scholarly journals Supplementary material to "Stratospheric aerosol radiative forcing simulated by the chemistry climate model EMAC using aerosol CCI satellite data"

Author(s):  
Christoph Brühl ◽  
Jennifer Schallock ◽  
Klaus Klingmüller ◽  
Charles Robert ◽  
Christine Bingen ◽  
...  
2018 ◽  
Vol 18 (17) ◽  
pp. 12845-12857 ◽  
Author(s):  
Christoph Brühl ◽  
Jennifer Schallock ◽  
Klaus Klingmüller ◽  
Charles Robert ◽  
Christine Bingen ◽  
...  

Abstract. This paper presents decadal simulations of stratospheric and tropospheric aerosol and its radiative effects by the chemistry general circulation model EMAC constrained with satellite observations in the framework of the ESA Aerosol CCI project such as GOMOS (Global Ozone Monitoring by Occultation of Stars) and (A)ATSR ((Advanced) Along Track Scanning Radiometer) on the ENVISAT (European Environmental Satellite), IASI (Infrared Atmospheric Sounding Interferometer) on MetOp (Meteorological Operational Satellite), and, additionally, OSIRIS (Optical Spectrograph and InfraRed Imaging System). In contrast to most other studies, the extinctions and optical depths from the model are compared to the observations at the original wavelengths of the satellite instruments covering the range from the UV (ultraviolet) to terrestrial IR (infrared). This avoids conversion artifacts and provides additional constraints for model aerosol and interpretation of the observations. MIPAS (Michelson Interferometer for Passive Atmospheric Sounding) SO2 limb measurements are used to identify plumes of more than 200 volcanic eruptions. These three-dimensional SO2 plumes are added to the model SO2 at the eruption times. The interannual variability in aerosol extinction in the lower stratosphere, and of stratospheric aerosol radiative forcing at the tropopause, is dominated by the volcanoes. To explain the seasonal cycle of the GOMOS and OSIRIS observations, desert dust simulated by a new approach and transported to the lowermost stratosphere by the Asian summer monsoon and tropical convection turns out to be essential. This also applies to the radiative heating by aerosol in the lowermost stratosphere. The existence of wet dust aerosol in the lowermost stratosphere is indicated by the patterns of the wavelength dependence of extinction in observations and simulations. Additional comparison with (A)ATSR total aerosol optical depth at different wavelengths and IASI dust optical depth demonstrates that the model is able to represent stratospheric as well as tropospheric aerosol consistently.


2009 ◽  
Vol 66 (4) ◽  
pp. 1033-1040 ◽  
Author(s):  
O. E. García ◽  
A. M. Díaz ◽  
F. J. Expósito ◽  
J. P. Díaz ◽  
A. Redondas ◽  
...  

Abstract The influence of mineral dust on ultraviolet energy transfer is studied for two different mineralogical origins. The aerosol radiative forcing ΔF and the forcing efficiency at the surface ΔFeff in the range 290–325 nm were estimated in ground-based stations affected by the Saharan and Asian deserts during the dusty seasons. UVB solar measurements were taken from the World Ozone and Ultraviolet Data Center (WOUDC) for four Asian stations (2000–04) and from the Santa Cruz Observatory, Canary Islands (2002–03), under Gobi and Sahara Desert influences, respectively. The Moderate Resolution Imaging Spectroradiometer (MODIS) aerosol optical depth at 550 nm was used to characterize the aerosol load τ, whereas the aerosol index provided by the Total Ozone Mapping Spectrometer (TOMS) sensor was employed to identify the mineral dust events. The ΔF is strongly affected by the aerosol load, the values found being comparable in both regions during the dusty seasons. Under those conditions, ΔF values as large as −1.29 ± 0.53 W m−2 (τ550 = 0.48 ± 0.24) and −1.43 ± 0.38 W m−2 (τ550 = 0.54 ± 0.26) were reached under Saharan and Asian dust conditions, respectively. Nevertheless, significant differences have been observed in the aerosol radiative forcing per unit of aerosol optical depth in the slant path, τS. The maximum ΔFeff values associated with dust influences were −1.55 ± 0.20 W m−2 τS550−1 for the Saharan region and −0.95 ± 0.11 W m−2 τS550−1 in the Asian area. These results may be used as a benchmark database for establishing aerosol corrections in UV satellite products or in global climate model estimations.


2021 ◽  
Author(s):  
Yaowei Li ◽  
John Dykema ◽  
Frank Keutsch

<p>Model results suggest organic aerosol represents a significant fraction of total stratospheric aerosol radiative forcing, which in itself could represent as much as a quarter of global radiative forcing. Other model investigations suggest that the radiative influence of organic aerosols and dust must be included to obtain consistency with satellite measurements of stratospheric aerosols. <em>In situ</em> observations suggest that stratospheric aerosol composition is strongly vertically dependent and contains a significant organic component in the lower stratosphere. Laboratory studies suggest a range of possible values for the complex refractive index of organic aerosols in the stratosphere. The real part of the refractive index could vary over a range that brackets the value of the real refractive index for pure sulfuric acid/water aerosols. The imaginary part of the refractive index of the organic component is highly uncertain, suggesting aerosols that range from being purely refractive to significantly absorbing (eg, brown carbon). The mixing state of these mixed composition aerosols is also uncertain; depending on the complex refractive index of the organic component, morphological variation could have a significant influence on aerosol radiative properties. In this work we perform a sensitivity study of shortwave radiative forcing of stratospheric aerosols, examining the influence of different plausible values of complex refractive index and particle morphologies. <em>In situ</em> measurements of aerosol size and composition are used to represent the size distribution, vertical profile, and organic mass fraction for the computation of aerosol optical properties. These profiles of aerosol optical properties are used as inputs to a radiative transfer model to calculate profiles of shortwave fluxes and radiative heating rates for standard model atmospheres. The implications of the variations in aerosol optical depth and resulting radiative forcing are interpreted in terms of implications for satellite measurements of stratospheric radiative forcing. The various radiative forcing results and remote sensing implications for different scenarios of organic complex refractive index and morphology call for better understandings of the effects of chemical evolution and transport dynamics on the aerosol optical properties in the stratosphere.</p>


2018 ◽  
Author(s):  
Jill S. Johnson ◽  
Leighton A. Regayre ◽  
Masaru Yoshioka ◽  
Kirsty J. Pringle ◽  
Lindsay A. Lee ◽  
...  

Abstract. Observational constraint of simulated aerosol and cloud properties is an essential part of building trustworthy climate models for calculating aerosol radiative forcing. Models are usually tuned to achieve good agreement with observations, but tuning produces just one of many potential variants of a model, so the model uncertainty cannot be determined. Here we estimate the uncertainty in aerosol effective radiative forcing (ERF) in a tuned climate model by constraining 4 million variants of the HadGEM3-UKCA aerosol-climate model to match nine common observations (top-of-atmosphere shortwave flux, aerosol optical depth, PM2.5, cloud condensation nuclei, concentrations of sulphate, black carbon and organic carbon, as well as decadal trends in aerosol optical depth and surface shortwave radiation.) The model uncertainty is calculated by using a perturbed parameter ensemble that samples twenty-seven uncertainties in both the aerosol model and the physical climate model. Focusing over Europe, we show that the aerosol ERF uncertainty can be reduced by about 30 % by constraining it to the nine observations, demonstrating that producing climate models with an observationally plausible base state can contribute to narrowing the uncertainty in aerosol ERF. However, the uncertainty in the aerosol ERF after observational constraint is large compared to the typical spread of a multi-model ensemble. Our results therefore raise questions about whether the underlying multi-model uncertainty would be larger if similar approaches as adopted here were applied more widely. It is hoped that aerosol ERF uncertainty can be further reduced by introducing process-related constraints, however, any such results will be robust only if the enormous number of potential model variants is explored.


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