Numerical simulations of optical properties of Saharan dust aerosols with emphasis on lidar applications

Abstract. As part of the international project entitled "African Monsoon Multidisciplinary Analysis (AMMA)", NAMMA (NASA AMMA) aimed to gain a better understanding of the relationship between the African Easterly Waves (AEWs), the Sahara Air Layer (SAL), and tropical cyclogenesis. The NAMMA airborne field campaign was based out of the Cape Verde Islands during the peak of the hurricane season, i.e., August and September 2006. Multiple Sahara dust layers were sampled during 62 encounters in the eastern portion of the hurricane main development region, covering both the eastern North Atlantic Ocean and the western Saharan desert (i.e., 5–22° N and 10–35° W). The centers of these layers were located at altitudes between 1.5 and 3.3 km and the layer thickness ranged from 0.5 to 3 km. Detailed dust microphysical and optical properties were characterized using a suite of in-situ instruments aboard the NASA DC-8 that included a particle counter, an Ultra-High Sensitivity Aerosol Spectrometer, an Aerodynamic Particle Sizer, a nephelometer, and a Particle Soot Absorption Photometer. The NAAMA sampling inlet has a size cut (i.e., 50% transmission efficiency size) of approximately 4 μm in diameter for dust particles, which limits the representativeness of the NAMMA observational findings. The NAMMA dust observations showed relatively low particle number densities, ranging from 268 to 461 cm−3, but highly elevated volume density with an average at 45 μm3 cm−3. NAMMA dust particle size distributions can be well represented by tri-modal lognormal regressions. The estimated volume median diameter (VMD) is averaged at 2.1 μm with a small range of variation regardless of the vertical and geographical sampling locations. The Ångström Exponent assessments exhibited strong wavelength dependence for absorption but a weak one for scattering. The single scattering albedo was estimated at 0.97 ± 0.02. The imaginary part of the refractive index for Sahara dust was estimated at 0.0022, with a range from 0.0015 to 0.0044. Closure analysis showed that observed scattering coefficients are highly correlated with those calculated from spherical Mie-Theory and observed dust particle size distributions. These values are generally consistent with literature values reported from studies with similar particle sampling size range.

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The Impact of Intense Winter Saharan Dust Events on PM and Optical Properties at Urban Sites in the Southeast of the Iberian Peninsula

Atmosphere ◽

10.3390/atmos12111469 ◽

2021 ◽

Vol 12 (11) ◽

pp. 1469

Author(s):

Alba López-Caravaca ◽

Ramón Castañer ◽

Alvaro Clemente ◽

Eduardo Yubero ◽

Nuria Galindo ◽

...

Keyword(s):

Optical Properties ◽

Iberian Peninsula ◽

Fine Particles ◽

Saharan Dust ◽

Percentile Method ◽

Angstrom Exponent ◽

Ångström Exponent ◽

Dust Events ◽

The Impact ◽

Ångstrom Exponent

The influence of three Saharan dust events (SDE) on particulate matter (PM) concentrations and aerosol optical properties (AOP) during February 2021 was studied. The physical characteristics of the African aerosol were different for each episode. Therefore, the impacts of the three events on PM and AOP were analyzed separately. The monitoring sites were placed in Elche, in the southeast of the Iberian Peninsula. The sites can be classified as urban background locations. The procedure used to obtain the contribution of SDE to PM10 mass concentrations was the 40th percentile method. Nearly half of the days during the study period were under the influence of Saharan air masses. The average contribution of mineral dust (MD) to the PM10 mean concentration was ~50%, which was the highest contribution during the month of February in the last 14 years. The results show that those events characterized by a high input of fine particles (PM1 and PM2.5) caused larger increases in the absorption (σap) and scattering (σsp) coefficients than SDE in which coarse particles predominated. Nevertheless, as expected, SAE (Scattering Angström Exponent) values were lowest during these episodes. AAE (Absorption Angström Exponent) values during SDE were slightly higher than those observed in the absence of African dust, suggesting some contribution from MD to the absorption process.

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Using the OMI Aerosol Index and Absorption Aerosol Optical Depth to evaluate the NASA MERRA Aerosol Reanalysis

Atmospheric Chemistry and Physics Discussions ◽

10.5194/acpd-14-32177-2014 ◽

2014 ◽

Vol 14 (23) ◽

pp. 32177-32231 ◽

Cited By ~ 6

Author(s):

V. Buchard ◽

A. M. da Silva ◽

P. R. Colarco ◽

A. Darmenov ◽

C. A. Randles ◽

...

Keyword(s):

Optical Properties ◽

Aerosol Optical Depth ◽

Optical Depth ◽

Biomass Burning ◽

Saharan Dust ◽

Aerosol Layer ◽

Anthropogenic Aerosols ◽

Aerosol Absorption ◽

Modis Aod ◽

Aerosol Index

Abstract. A radiative transfer interface has been developed to simulate the UV Aerosol Index (AI) from the NASA Goddard Earth Observing System version 5 (GEOS-5) aerosol assimilated fields. The purpose of this work is to use the AI and Aerosol Absorption Optical Depth (AAOD) derived from the Ozone Monitoring Instrument (OMI) measurements as independent validation for the Modern Era Retrospective analysis for Research and Applications Aerosol Reanalysis (MERRAero). MERRAero is based on a version of the GEOS-5 model that is radiatively coupled to the Goddard Chemistry, Aerosol, Radiation, and Transport (GOCART) aerosol module and includes assimilation of Aerosol Optical Depth (AOD) from the Moderate Resolution Imaging Spectroradiometer (MODIS) sensor. Since AI is dependent on aerosol concentration, optical properties and altitude of the aerosol layer, we make use of complementary observations to fully diagnose the model, including AOD from the Multi-angle Imaging SpectroRadiometer (MISR), aerosol retrievals from the Aerosol Robotic Network (AERONET) and attenuated backscatter coefficients from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation (CALIPSO) mission to ascertain potential misplacement of plume height by the model. By sampling dust, biomass burning and pollution events in 2007 we have compared model produced AI and AAOD with the corresponding OMI products, identifying regions where the model representation of absorbing aerosols was deficient. As a result of this study over the Saharan dust region, we have obtained a new set of dust aerosol optical properties that retains consistency with the MODIS AOD data that were assimilated, while resulting in better agreement with aerosol absorption measurements from OMI. The analysis conducted over the South African and South American biomass burning regions indicates that revising the spectrally-dependent aerosol absorption properties in the near-UV region improves the modeled-observed AI comparisons. Finally, during a period where the Asian region was mainly dominated by anthropogenic aerosols, we have performed a qualitative analysis in which the specification of anthropogenic emissions in GEOS-5 is adjusted to provide insight into discrepancies observed in AI comparisons.

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Detection of Saharan dust and biomass burning events using near real-time intensive aerosol optical properties in the northwestern Mediterranean

10.5194/acp-2015-902 ◽

2016 ◽

Author(s):

M. Ealo ◽

A. Alastuey ◽

A. Ripoll ◽

N. Pérez ◽

M. C. Minguillón ◽

...

Keyword(s):

Optical Properties ◽

Biomass Burning ◽

Mineral Dust ◽

Organic Aerosol ◽

Saharan Dust ◽

Aerosol Optical Properties ◽

Angstrom Exponent ◽

Ångström Exponent ◽

Dust Events ◽

Ångstrom Exponent

Abstract. The study of Saharan dust events (SDE) and biomass burning (BB) emissions are both topic of great scientific interest since they are frequent and important polluting scenarios affecting air quality and climate. The main aim of this work is evaluating the feasibility of using near real-time in situ aerosol optical measurements for the detection of these atmospheric events in the Western Mediterranean Basin (WMB). With this aim, intensive aerosol optical properties (SAE: scattering Ångström exponent, AAE: absorption Ångström exponent, SSAAE: single scattering albedo Ångström exponent, and g: asymmetry parameter) were derived from multi-wavelength aerosol light scattering, hemispheric backscattering and absorption measurements performed at regional (Montseny; MSY, 720 m a.s.l.) and continental (Montsec; MSA, 1570 m a.s.l.) background sites in the WMB. A sensitivity study aiming at calibrating the measured intensive optical properties for SDE and BB detection is presented and discussed. The detection of Saharan dust events (SDE) by means of the SSAAE parameter and Ångström matrix depended on the altitude of the measurement station, and on SDE intensity. At MSA (mountain-top site) SSAAE detected around 85% of SDE compared with 50% at MSY station, where pollution episodes dominated by fine anthropogenic particles frequently masked the effect of mineral dust on optical properties during less intense SDE. Furthermore, an interesting feature of SSAAE was its capability to detect the presence of mineral dust after the end of SDE. Thus, resuspension processes driven by summer regional atmospheric circulations and dry conditions after SDE favored the accumulation of mineral dust at regional level having important consequences for air quality. On average, SAE, AAE and g ranged between -0.7 and 1, 1.3 and 2.5, and 0.5 and 0.75, respectively, during SDE. Based on the Aethalometer model, biomass burning (BB) contribution to equivalent black carbon (BC) accounted for 36% and 40% at MSY and MSA respectively. Linear relationships were found between AAE and %BCbb, with AAE values reaching around 1.5 when %BCbb was higher than 50%. BB contribution to organic matter (OM) at MSY was around 30%. Thus FF combustion sources showed important contributions to both BC and OM in the region under study. Results for OM source apportionment showed good agreement with simultaneous biomass burning organic aerosol (BBOA) and hydrocarbon-like organic aerosol (HOA) calculated from Positive Matrix Factorization (PMF) applied to simultaneous Aerosol Mass Spectrometer (ACSM) measurements. A wildfire episode was identified at MSY, showing AAE values up to 2 when daily BB contributions to BC and OM were 73% and 78% respectively.

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Optical properties of Saharan dust during ACE 2

Journal of Geophysical Research Atmospheres ◽

10.1029/98jd01930 ◽

1998 ◽

Vol 103 (D21) ◽

pp. 28079-28092 ◽

Cited By ~ 52

Author(s):

A. Smirnov ◽

B. N. Holben ◽

I. Slutsker ◽

E. J. Welton ◽

P. Formenti

Keyword(s):

Optical Properties ◽

Saharan Dust

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Modelling lidar-relevant optical properties of complex mineral dust aerosols

Tellus B ◽

10.1111/j.1600-0889.2011.00559.x ◽

2011 ◽

Vol 63 (4) ◽

pp. 725-741 ◽

Cited By ~ 76

Author(s):

Josef Gasteiger ◽

Matthias Wiegner ◽

Silke Groß ◽

Volker Freudenthaler ◽

Carlos Toledano ◽

...

Keyword(s):

Optical Properties ◽

Mineral Dust ◽

Dust Aerosols ◽

Mineral Dust Aerosols

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Contribution of IASI to the observation of the dust aerosol diurnal cycle over Sahara

10.5194/egusphere-egu2020-15180 ◽

2020 ◽

Author(s):

virginie capelle ◽

alain chedin ◽

Noelle Scott ◽

Martin Todd

Keyword(s):

Diurnal Cycle ◽

Deep Convection ◽

Dust Emission ◽

Saharan Dust ◽

Dust Aerosols ◽

Source Regions ◽

Resolution Model ◽

High Resolution Model ◽

Dust Distribution ◽

Realistic Information

<p>The Infrared Atmospheric Sounder Interferometer (IASI) is well suited for monitoring of dust aerosols because of its capability to determine both AOD and altitude of the dust layer, and because of the good match between the IASI times of observation (9.30 am and pm, local time) and the time of occurrence of the main Saharan dust uplift mechanisms. Here, starting from IASI-derived dust characteristics for an 11-year period, we assess the capability of IASI to bring realistic information on the dust diurnal cycle. We first show the morning and nighttime climatology of IASI-derived dust AOD for two major dust source regions of the Sahara: The Bodele Depression and the Adrar region. Compared with simulations from a high resolution model, permitting deep convection to be explicitly resolved, IASI performs well. In a second step, a Dust Emission Index specific to IASI is constructed, combining simultaneous information on dust AOD and mean altitude, with the aim of observing the main dust emission areas, daytime and nighttime. Comparisons are then made with other equivalent existing results derived from ground based or other satellite observations. Results demonstrate the capability of IASI to improve the documentation of dust distribution over Sahara over a long period of time. Associating observations of dust aerosols in the visible, on which a majority of aerosol studies are so far based, and in the infrared thus appears as a way to complement the results from other satellite instruments in view of improving our knowledge of their impact on climate.</p>

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