scholarly journals Distribution and Driving Mechanism of N2O in Sea Ice and Its Underlying Seawater during Arctic Melt Season

Water ◽  
2022 ◽  
Vol 14 (2) ◽  
pp. 145
Author(s):  
Jian Liu ◽  
Liyang Zhan ◽  
Qingkai Wang ◽  
Man Wu ◽  
Wangwang Ye ◽  
...  

Nitrous oxide (N2O) is the third most important greenhouse gas in the atmosphere, and the ocean is an important source of N2O. As the Arctic Ocean is strongly affected by global warming, rapid ice melting can have a significant impact on the N2O pattern in the Arctic environment. To better understand this impact, N2O concentration in ice core and underlying seawater (USW) was measured during the seventh Chinese National Arctic Research Expedition (CHINARE2016). The results showed that the average N2O concentration in first-year ice (FYI) was 4.5 ± 1.0 nmol kg−1, and that in multi-year ice (MYI) was 4.8 ± 1.9 nmol kg−1. Under the influence of exchange among atmosphere-sea ice-seawater systems, brine dynamics and possible N2O generation processes at the bottom of sea ice, the FYI showed higher N2O concentrations at the bottom and surface, while lower N2O concentrations were seen inside sea ice. Due to the melting of sea ice and biogeochemical processes, USW presented as the sink of N2O, and the saturation varied from 47.2% to 102.2%. However, the observed N2O concentrations in USW were higher than that of T-N2OUSW due to the sea–air exchange, diffusion process, possible N2O generation mechanism, and the influence of precipitation, and a more detailed mechanism is needed to understand this process in the Arctic Ocean.

2008 ◽  
Vol 21 (5) ◽  
pp. 866-882 ◽  
Author(s):  
Irina V. Gorodetskaya ◽  
L-Bruno Tremblay ◽  
Beate Liepert ◽  
Mark A. Cane ◽  
Richard I. Cullather

Abstract The impact of Arctic sea ice concentrations, surface albedo, cloud fraction, and cloud ice and liquid water paths on the surface shortwave (SW) radiation budget is analyzed in the twentieth-century simulations of three coupled models participating in the Intergovernmental Panel on Climate Change Fourth Assessment Report. The models are the Goddard Institute for Space Studies Model E-R (GISS-ER), the Met Office Third Hadley Centre Coupled Ocean–Atmosphere GCM (UKMO HadCM3), and the National Center for Atmosphere Research Community Climate System Model, version 3 (NCAR CCSM3). In agreement with observations, the models all have high Arctic mean cloud fractions in summer; however, large differences are found in the cloud ice and liquid water contents. The simulated Arctic clouds of CCSM3 have the highest liquid water content, greatly exceeding the values observed during the Surface Heat Budget of the Arctic Ocean (SHEBA) campaign. Both GISS-ER and HadCM3 lack liquid water and have excessive ice amounts in Arctic clouds compared to SHEBA observations. In CCSM3, the high surface albedo and strong cloud SW radiative forcing both significantly decrease the amount of SW radiation absorbed by the Arctic Ocean surface during the summer. In the GISS-ER and HadCM3 models, the surface and cloud effects compensate one another: GISS-ER has both a higher summer surface albedo and a larger surface incoming SW flux when compared to HadCM3. Because of the differences in the models’ cloud and surface properties, the Arctic Ocean surface gains about 20% and 40% more solar energy during the melt period in the GISS-ER and HadCM3 models, respectively, compared to CCSM3. In twenty-first-century climate runs, discrepancies in the surface net SW flux partly explain the range in the models’ sea ice area changes. Substantial decrease in sea ice area simulated during the twenty-first century in CCSM3 is associated with a large drop in surface albedo that is only partly compensated by increased cloud SW forcing. In this model, an initially high cloud liquid water content reduces the effect of the increase in cloud fraction and cloud liquid water on the cloud optical thickness, limiting the ability of clouds to compensate for the large surface albedo decrease. In HadCM3 and GISS-ER, the compensation of the surface albedo and cloud SW forcing results in negligible changes in the net SW flux and is one of the factors explaining moderate future sea ice area trends. Thus, model representations of cloud properties for today’s climate determine the ability of clouds to compensate for the effect of surface albedo decrease on the future shortwave radiative budget of the Arctic Ocean and, as a consequence, the sea ice mass balance.


2015 ◽  
Vol 28 (10) ◽  
pp. 4027-4033 ◽  
Author(s):  
Doo-Sun R. Park ◽  
Sukyoung Lee ◽  
Steven B. Feldstein

Abstract Wintertime Arctic sea ice extent has been declining since the late twentieth century, particularly over the Atlantic sector that encompasses the Barents–Kara Seas and Baffin Bay. This sea ice decline is attributable to various Arctic environmental changes, such as enhanced downward infrared (IR) radiation, preseason sea ice reduction, enhanced inflow of warm Atlantic water into the Arctic Ocean, and sea ice export. However, their relative contributions are uncertain. Utilizing ERA-Interim and satellite-based data, it is shown here that a positive trend of downward IR radiation accounts for nearly half of the sea ice concentration (SIC) decline during the 1979–2011 winter over the Atlantic sector. Furthermore, the study shows that the Arctic downward IR radiation increase is driven by horizontal atmospheric water flux and warm air advection into the Arctic, not by evaporation from the Arctic Ocean. These findings suggest that most of the winter SIC trends can be attributed to changes in the large-scale atmospheric circulations.


2009 ◽  
Vol 22 (1) ◽  
pp. 165-176 ◽  
Author(s):  
R. W. Lindsay ◽  
J. Zhang ◽  
A. Schweiger ◽  
M. Steele ◽  
H. Stern

Abstract The minimum of Arctic sea ice extent in the summer of 2007 was unprecedented in the historical record. A coupled ice–ocean model is used to determine the state of the ice and ocean over the past 29 yr to investigate the causes of this ice extent minimum within a historical perspective. It is found that even though the 2007 ice extent was strongly anomalous, the loss in total ice mass was not. Rather, the 2007 ice mass loss is largely consistent with a steady decrease in ice thickness that began in 1987. Since then, the simulated mean September ice thickness within the Arctic Ocean has declined from 3.7 to 2.6 m at a rate of −0.57 m decade−1. Both the area coverage of thin ice at the beginning of the melt season and the total volume of ice lost in the summer have been steadily increasing. The combined impact of these two trends caused a large reduction in the September mean ice concentration in the Arctic Ocean. This created conditions during the summer of 2007 that allowed persistent winds to push the remaining ice from the Pacific side to the Atlantic side of the basin and more than usual into the Greenland Sea. This exposed large areas of open water, resulting in the record ice extent anomaly.


2021 ◽  
Author(s):  
David Gareth Babb ◽  
Ryan J. Galley ◽  
Stephen E. L. Howell ◽  
Jack Christopher Landy ◽  
Julienne Christine Stroeve ◽  
...  

2021 ◽  
Vol 34 (10) ◽  
pp. 3799-3819
Author(s):  
Hyung-Gyu Lim ◽  
Jong-Yeon Park ◽  
John P. Dunne ◽  
Charles A. Stock ◽  
Sung-Ho Kang ◽  
...  

AbstractHuman activities such as fossil fuel combustion, land-use change, nitrogen (N) fertilizer use, emission of livestock, and waste excretion accelerate the transformation of reactive N and its impact on the marine environment. This study elucidates that anthropogenic N fluxes (ANFs) from atmospheric and river deposition exacerbate Arctic warming and sea ice loss via physical–biological feedback. The impact of physical–biological feedback is quantified through a suite of experiments using a coupled climate–ocean–biogeochemical model (GFDL-CM2.1-TOPAZ) by prescribing the preindustrial and contemporary amounts of riverine and atmospheric N fluxes into the Arctic Ocean. The experiment forced by ANFs represents the increase in ocean N inventory and chlorophyll concentrations in present and projected future Arctic Ocean relative to the experiment forced by preindustrial N flux inputs. The enhanced chlorophyll concentrations by ANFs reinforce shortwave attenuation in the upper ocean, generating additional warming in the Arctic Ocean. The strongest responses are simulated in the Eurasian shelf seas (Kara, Barents, and Laptev Seas; 65°–90°N, 20°–160°E) due to increased N fluxes, where the annual mean surface temperature increase by 12% and the annual mean sea ice concentration decrease by 17% relative to the future projection, forced by preindustrial N inputs.


2017 ◽  
Vol 122 (7) ◽  
pp. 1632-1654 ◽  
Author(s):  
Pedro Duarte ◽  
Amelie Meyer ◽  
Lasse M. Olsen ◽  
Hanna M. Kauko ◽  
Philipp Assmy ◽  
...  

2018 ◽  
Vol 32 (1) ◽  
pp. 15-32 ◽  
Author(s):  
Qiang Wang ◽  
Claudia Wekerle ◽  
Sergey Danilov ◽  
Dmitry Sidorenko ◽  
Nikolay Koldunov ◽  
...  

Abstract The freshwater stored in the Arctic Ocean is an important component of the global climate system. Currently the Arctic liquid freshwater content (FWC) has reached a record high since the beginning of the last century. In this study we use numerical simulations to investigate the impact of sea ice decline on the Arctic liquid FWC and its spatial distribution. The global unstructured-mesh ocean general circulation model Finite Element Sea Ice–Ocean Model (FESOM) with 4.5-km horizontal resolution in the Arctic region is applied. The simulations show that sea ice decline increases the FWC by freshening the ocean through sea ice meltwater and modifies upper ocean circulation at the same time. The two effects together significantly increase the freshwater stored in the Amerasian basin and reduce its amount in the Eurasian basin. The salinification of the upper Eurasian basin is mainly caused by the reduction in the proportion of Pacific Water and the increase in that of Atlantic Water (AW). Consequently, the sea ice decline did not significantly contribute to the observed rapid increase in the Arctic total liquid FWC. However, the changes in the Arctic freshwater spatial distribution indicate that the influence of sea ice decline on the ocean environment is remarkable. Sea ice decline increases the amount of Barents Sea branch AW in the upper Arctic Ocean, thus reducing its supply to the deeper Arctic layers. This study suggests that all the dynamical processes sensitive to sea ice decline should be taken into account when understanding and predicting Arctic changes.


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