scholarly journals Giant excitonic upconverted emission of two-dimensional semiconductor in doubly resonant plasmonic nanocavity

Author(s):  
Pengfei Qi ◽  
Yuchen Dai ◽  
Luo Yang ◽  
Guangyi Tao ◽  
Liheng Zheng ◽  
...  

Abstract Phonon-assisted upconverted emission lies at the heart of energy harvesting, bioimaging, optical cryptography and optical refrigeration. It has been demonstrated that the emerging two-dimensional (2D) semiconductors can provide a great platform for efficient phonon-assisted upconversion due to the enhanced optical transition strength and phonon-exciton interaction of 2D excitons. However, the research on the further enhancement of excitonic upconverted emission in 2D semiconductors is almost blank. Here we report the enhanced multiphoton upconverted emission of 2D excitons in doubly resonant plasmonic nanocavity. Owing to the enhanced light collection, enhanced excitation rate and quantum efficiency enhancement arising from Purcell effect, the upconverted emission amplification of > 1000 folds and the decrease of 2 ~ 3 orders of magnitude for saturated excitation energy density are achieved. These findings pave the way to the development of excitonic upconversion lasing, nanoscopic thermometry and sensing, and open up the possibility of optical refrigeration in future 2D electronic or excitonic devices.

2021 ◽  
Author(s):  
Xiang Wang ◽  
Xin Zhou ◽  
Anyang Cui ◽  
Menghan Deng ◽  
Xionghu Xu ◽  
...  

We demonstrate flexo-photoelectronic effects of both n-type and p-type 2D semiconductors.


Nanoscale ◽  
2015 ◽  
Vol 7 (16) ◽  
pp. 7402-7408 ◽  
Author(s):  
Long Yuan ◽  
Libai Huang

We systematically investigate the exciton dynamics in monolayered, bilayered, and trilayered WS2 two-dimensional (2D) crystals by time-resolved photoluminescence (TRPL) spectroscopy.


2010 ◽  
Vol 25 (11) ◽  
pp. 2355-2363 ◽  
Author(s):  
L. H. FORD

Quantum field theory allows for the suppression of vacuum fluctuations, leading to sub-vacuum phenomena. One of these is the appearance of local negative energy density. Selected aspects of negative energy will be reviewed, including the quantum inequalities which limit its magnitude and duration. However, these inequalities allow the possibility that negative energy and related effects might be observable. Some recent proposals for experiments to search for sub-vacuum phenomena will be discussed. Fluctuations of the energy density around its mean value will also be considered, and some recent results on a probability distribution for the energy density in two dimensional spacetime are summarized.


Nanoscale ◽  
2021 ◽  
Author(s):  
Yiduo Wang ◽  
Yingwei Wang ◽  
Yulan Dong ◽  
Li Zhou ◽  
Hao Wei ◽  
...  

To date, outstanding linear and nonlinear optical properties of tellurene, caused by multiple two-dimensional (2D) phases and optical anisotropy, have been attracted considerable interest for potential nanophotonics applications. In this...


2017 ◽  
pp. 1584-1596
Author(s):  
Ravinder Singh ◽  
Helen Huiru Lou

Liquefaction of natural gas helps in transporting it over long distances by sea vessels. It is then regasified and transported through pipelines to the consumer. Due to large energy density of Liquefied Natural Gas (LNG), and associated flammability issues, the LNG terminal involves high risk. Consequently, safety is an important factor in the operation of LNG terminals. Although a substantial amount of time money and effort has been put in this area, there is always some possibility of improving the process so that less risk is involved. Rapid advancement in process simulation software like Aspen Plus and Aspen HYSYS, has led to the convenience of experimenting the various control methodologies on the computer offline from the actual plant operation, before they are implemented in real time. In this chapter, main hazards associated with LNG terminal operation will be highlighted. Further, recent advancements in research for safety enhancement and efficiency enhancement in the liquefaction and regasification processes will also be included.


Nanoscale ◽  
2019 ◽  
Vol 11 (21) ◽  
pp. 10546-10554 ◽  
Author(s):  
Zhongbin Pan ◽  
Qiling Ding ◽  
Lingmin Yao ◽  
Shuangwu Huang ◽  
Shuang Xing ◽  
...  

Nanocomposite films loaded with small 2D NaNbO3@Al2O3 platelets exhibit a high discharge energy density of 14.59 J cm−3 and simultaneously an outstanding discharge efficiency of 70.1%.


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