periods of enhanced methanogenesis relate to periods of high/increasing temperatures, supporting a temperature control on the wetland methane cycle. We found no biomarker evidence for intense methanotrophy throughout the past 16 k.y., and, contrary to previous studies, we found no clear control of hydrology on the peatland methane cycle. Although the onset of methanogenesis at Hani at ca. 15 ka coincided with a negative shift in methane δ13C in the ice cores, there is no consistent correlation between changes in the reconstructed methane cycle of the boreal Hani peat and atmospheric CH4 concentrations.

2012 ◽  
Vol 8 (4) ◽  
pp. 1213-1221 ◽  
Author(s):  
J. B. Pedro ◽  
S. O. Rasmussen ◽  
T. D. van Ommen

Abstract. Antarctic ice cores provide clear evidence of a close coupling between variations in Antarctic temperature and the atmospheric concentration of CO2 during the glacial/interglacial cycles of at least the past 800-thousand years. Precise information on the relative timing of the temperature and CO2 changes can assist in refining our understanding of the physical processes involved in this coupling. Here, we focus on the last deglaciation, 19 000 to 11 000 yr before present, during which CO2 concentrations increased by ~80 parts per million by volume and Antarctic temperature increased by ~10 °C. Utilising a recently developed proxy for regional Antarctic temperature, derived from five near-coastal ice cores and two ice core CO2 records with high dating precision, we show that the increase in CO2 likely lagged the increase in regional Antarctic temperature by less than 400 yr and that even a short lead of CO2 over temperature cannot be excluded. This result, consistent for both CO2 records, implies a faster coupling between temperature and CO2 than previous estimates, which had permitted up to millennial-scale lags.


2012 ◽  
Vol 8 (1) ◽  
pp. 621-636 ◽  
Author(s):  
J. B. Pedro ◽  
S. O. Rasmussen ◽  
T. D. van Ommen

Abstract. Antarctic ice cores provide clear evidence of a close coupling between variations in Antarctic temperature and the atmospheric concentration of CO2 during the glacial/interglacial cycles of the past 800 thousand years. Precise information on the relative timing of the temperature and CO2 changes can assist in refining our understanding of the physical processes involved in this coupling. Here, we focus on the last deglaciation, 19 000 to 11 000 years before present, during which CO2 concentrations increased by ~80 parts per million by volume and Antarctic temperature increased by ~10 °C. Utilising a recently developed proxy for regional Antarctic temperature, derived from five near-coastal ice cores, and two ice core CO2 records with high dating precision, we show that the increase in CO2 lagged the increase in regional Antarctic temperature by only 0–400 years. This new value for the lag, consistent for both CO2 records, implies a faster feedback between temperature and CO2 than the centennial to millennial-scale lags suggested by previous studies.


2013 ◽  
Vol 9 (3) ◽  
pp. 983-999 ◽  
Author(s):  
E. Capron ◽  
A. Landais ◽  
D. Buiron ◽  
A. Cauquoin ◽  
J. Chappellaz ◽  
...  

Abstract. Correct estimation of the firn lock-in depth is essential for correctly linking gas and ice chronologies in ice core studies. Here, two approaches to constrain the firn depth evolution in Antarctica are presented over the last deglaciation: outputs of a firn densification model, and measurements of δ15N of N2 in air trapped in ice core, assuming that δ15N is only affected by gravitational fractionation in the firn column. Since the firn densification process is largely governed by surface temperature and accumulation rate, we have investigated four ice cores drilled in coastal (Berkner Island, BI, and James Ross Island, JRI) and semi-coastal (TALDICE and EPICA Dronning Maud Land, EDML) Antarctic regions. Combined with available ice core air-δ15N measurements from the EPICA Dome C (EDC) site, the studied regions encompass a large range of surface accumulation rates and temperature conditions. Our δ15N profiles reveal a heterogeneous response of the firn structure to glacial–interglacial climatic changes. While firn densification simulations correctly predict TALDICE δ15N variations, they systematically fail to capture the large millennial-scale δ15N variations measured at BI and the δ15N glacial levels measured at JRI and EDML – a mismatch previously reported for central East Antarctic ice cores. New constraints of the EDML gas–ice depth offset during the Laschamp event (~41 ka) and the last deglaciation do not favour the hypothesis of a large convective zone within the firn as the explanation of the glacial firn model–δ15N data mismatch for this site. While we could not conduct an in-depth study of the influence of impurities in snow for firnification from the existing datasets, our detailed comparison between the δ15N profiles and firn model simulations under different temperature and accumulation rate scenarios suggests that the role of accumulation rate may have been underestimated in the current description of firnification models.


2018 ◽  
Author(s):  
Amaëlle Landais ◽  
Emilie Capron ◽  
Valérie Masson-Delmotte ◽  
Samuel Toucanne ◽  
Rachael Rhodes ◽  
...  

Abstract. The last deglaciation represents the most recent example of natural global warming associated with large-scale climate changes. In addition to the long-term global temperature increase, the last deglaciation onset is punctuated by a sequence of abrupt changes in the Northern Hemisphere. Such interplay between orbital- and millennial-scale variability is widely documented in paleoclimatic records but the underlying mechanisms are not fully understood. Limitations arise from the difficulty in constraining the sequence of events between external forcing, high- and low- latitude climate and environmental changes. Greenland ice cores provide sub-decadal-scale records across the last deglaciation and contain fingerprints of climate variations occurring in different regions of the Northern Hemisphere. Here, we combine new ice d-excess and 17O-excess records, tracing changes in the mid-latitudes, with ice δ18O records of polar climate. Within Heinrich Stadial 1, we demonstrate a decoupling between climatic conditions in Greenland and those of the lower latitudes. While Greenland temperature remains mostly stable from 17.5 to 14.7 ka, significant change in the mid latitudes of northern Atlantic takes place at ~ 16.2 ka, associated with warmer and wetter conditions of Greenland moisture sources. We show that this climate modification is coincident with abrupt changes in atmospheric CO2 and CH4 concentrations recorded in an Antarctic ice core. Our coherent ice core chronological framework and comparison with other paleoclimate records suggests a mechanism involving two-step freshwater fluxes in the North Atlantic associated with a southward shift of the intertropical convergence zone.


2020 ◽  
Author(s):  
Loïc Schmidely ◽  
Lucas Silva ◽  
Christoph Nehrbass-Ahles ◽  
Juhyeong Han ◽  
Jinhwa Shin ◽  
...  

<p> Small air inclusions in ice cores represent a direct archive of past atmospheric compositions, allowing us to measure the concentration of the three most potent non-condensable Greenhouse Gases (GHG) CO<sub>2</sub>, CH<sub>4</sub> and N<sub>2</sub>O as far back as 800,000 years before present (kyr BP). These records demonstrate that transitions from glacial to interglacial conditions are accompanied by a substantial net increase of CO<sub>2</sub>, CH<sub>4</sub> and N<sub>2</sub>O in the atmosphere (Lüthi et al. 2008, Loulergue et al. 2008, Schilt et al. 2010). A sound understanding of the interplay between the reorganization of the climate system and the perturbation of GHG inventories during glacial terminations is partly limited by the temporal resolution of the records derived from ice cores. In fact, with the exception of the last deglaciation (23-9 kyr BP) centennial-scale GHG variability remained uncaptured for precedings glacial terminations.</p><p>In this work, we exploit the exceptionally long temporal coverage of the EPICA Dome C (EDC) ice core to reconstruct, for the first time, centennial-scale fluctuations of CH<sub>4</sub> mole fractions from 145 to 125 kyr BP, encompassing the entire penultimate deglaciation (138-128 kyr BP). With a temporal resolution of ~100 years, our new record is now unveiling all climate-driven signals enclosed into the EDC ice core, exploiting the maximum resolution possible at Dome C (). This offers us the opportunity to study the timing and rates of change of CH<sub>4</sub> in unprecedented details.</p><p>Preliminary analysis reveals that the deglacial CH<sub>4 </sub>rise is a superimposition of gradual millennial-scale increases (~0.01-0.02 ppb/year) and abrupt and partly intermittent centennial-scale events (~80-200 ppb in less than a millennium). We will investigate processes modulating the observed changes in the CH<sub>4</sub> cycle, compare the structure of our record with the CH<sub>4</sub> profile of the last deglaciation (Marcott, 2014) and contrast it with the EDC CO<sub>2</sub> and N<sub>2</sub>O records over the penultimate glacial termination now available in similar resolution.</p>


2017 ◽  
Author(s):  
Léa Gest ◽  
Frédéric Parrenin ◽  
Jai Chowdhry Beeman ◽  
Dominique Raynaud ◽  
Tyler J. Fudge ◽  
...  

Abstract. To understand causal relationships in past climate variations, it is essential to have accurate chronologies of paleoclimate records. The last deglaciation, which occurred from 18 000 to 11 000 years ago, is especially interesting, since it is the most recent large climatic variation of global extent. Ice cores in Antarctica provide important paleoclimate proxies, such as regional temperature and global atmospheric CO2. However, temperature is recorded in the ice while CO2 is recorded in the enclosed air bubbles. The ages of the former and of the latter are different since air is trapped at 50–120 m below the surface. It is therefore necessary to correct for this air-ice shift to accurately infer the sequence of events. Here we accurately determine the phasing between East Antarctic temperature and atmospheric CO2 variations during the last deglacial warming based on Antarctic ice core records. We build a stack of East Antarctic temperature variations by averaging the records from 4 ice cores (EPICA Dome C, Dome Fuji, EPICA Dronning Maud Land and Talos Dome), all accurately synchronized by volcanic event matching. We place this stack onto the WAIS Divide WD2014 age scale by synchronizing EPICA Dome C and WAIS Divide using volcanic event matching, which allows comparison with the high resolution CO2 record from WAIS Divide. Since WAIS Divide is a high accumulation site, its air age scale, which has previously been determined by firn modeling, is more robust. Finally, we assess the CO2/Antarctic temperature phasing by determining four periods when their trends change abruptly. We find that at the onset of the last deglaciation and at the onset of the Antarctic Cold Reversal (ACR) period CO2 and Antarctic temperature are synchronous within a range of 210 years. Then CO2 slightly leads by 165 ± 116 years at the end of the Antarctic Cold Reversal (ACR) period. Finally, Antarctic temperature significantly leads by 406 ± 200 years at the onset of the Holocene period. Our results further support the hypothesis of no convective zone at EPICA Dome C during the last deglaciation and the use of nitrogen-15 to infer the height of the diffusive zone. Future climate and carbon cycle modeling works should take into account this robust phasing constraint.


2021 ◽  
Vol 17 (4) ◽  
pp. 1627-1643
Author(s):  
Loïc Schmidely ◽  
Christoph Nehrbass-Ahles ◽  
Jochen Schmitt ◽  
Juhyeong Han ◽  
Lucas Silva ◽  
...  

Abstract. Deglaciations are characterized by the largest natural changes in methane (CH4) and nitrous oxide (N2O) concentrations of the past 800 000 years. Reconstructions of millennial- to centennial-scale variability within these periods are mostly restricted to the last deglaciation. In this study, we present composite records of CH4 and N2O concentrations from the EPICA Dome C ice core covering the penultimate deglaciation at temporal resolutions of ∼100 years. Our data permit the identification of centennial-scale fluctuations during the transition from glacial to interglacial levels. At ∼134 000 and ∼129 000 years before present (hereafter ka), both CH4 and N2O increased on centennial timescales. These abrupt rises are similar to the fluctuations associated with the Dansgaard–Oeschger events identified in the last glacial period. In addition, gradually rising N2O levels at ∼130 ka resemble a pattern of increasing N2O concentrations on millennial timescales characterizing the later part of Heinrich stadials. Overall, the events in CH4 and N2O during the penultimate deglaciation exhibit modes of variability that are also found during the last deglaciation and glacial cycle, suggesting that the processes leading to changes in emission during the transitions were similar but their timing differed.


2012 ◽  
Vol 8 (2) ◽  
pp. 1089-1131 ◽  
Author(s):  
F. Parrenin ◽  
S. Barker ◽  
T. Blunier ◽  
J. Chappellaz ◽  
J. Jouzel ◽  
...  

Abstract. We compare a variety of methods for estimating the gas/ice depth offset (Δdepth) at EPICA Dome C (EDC, East Antarctica). (1) Purely based on modelling efforts, Δdepth can be estimated combining a firn densification with an ice flow model. Observations allow direct and indirect estimate of Δdepth. (2) The diffusive column height can be estimated from δ15N and converted to Δdepth using an ice flow model and assumptions about past average firn density and thickness of the convective zone. (3) Ice and gas synchronisation of the EDC ice core to the GRIP, EDML and TALDICE ice cores shifts the ice/gas offset problem into higher accumulation ice cores where it can be more accurately evaluated. (4) Finally, the bipolar seesaw hypothesis allows us to synchronise the ice isotopic record with the gas CH4 record, the later being taken as a proxy of Greenland temperature. The bipolar seesaw antiphase relationship is generally supported by the ice-gas cross synchronisation between EDC and the GRIP, EDML and TALDICE ice cores, which provide support for method 4. Applying the bipolar seesaw hypothesis to the deeper section of the EDC core confirms that the ice flow is complex and can help improving our reconstruction of the thinning function and thus of the EDC age scale. We confirm that method 1 overestimates the glacial Δdepth at EDC and we suggested that it is due to an overestimation of the glacial Close Off Depth by the firn densification model. In contrast we find that the glaciological models probably underestimate the Δdepth during termination II. Finally, we show that method 2 based on 15N data produces for the last deglaciation a Δdepth estimate which is in good agreement with methods 3 and 4.


2014 ◽  
Vol 10 (3) ◽  
pp. 1195-1209 ◽  
Author(s):  
T. J. Fudge ◽  
E. D. Waddington ◽  
H. Conway ◽  
J. M. D. Lundin ◽  
K. Taylor

Abstract. Antarctic ice cores have often been dated by matching distinctive features of atmospheric methane to those detected in annually dated ice cores from Greenland. Establishing the timescale between these tie-point ages requires interpolation. While the uncertainty at tie points is relatively well described, uncertainty of the interpolation is not. Here we assess the accuracy of three interpolation schemes using data from the WAIS Divide ice core in West Antarctica; we compare the interpolation methods with the annually resolved timescale for the past 30 kyr. Linear interpolation yields large age errors (up to 380 years) between tie points, abrupt changes in duration of climate events at tie points, and an age bias. Interpolations based on the smoothest accumulation rate (ACCUM) or the smoothest annual-layer thickness (ALT) yield timescales that more closely agree with the annually resolved timescale and do not have abrupt changes in duration at tie points. We use ALT to assess the uncertainty in existing timescales for the past 30 kyr from Byrd, Siple Dome, and Law Dome. These ice-core timescales were developed with methods similar to linear interpolation. Maximum age differences exceed 1000 years for Byrd and Siple Dome, and 500 years for Law Dome. For the glacial–interglacial transition (21 to 12 kyr), the existing timescales are, on average, older than ALT by 40 years for Byrd, 240 years for Siple Dome, and 150 years for Law Dome. Because interpolation uncertainty is often not considered, age uncertainties for ice-core records are often underestimated.


2018 ◽  
Vol 14 (10) ◽  
pp. 1405-1415 ◽  
Author(s):  
Amaëlle Landais ◽  
Emilie Capron ◽  
Valérie Masson-Delmotte ◽  
Samuel Toucanne ◽  
Rachael Rhodes ◽  
...  

Abstract. The last deglaciation represents the most recent example of natural global warming associated with large-scale climate changes. In addition to the long-term global temperature increase, the last deglaciation onset is punctuated by a sequence of abrupt changes in the Northern Hemisphere. Such interplay between orbital- and millennial-scale variability is widely documented in paleoclimatic records but the underlying mechanisms are not fully understood. Limitations arise from the difficulty in constraining the sequence of events between external forcing, high- and low- latitude climate, and environmental changes. Greenland ice cores provide sub-decadal-scale records across the last deglaciation and contain fingerprints of climate variations occurring in different regions of the Northern Hemisphere. Here, we combine new ice d-excess and 17O-excess records, tracing changes in the midlatitudes, with ice δ18O records of polar climate. Within Heinrich Stadial 1, we demonstrate a decoupling between climatic conditions in Greenland and those of the lower latitudes. While Greenland temperature remains mostly stable from 17.5 to 14.7 ka, significant change in the midlatitudes of the northern Atlantic takes place at ∼16.2 ka, associated with warmer and wetter conditions of Greenland moisture sources. We show that this climate modification is coincident with abrupt changes in atmospheric CO2 and CH4 concentrations recorded in an Antarctic ice core. Our coherent ice core chronological framework and comparison with other paleoclimate records suggests a mechanism involving two-step freshwater fluxes in the North Atlantic associated with a southward shift of the Intertropical Convergence Zone.


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