scholarly journals The characterization of Taklamakan dust properties using a multi-wavelength Raman polarization lidar in Kashi, China

Author(s):  
Qiaoyun Hu ◽  
Haofei Wang ◽  
Philippe Goloub ◽  
Zhengqiang Li ◽  
Igor Veselovskii ◽  
...  

Abstract. The Taklamakan desert is an important dust source for the global atmospheric dust budget and a cause of the dust weather in Eastern Asia. The characterization of the properties and vertical distributions of Taklamakan dust in the source region is still very limited. To fill this gap, the DAO (Dust Aerosol Observation) was conducted in Kashi, China in 2019. Kashi site is about 150 km to the west rim of the Taklamakan desert and is strongly impacted by desert dust aerosols, especially in spring time, i.e. April and May. Apart from dust, fine particles coming from local anthropogenic emissions or/and transported aerosols are also a non-negligible aerosol component. In this study, we provide the first profiling of the 2α + 3β + 3δ lidar profiles of Taklamakan dust based on a multi-wavelength Raman polarization lidar. Four cases, including two Taklamakan dust events (Case 1 and 2) and two polluted dust events (Case 3 and 4) are presented. The lidar ratio in the Taklamakan dust outbreak is found to be 51 ± 8–56 ± 8 sr at 355 nm and 45 ± 7 sr at 532 nm. The particle linear depolarization ratios are about 0.28 ± 0.04–0.32 ± 0.05 at 355 nm, 0.35 ± 0.05 at 532 nm and 0.31 ± 0.05 at 1064 nm. The observed polluted dust is commonly featured with reduced particle linear depolarization ratio and enhanced extinction and backscatter Angstrom exponent. In Case 3, the lidar ratio of polluted dust is about 42 ± 6 sr at 355 nm and 40 ± 6 sr at 532 nm. The particles linear depolarization ratios decrease to about 0.25, with a weak spectral dependence. In Case 4, the variability of lidar ratio and particle linear depolarization ratio is higher than in Case 3, which reflects the complexity of the nature of mixed pollutant and the mixing state. The results provide the first reference for the characteristics of Taklamakan dust measured by Raman lidar. The data could contribute to complementing the dust model and improving the accuracy of climate modeling.

2020 ◽  
Author(s):  
Kevin Ohneiser ◽  
Albert Ansmann ◽  
Holger Baars ◽  
Patric Seifert ◽  
Boris Barja ◽  
...  

Abstract. We present particle optical properties of stratospheric smoke layers observed over Punta Arenas (53.2° S, 70.9° W), Chile, at the southernmost tip of South America in January 2020. The smoke originated from the record-breaking bushfires in Australia. The stratospheric aerosol optical thickness reached values up to 0.7 at 532 nm in mid January 2020. The measured smoke extinction-to-backscatter ratios (lidar ratios) and linear depolarization ratios at 355 and 532 nm wavelength indicate shape, size, and light-absorption properties and are important input parameters in the analysis of spaceborne lidar observations of the CALIPSO and Aeolus missions. They are also of key importance regarding the homogenization of the overall Aeolus (355 nm wavelength) and CALIPSO (532 nm wavelength) smoke data sets and interpretation of the observations with respect to the spread of the smoke particles across the southern hemisphere and decay of the stratospheric perturbation. We found typical values and spectral dependencies of the lidar ratio and linear depolarization ratio for aged stratospheric smoke. At 355 nm, the lidar ratio and depolarization ratio ranged from 53–97 sr and 0.2–0.26, respectively. At 532 nm, the lidar ratios were higher (76–104 sr) and the depolarization ratios were lower with values around 0.15. The found lidar ratio and depolarization ratio values for Australian smoke are in good agreement with respective ones obtained from observations of stratospheric smoke layers over central Europe originating from the record-breaking Canadian wildfires in the summer of 2017. The higher 532 nm lidar ratios, however, indicate stronger absorption by the Australian smoke particles.


2020 ◽  
Vol 20 (13) ◽  
pp. 8003-8015 ◽  
Author(s):  
Kevin Ohneiser ◽  
Albert Ansmann ◽  
Holger Baars ◽  
Patric Seifert ◽  
Boris Barja ◽  
...  

Abstract. We present particle optical properties of stratospheric smoke layers observed with multiwavelength polarization Raman lidar over Punta Arenas (53.2∘ S, 70.9∘ W), Chile, at the southernmost tip of South America in January 2020. The smoke originated from the record-breaking bushfires in Australia. The stratospheric aerosol optical thickness reached values up to 0.85 at 532 nm in mid-January 2020. The main goal of this rapid communication letter is to provide first stratospheric measurements of smoke extinction-to-backscatter ratios (lidar ratios) and particle linear depolarization ratios at 355 and 532 nm wavelengths. These aerosol parameters are important input parameters in the analysis of spaceborne CALIPSO and Aeolus lidar observations of the Australian smoke spreading over large parts of the Southern Hemisphere in January and February 2020 up to heights of around 30 km. Lidar and depolarization ratios, simultaneously measured at 355 and 532 nm, are of key importance regarding the homogenization of the overall Aeolus (355 nm wavelength) and CALIPSO (532 nm wavelength) lidar data sets documenting the spread of the smoke and the decay of the stratospheric perturbation, which will be observable over the entire year of 2020. We found typical values and spectral dependencies of the lidar ratio and linear depolarization ratio for aged stratospheric smoke. At 355 nm, the lidar ratio and depolarization ratio ranged from 53 to 97 sr (mean 71 sr) and 0.2 to 0.26 (mean 0.23), respectively. At 532 nm, the lidar ratios were higher (75–112 sr, mean 97 sr) and the depolarization ratios were lower with values of 0.14–0.22 (mean 0.18). The determined depolarization ratios for aged Australian smoke are in very good agreement with respective ones for aged Canadian smoke, observed with lidar in stratospheric smoke layers over central Europe in the summer of 2017. The much higher 532 nm lidar ratios, however, indicate stronger absorption by the Australian smoke particles.


2020 ◽  
Vol 20 (22) ◽  
pp. 13817-13834 ◽  
Author(s):  
Qiaoyun Hu ◽  
Haofei Wang ◽  
Philippe Goloub ◽  
Zhengqiang Li ◽  
Igor Veselovskii ◽  
...  

Abstract. The Taklamakan desert is an important dust source for the global atmospheric dust budget and a cause of the dust weather in East Asia. The characterization of Taklamakan dust in the source region is still very limited. To fill this gap, the DAO (dust aerosol observation) was conducted in April 2019 in Kashi, China. The Kashi site is about 150 km from the western rim of the Taklamakan desert and is strongly impacted by desert dust aerosols, especially in spring time, i.e., April and May. According to sun–sky photometer measurements, the aerosol optical depth (at 500 nm) varied in the range of 0.07–4.70, and the Ångström exponent (between 440 and 870 nm) in the range of 0.0–0.8 in April 2019. In this study, we provide the first profiling of the 2α+3β+3δ parameters of Taklamakan dust based on a multiwavelength Mie–Raman polarization lidar. For Taklamakan dust, the Ångström exponent related to the extinction coefficient (EAE, between 355 and 532 nm) is about 0.01 ± 0.30, and the lidar ratio is found to be 45 ± 7 sr (51 ± 8–56 ± 8 sr) at 532 (355) nm. The particle linear depolarization ratios (PLDRs) are about 0.28–0.32 ± 0.07 at 355 nm, 0.36 ± 0.05 at 532 nm and 0.31 ± 0.05 at 1064 nm. Both lidar ratios and depolarization ratios are higher than the typical values of Central Asian dust in the literature. The difference is probably linked to the fact that observations in the DAO campaign were collected close to the dust source; therefore, there is a large fraction of coarse-mode and giant particles (radius >20 µm) in the Taklamakan dust. Apart from dust, fine particles coming from local anthropogenic emissions and long-range transported aerosols are also non-negligible aerosol components. The signatures of pollution emerge when dust concentration decreases. The polluted dust (defined by PLDR532≤0.30 and EAE355-532≥0.20) is featured with reduced PLDRs and enhanced EAE355−532 compared to Taklamakan dust. The mean PLDRs of polluted dust generally distributed in the range of 0.20–0.30. Due to the complexity of the nature of the involved pollutants and their mixing state with dust, the lidar ratios exhibit larger variabilities compared to those of dust. The study provides the first reference of novel characteristics of Taklamakan dust measured by Mie–Raman polarization lidar. The data could contribute to complementing the dust model and improving the accuracy of climate modeling.


2011 ◽  
Vol 11 (4) ◽  
pp. 12763-12803 ◽  
Author(s):  
L. Mona ◽  
A. Amodeo ◽  
G. D'Amico ◽  
A. Giunta ◽  
F. Madonna ◽  
...  

Abstract. Multi-wavelength Raman lidar measurements were performed at CNR-IMAA Atmospheric Observatory (CIAO) during the entire Eyjafjallajökull explosive eruptive period in April–May 2010, whenever weather conditions permitted. A methodology for volcanic layer identification and accurate aerosol typing has been developed on the basis both of the multi-wavelength Raman lidar measurements and EARLINET measurements performed at CIAO since 2000. The aerosol mask for lidar measurements performed at CIAO during the 2010 Eyjafjallajökull eruption has been obtained. Volcanic aerosol layers have been observed in different periods: 19–22 April, 27–29 April, 8–9 May, 13–14 May and 18–19 May. A maximum aerosol optical depth of about 0.12–0.13 was observed on 20 April, 22:00 UTC and 13 May, 20:30 UTC. Volcanic particles have been detected both at low altitudes, in the free troposphere and in the upper troposphere. Intrusions into the PBL have been revealed on 21–22 April and 13 May. In the April–May period Saharan dust intrusions typically occur in Southern Italy. For the period under investigations, a Saharan dust intrusion was observed on 13–14 May: dust and volcanic particles have been simultaneously observed at CIAO both at separated different levels and mixed within the same layer. Lidar ratios at 355 and 532 nm, Ångström exponent at 355/532 nm, backscatter related Ångström exponent at 532/1064 nm and particle linear depolarization ratio at 532 nm measured inside the detected volcanic layers have been discussed. The dependence of these quantities on relative humidity (RH) has been investigated by using co-located microwave profiler measurements. The particle linear depolarization ratio increasing with RH, lidar ratio values at 355 nm around 80 sr, and values of the ratio of lidar ratios greater than 1 suggest the presence of sulfates mixed with continental aerosol. Lower lidar ratio values (around 40 sr) increasing with RH and values of the ratio of lidar ratios lower than 1 indicate the presence of some aged ash inside these sulfate layers.


2020 ◽  
Vol 13 (2) ◽  
pp. 893-905 ◽  
Author(s):  
Elina Giannakaki ◽  
Panos Kokkalis ◽  
Eleni Marinou ◽  
Nikolaos S. Bartsotas ◽  
Vassilis Amiridis ◽  
...  

Abstract. A new method, called ElEx (elastic extinction), is proposed for the estimation of extinction coefficient lidar profiles using only the information provided by the elastic and polarization channels of a lidar system. The method is applicable to lidar measurements both during daytime and nighttime under well-defined aerosol mixtures. ElEx uses the particle backscatter profiles at 532 nm and the vertically resolved particle linear depolarization ratio measurements at the same wavelength. The particle linear depolarization ratio and the lidar ratio values of pure aerosol types are also taken from literature. The total extinction profile is then estimated and compared well with Raman retrievals. In this study, ElEx was applied in an aerosol mixture of marine and dust particles at Finokalia station during the CHARADMExp campaign. Any difference between ElEx and Raman extinction profiles indicates that the nondust component could be probably attributed to polluted marine or polluted continental aerosols. Comparison with sun photometer aerosol optical depth observations is performed as well during daytime. Differences in the total aerosol optical depth are varying between 1.2 % and 72 %, and these differences are attributed to the limited ability of the lidar to correctly represent the aerosol optical properties in the near range due to the overlap problem.


2019 ◽  
Vol 99 ◽  
pp. 02006 ◽  
Author(s):  
Hossein Panahifar ◽  
Hamid Reza Khalesifard

Continuous vertically resolved aerosol measurements using lidar were performed in Tehran, Iran. Lidar results has been used in combination with particulate matter monitoring, synoptic meteorology observa- tion as well as satellite-based measurements. The aerosol types are classified by their optical properties. The volume linear depolarization ratio (VLDR) at 532 nm lies mostly between 0:05-0:10. These results show that mostly urban pollution mixed with particles are present in the atmosphere above Tehran. During dust events, the VLDR at 532 nm lies between 0:20-0:35.


2020 ◽  
Vol 237 ◽  
pp. 05010
Author(s):  
Ourania Soupiona ◽  
Alex Papayannis ◽  
Maria Mylonaki ◽  
Nikolaos Papagiannopoulos ◽  
Pablo Ortiz-Amezcua ◽  
...  

Four years (2014-2017) of observations of depolarization Raman Lidar systems of four EARLINET (European Aerosol research Lidar Network) stations [from West to East: Granada (Spain), Potenza (Italy), Athens (Greece) and Limassol (Cyprus)] were collected and used to a statistical analysis of Saharan dust events over Mediterranean basin. In this study, emphasis is given to the consistency of the particle linear depolarization ratio (δp532), the extinction-to-backscatter ratio mentioned as Lidar Ratio (LR532) and the Aerosol Optical Thickness (AOT532) within the observed Saharan dust layers, corresponding to the visible range (532 nm). Geometrical properties and clusters of aerosol mixtures are also presented. Our clustering was based on previous classification by airborne High Spectral Resolution Lidar (HSRL) observations and was further supported by backward trajectory analysis. We found mean δp532 values of 0.24±0.05, 0.26±0.06, 0.28±0.05 and 0.28±0.04, mean LR532 values of 52±8 sr, 51±9 sr, 52±9 sr and 49±6 sr, mean AOT532 values of 0.40±0.31, 0.11±0.07, 0.12±0.10 and 0.32±0.17 and mean layer thicknesses of 3392±1458 m, 2150±1082 m, 1872±816 m and 1716±567 m for Granada, Potenza, Athens and Limassol respectively. This work could assist in bridging the existing gaps related to the extensive and intensive dust aerosol properties over the Mediterranean and enriching the bibliography about mixed aerosol layers from different sources (e.g. dust and biomass burning (BB) aerosols, dust and urban/ industrial aerosols).


2020 ◽  
Vol 237 ◽  
pp. 02036
Author(s):  
Moritz Haarig ◽  
Holger Baars ◽  
Albert Ansmann ◽  
Ronny Engelmann ◽  
Kevin Ohneiser ◽  
...  

Canadian wildfire smoke was detected in the troposphere and lower stratosphere over Europe in August and September 2017. Lidar measurements from various stations of the European Aerosol Research Lidar Network (EARLINET) observed the stratospheric smoke layer. Triple-wavelength (355, 532, and 1064 nm) lidar measurements of the depolarization and the lidar ratio are reported from Leipzig, Germany. The particle linear depolarization ratio of the wildfire smoke in the stratosphere had an exceptional strong wavelength dependence reaching from 0.22 at 355 nm, to 0.18 at 532 nm, and 0.04 at 1064 nm. The lidar ratio increased with wavelength from 40±16 sr at 355 nm, to 66±12 sr at 532 nm, and 92±27 sr at 1064 nm. The development of the stratospheric smoke plume over several months was studied by long-term lidar measurements in Cyprus. The stratospheric smoke layers increased in altitude up to 24 km height.


2015 ◽  
Vol 15 (23) ◽  
pp. 35237-35276
Author(s):  
E. Giannakaki ◽  
P. G. van Zyl ◽  
D. Müller ◽  
D. Balis ◽  
M. Komppula

Abstract. Optical and microphysical properties of different aerosol types over South Africa measured with a multi-wavelength polarization Raman lidar are presented. This study could assist in bridging existing gaps relating to aerosol properties over South Africa, since limited long-term data of this type is available for this region. The observations were performed under the framework of the EUCAARI campaign in Elandsfontein. The multi-wavelength PollyXT Raman lidar system was used to determine vertical profiles of the aerosol optical properties, i.e. extinction and backscatter coefficients, Ångström exponents, lidar ratio and depolarization ratio. The mean microphysical aerosol proper ties, i.e. effective radius and single scattering, albedo were retrieved with an advanced inversion algorithm. Clear differences were observed for the intensive optical properties of atmospheric layers of biomass burning and urban/industrial aerosols. Our results reveal a wide range of optical and microphysical parameters for biomass burning aerosols. This indicates probable mixing of biomass burning aerosols with desert dust particles, as well as the possible continuous influence of urban/industrial aerosol load in the region. The lidar ratio at 355 nm, the linear particle depolarization ratio at 355 nm and the extinction-related Ångström exponent from 355 to 532 nm were 52 ± 7 sr; 0.9 ± 0.4 % and 2.3 ± 0.5, respectively for urban/industrial aerosols, while these values were 92 ± 10 sr; 3.2 ± 1.3 %; 2.0 ± 0.4 respectively for biomass burning aerosols layers. Biomass burning particles are larger and slightly less absorbing compared to urban/industrial aerosols. The particle effective radius were found to be 0.10 ± 0.03, 0.17 ± 0.04 and 0.13 ± 0.03 μm for urban/industrial, biomass burning, and mixed biomass burning and desert dust aerosols, respectively, while the single scattering albedo at 532 nm were 0.87 ± 0.06, 0.90 ± 0.06, and 0.88 ± 0.07 (at 532 nm), respectively for these three types of aerosols. Our results were within the same range of previously reported values.


2020 ◽  
Author(s):  
Ville Vakkari ◽  
Holger Baars ◽  
Stephanie Bohlmann ◽  
Johannes Bühl ◽  
Mika Komppula ◽  
...  

Abstract. Depolarization ratio is a valuable parameter for lidar-based aerosol categorization. Usually, aerosol particle depolarization ratio is determined at relatively short wavelengths of 355 nm and/or 532 nm, but some multi-wavelength studies including longer wavelengths indicate strong spectral dependency. Here, we investigate the capabilities of Halo Photonics Stream Line Doppler lidars to retrieve the particle linear depolarization ratio at 1565 nm wavelength. We utilize collocated measurements with another lidar system, PollyXT at Limassol, Cyprus, and at Kuopio, Finland, to compare the depolarization ratio observed by the two systems. For mineral dust-dominated cases we find typically a little lower depolarization ratio at 1565 nm than at 355 nm and 532 nm. However, for dust mixed with other aerosol we find higher depolarization ratio at 1565 nm. For polluted marine aerosol we find marginally lower depolarization ratio at 1565 nm compared to 355 nm and 532 nm. For mixed spruce and birch pollen we find a little higher depolarization ratio at 1565 nm compared to 532 nm. Overall, we conclude that Halo Doppler lidars can provide particle linear depolarization ratio at 1565 nm wavelength at least in the lowest 2–3 km above ground.


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