scholarly journals Mixing state of refractory black carbon aerosol in the South Asian outflow over the northern Indian Ocean during winter

2020 ◽  
Author(s):  
Sobhan Kumar Kompalli ◽  
Surendran Nair Suresh Babu ◽  
Krishnaswamy Krishnamoorthy ◽  
Sreedharan Krishnakumari Satheesh ◽  
Mukunda M. Gogoi ◽  
...  
Keyword(s):  
Indian Ocean ◽  
Black Carbon ◽  
South Asian ◽  
Arabian Sea ◽  
Equatorial Indian Ocean ◽  
Mixing State ◽  
Air Masses ◽  
Continental Outflow ◽  
Mass Concentrations

Abstract. Regional climatic implications of aerosol black carbon (BC) are well recognized over South Asia, which has a wide variety of anthropogenic sources in a large abundance. Significant uncertainties remain in its quantification due to lack of sufficient information on the microphysical properties (its concentration, size, and mixing state with other aerosol components), which determine the absorption potential of BC. Especially the information on mixing state of BC is extremely sparse over this region. In this study, first-ever observations of the size distribution and mixing state of individual refractory black carbon (rBC) particles in the south Asian outflow to Southeastern Arabian Sea, northern and equatorial Indian Ocean regions are presented based on measurements using a single particle soot photometer (SP2) aboard the ship cruise of the Integrated Campaign for Aerosols, gases, and Radiation Budget (ICARB-2018) during winter-2018 (16 January to 13 February). The results revealed significant spatial heterogeneity of BC characteristics. Highest rBC mass concentrations (~ 938 ± 293 ng m−3) with the highest relative coating thickness (RCT; the ratio of BC core to its coating diameters) of ~ 2.16 ± 0.19 are found over the Southeast Arabian Sea (SEAS) region, which is in the proximity of the continental outflow. As we move to farther oceanic regions, though the mass concentrations decreased by nearly half (~ 546 ± 80 ng m−3), BC still remained thickly coated (RCT ~ 2.05 ± 0.07). The air over the remote equatorial Indian Ocean, which received considerable marine air masses compared to the other regions, showed the lowest rBC mass concentrations (~ 206 ± 114 ng m−3), with a moderately thick coating (RCT ~ 1.73 ± 0.16). Even over oceanic regions far from the landmass, regions which received the outflow from more industrialized east coast/the Bay of Bengal had thicker coating (~ 104 nm) compared to regions that received outflow from the west coast/peninsular India (~ 86 nm). Although different regions of the ocean depicted contrasting concentrations and mixing state parameters due to varying extent and nature of the continental outflow as well as the atmospheric lifetime of air masses, the modal parameters of rBC mass-size distributions were similar over all the regions. The observed mono-modal distribution with mean mass median diameters (MMD) in the range of 0.19–0.20 μm suggested mixed sources of BC. The mean fraction of BC containing particles (FBC) varied in the range 0.20–0.28 (suggesting significant amounts of non-BC particles), whereas the bulk mixing ratio of coating mass to rBC mass was highest (8.77 ± 2.77) over the outflow regions compared to the remote ocean (4.29 ± 1.54) highlighting the role of outflow in providing condensable material for coating on rBC. These parameters, along with the information on size-resolved mixing state of BC cores, throw light on the role of sources and secondary processing of their complex mixtures for coating on BC under highly polluted conditions. Examination of the non-refractory sub-micrometre aerosol chemical composition obtained using the aerosol chemical speciation monitor (ACSM) suggested that the overall aerosol system was sulfate dominated over the far-oceanic regions. In contrast, organics were equally prominent adjacent to the coastal landmass. Association between the BC mixing state and aerosol chemical composition suggested that sulfate was the probable dominant coating material on rBC cores.

scholarly journals Mixing state of refractory black carbon aerosol in the South Asian outflow over the northern Indian Ocean during winter

2021 ◽  
Vol 21 (11) ◽  
pp. 9173-9199
Author(s):  
Sobhan Kumar Kompalli ◽  
Surendran Nair Suresh Babu ◽  
Krishnaswamy Krishna Moorthy ◽  
Sreedharan Krishnakumari Satheesh ◽  
Mukunda Madhab Gogoi ◽  
...  
Keyword(s):  
Indian Ocean ◽  
Black Carbon ◽  
South Asian ◽  
Equatorial Indian Ocean ◽  
Mixing State ◽  
The South ◽  
Air Masses ◽  
Continental Outflow ◽  
Mass Concentrations

Abstract. Regional climatic implications of aerosol black carbon (BC), which has a wide variety of anthropogenic sources in large abundance, are well recognized over South Asia. Significant uncertainties remain in its quantification due to a lack of sufficient information on the microphysical properties (its concentration, size, and mixing state with other aerosol components) that determine the absorption potential of BC. In particular, the information on the mixing state of BC is extremely sparse over this region. In this study, the first observations of the size distribution and mixing state of individual refractory black carbon (rBC) particles in the South Asian outflow to the south-eastern Arabian Sea and the northern and equatorial Indian Ocean regions are presented based on measurements using a single particle soot photometer (SP2) aboard the Integrated Campaign for Aerosols, gases, and Radiation Budget (ICARB-2018) ship during winter 2018 (16 January to 13 February). The results revealed significant spatial heterogeneity of BC characteristics. The highest rBC mass concentrations (∼938±293 ng m−3) with the highest relative coating thickness (RCT; the ratio of BC core to its coating diameters) of ∼2.16±0.19 are found over the south-east Arabian Sea (SEAS) region, which is in the proximity of the continental outflow. As we move to farther oceanic regions, though the mass concentrations decreased by nearly half (∼546±80 ng m−3), BC still remained thickly coated (RCT∼2.05±0.07). The air over the remote equatorial Indian Ocean, which received considerable marine air masses compared to the other regions, showed the lowest rBC mass concentrations (∼206±114 ng m−3) with a moderately thick coating (RCT∼1.73±0.16). Even over oceanic regions far from the landmass, regions that received the outflow from the more industrialized east coast/the Bay of Bengal had a thicker coating (∼104 nm) compared to regions that received outflow from the west coast and/or peninsular India (∼86 nm). Although different regions of the ocean depicted contrasting concentrations and mixing state parameters due to the varied extent and nature of the continental outflow as well as the atmospheric lifetime of air masses, the modal parameters of rBC mass–size distributions (mean mass median diameters ∼ 0.19–0.20 µm) were similar over all regions. The mean fraction of BC-containing particles (FBC) varied in the range of 0.08–0.12 (suggesting significant amounts of non-BC particles), whereas the bulk mixing ratio of coating mass to rBC mass was highest (8.31±2.40) over the outflow regions compared to the remote ocean (4.24±1.45), highlighting the role of outflow in providing condensable material for coatings on rBC. These parameters, along with the information on the size-resolved mixing state of BC cores, throw light on the role of sources and secondary processing of their complex mixtures for coatings on BC under highly polluted conditions. Examination of the non-refractory sub-micrometre aerosol chemical composition obtained using the aerosol chemical speciation monitor (ACSM) suggested that the overall aerosol system was sulfate-dominated over the far-oceanic regions. In contrast, organics were equally prominent adjacent to the coastal landmass. An association between the BC mixing state and aerosol chemical composition suggested that sulfate was the probable dominant coating material on rBC cores.

scholarly journals Supplementary material to "Mixing state of refractory black carbon aerosol in the South Asian outflow over the northern Indian Ocean during winter"

2020 ◽  
Author(s):  
Sobhan Kumar Kompalli ◽  
Surendran Nair Suresh Babu ◽  
Krishnaswamy Krishnamoorthy ◽  
Sreedharan Krishnakumari Satheesh ◽  
Mukunda M. Gogoi ◽  
...  
Keyword(s):  
Indian Ocean ◽  
Black Carbon ◽  
South Asian ◽  
Mixing State ◽  
The South ◽  
Northern Indian Ocean ◽  
Supplementary Material ◽  
Black Carbon Aerosol

Spatial gradient of aerosol mass concentrations and size distributions over southeastern Arabian Sea and equatorial Indian Ocean during ICARB-2018

2019 ◽  
Vol 213 ◽  
pp. 727-738 ◽  
Author(s):  
Mukunda M. Gogoi ◽  
Chakradhar Rao Tandule ◽  
Jayachandran V ◽  
Sobhan Kumar Kompalli ◽  
Vijayakumar S. Nair ◽  
...  
Keyword(s):  
Indian Ocean ◽  
Arabian Sea ◽  
Equatorial Indian Ocean ◽  
Spatial Gradient ◽  
Size Distributions ◽  
Aerosol Mass ◽  
Southeastern Arabian Sea ◽  
Mass Concentrations

Spatial Structure, Forecast Errors, and Predictability of the South Asian Monsoon in CFS Monthly Retrospective Forecasts

2010 ◽  
Vol 23 (18) ◽  
pp. 4750-4769 ◽  
Author(s):  
Hae-Kyung Lee Drbohlav ◽  
V. Krishnamurthy
Keyword(s):  
Indian Ocean ◽  
Spatial Structure ◽  
South Asian ◽  
Arabian Sea ◽  
Asian Monsoon ◽  
Equatorial Indian Ocean ◽  
Western Indian Ocean ◽  
Eastern Indian Ocean ◽  
Forecast Errors ◽  
Precipitation Anomalies

Abstract The spatial structure of the boreal summer South Asian monsoon in the ensemble mean of monthly retrospective forecasts by the Climate Forecast System of the National Centers for Environmental Prediction is examined. The forecast errors and predictability of the model are assessed. Systematic errors in the forecasts consist of deficient rainfall over India, excess rainfall over the Arabian Sea, and a dipole structure over the equatorial Indian Ocean. On interannual time scale during 1981–2003, two different characteristics of the monsoon are recognized—both in observation and forecasts. One feature seems to indicate that the monsoon is regionally controlled, while the other shows a strong relation with El Niño–Southern Oscillation (ENSO). The spatial structure of the regional monsoon can be characterized by the dominant rainfall between the latitudes of 15°N and 5°S in the western Indian Ocean. The maximum precipitation anomalies in the northern Arabian Sea are associated with the cyclonic circulation, while the precipitation anomalies in the equatorial western Indian Ocean accompany the easterlies over the equatorial Indian Ocean. In the ENSO-related monsoon, strong positive precipitation anomalies prevail from the equatorial eastern Indian Ocean to the western Pacific, inducing westerlies over the equatorial Indian Ocean. The spatial structure of the forecast error shows that the model is inclined to predict the ENSO-related feature more accurately than the regional feature. The predictability is found to be lower over certain areas in the northern and equatorial eastern Indian Ocean. The predictability errors in the northern Indian Ocean diminish for longer forecast leads, presumably because the impact of different initial conditions dissipates with time. On the other hand, predictability errors over the equatorial eastern Indian Ocean grow as the forecast lead increases.

scholarly journals Systematic Errors in South Asian Monsoon Simulation: Importance of Equatorial Indian Ocean Processes

2017 ◽  
Vol 30 (20) ◽  
pp. 8159-8178 ◽  
Author(s):  
H. Annamalai ◽  
Bunmei Taguchi ◽  
Julian P. McCreary ◽  
Motoki Nagura ◽  
Toru Miyama
Keyword(s):  
Indian Ocean ◽  
South Asia ◽  
South Asian ◽  
Coupled Model ◽  
Equatorial Indian Ocean ◽  
Coupled Processes ◽  
Cmip5 Models ◽  
Model Errors ◽  
Bjerknes Feedback ◽  
Sst Bias

Abstract Forecasting monsoon rainfall using dynamical climate models has met with little success, partly due to models’ inability to represent the monsoon climatological state accurately. In this article the nature and dynamical causes of their biases are investigated. The approach is to analyze errors in multimodel-mean climatological fields determined from CMIP5, and to carry out sensitivity experiments using a coupled model [the Coupled Model for the Earth Simulator (CFES)] that does represent the monsoon realistically. Precipitation errors in the CMIP5 models persist throughout the annual cycle, with positive (negative) errors occurring over the near-equatorial western Indian Ocean (South Asia). Model errors indicate that an easterly wind stress bias Δτ along the equator begins during April–May and peaks during November; the severity of the Δτ is that the Wyrtki jets, eastward-flowing equatorial currents during the intermonsoon seasons (April–May and October–November), are almost eliminated. An erroneous east–west SST gradient (warm west and cold east) develops in June. The structure of the model errors indicates that they arise from Bjerknes feedback in the equatorial Indian Ocean (EIO). Vertically integrated moisture and moist static energy budgets confirm that warm SST bias in the western EIO anchors moist processes that cause the positive precipitation bias there. In CFES sensitivity experiments in which Δτ or warm SST bias over the western EIO is artificially introduced, errors in the EIO are similar to those in the CMIP5 models; moreover, precipitation over South Asia is reduced. An overall implication of these results is that South Asian rainfall errors in CMIP5 models are linked to errors of coupled processes in the western EIO, and in coupled models correct representation of EIO coupled processes (Bjerknes feedback) is a necessary condition for realistic monsoon simulation.

scholarly journals Seasonal and interannual variations in the nitrogen cycle in the Arabian Sea

2014 ◽  
Vol 11 (20) ◽  
pp. 5733-5747 ◽  
Author(s):  
T. Rixen ◽  
A. Baum ◽  
B. Gaye ◽  
B. Nagel
Keyword(s):  
Indian Ocean ◽  
Nitrogen Cycle ◽  
Arabian Sea ◽  
Equatorial Indian Ocean ◽  
Global Ocean ◽  
Interannual Variations ◽  
Minimum Zone ◽  
Induced Changes ◽  
Seasonal And Interannual Variations ◽  
Sw Monsoon

Abstract. The Arabian Sea plays an important role in the marine nitrogen cycle because of its pronounced mid-water oxygen minimum zone (OMZ) in which bio-available nitrate (NO3−) is reduced to dinitrogen gas (N2). As the nitrogen cycle can respond fast to climate-induced changes in productivity and circulation, the Arabian Sea sediments are an important palaeoclimatic archive. In order to understand seasonal and interannual variations in the nitrogen cycle, nutrient data were obtained from the literature published prior to 1993, evaluated, and compared with data measured during five expeditions carried out in the framework of the Joint Global Ocean Flux Study (JGOFS) in the Arabian Sea in 1995 and during a research cruise of RV Meteor in 2007. The data comparison showed that the area characterized by a pronounced secondary nitrite maximum (SNM) was by 63% larger in 1995 than a similarly determined estimate based on pre-JGOFS data. This area, referred to as the core of the denitrifying zone, showed strong seasonal and interannual variations driven by the monsoon. During the SW monsoon, the SNM retreated eastward due to the inflow of oxygen-enriched Indian Ocean Central Water (ICW). During the NE monsoon, the SNM expanded westward because of the reversal of the current regime. On an interannual timescale, a weaker SW monsoon decreased the inflow of ICW from the equatorial Indian Ocean and increased the accumulation of denitrification tracers by extending the residence time of water in the SNM. This is supported by palaeoclimatic studies showing an enhanced preservation of accumulative denitrification tracers in marine sediments in conjunction with a weakening of the SW monsoon during the late Holocene.

scholarly journals Response of the South Asian Summer Monsoon to Global Warming: Mean and Synoptic Systems*

2009 ◽  
Vol 22 (4) ◽  
pp. 1014-1036 ◽  
Author(s):  
Markus Stowasser ◽  
H. Annamalai ◽  
Jan Hafner
Keyword(s):  
Indian Ocean ◽  
Arabian Sea ◽  
Climate Model ◽  
Asian Summer Monsoon ◽  
Equatorial Indian Ocean ◽  
South Asian Summer Monsoon ◽  
Eastern Equatorial Indian Ocean ◽  
Asian Summer ◽  
The Mean ◽  
Gfdl Model

Abstract Recent diagnostics with the Geophysical Fluid Dynamics Laboratory Climate Model, version 2.1 (GFDL CM2.1), coupled model’s twentieth-century simulations reveal that this particular model demonstrates skill in capturing the mean and variability associated with the South Asian summer monsoon precipitation. Motivated by this, the authors examine the future projections of the mean monsoon and synoptic systems in this model’s simulations in which quadrupling of CO2 concentrations are imposed. In a warmer climate, despite a weakened cross-equatorial flow, the time-mean precipitation over peninsular parts of India increases by about 10%–15%. This paradox is interpreted as follows: the increased precipitation over the equatorial western Pacific forces an anomalous descending circulation over the eastern equatorial Indian Ocean, the two regions being connected by an overturning mass circulation. The spatially well-organized anomalous precipitation over the eastern equatorial Indian Ocean forces twin anticyclones as a Rossby wave response in the lower troposphere. The southern component of the anticyclone opposes and weakens the climatological cross-equatorial monsoon flow. The patch of easterly anomalies centered in the southern Arabian Sea is expected to deepen the thermocline north of the equator. Both these factors limit the coastal upwelling along Somalia, resulting in local sea surface warming and eventually leading to a local maximum in evaporation over the southern Arabian Sea. It is shown that changes in SST are predominantly responsible for the increase in evaporation over the southern Arabian Sea. The diagnostics suggest that in addition to the increased CO2-induced rise in temperature, evaporation, and atmospheric moisture, local circulation changes in the monsoon region further increase SST, evaporation, and atmospheric moisture, leading to increased rainfall over peninsular parts of India. This result implies that accurate observation of SST and surface fluxes over the Indian Ocean is of urgent need to understand and monitor the response of the monsoon in a warming climate. To understand the regional features of the rainfall changes, the International Pacific Research Center (IPRC) Regional Climate Model (RegCM), with three different resolution settings (0.5° × 0.5°, 0.75° × 0.75°, and 1.0° × 1.0°), was integrated for 20 yr, with lateral and lower boundary conditions taken from the GFDL model. The RegCM solutions confirm the major results obtained from the GFDL model but also capture the orographic nature of monsoon precipitation and regional circulation changes more realistically. The hypothesis that in a warmer climate, an increase in troposphere moisture content favors more intense monsoon depressions is tested. The GFDL model does not reveal any changes, but solutions from the RegCM suggest a statistically significant increase in the number of storms that have wind speeds of 15–20 m s−1 or greater, depending on the resolution employed. Based on these regional model solutions a possible implication is that in a CO2-richer climate an increase in the number of flood days over central India can be expected. The model results obtained here, though plausible, need to be taken with caution since even in this “best” model systematic errors still exist in simulating some aspects of the tropical and monsoon climates.

Arabic as a Language of the South Asian Chancery: Bahmani Communications to the Mamluk Sultanate

Arabica ◽  
2020 ◽  
Vol 67 (4) ◽  
pp. 409-435
Author(s):  
Meia Walravens
Keyword(s):  
Indian Ocean ◽  
Fifteenth Century ◽  
Red Sea ◽  
South Asian ◽  
Cultural Exchange ◽  
The South ◽  
Growing Body ◽  
The Indian Ocean

Abstract A growing body of literature on trade and cultural exchange between the Indian Ocean regions has already contributed significantly to our understanding of these processes and the role of language and writing within them. Yet, the question remains how Arabic correspondence played a part in communications between South Asian powers and the rulers in the Red Sea region. In order to begin filling this lacuna, this article studies epistolary writings from the Bahmani Sultanate (748/1347-934/1528) to the Mamluk Sultanate (648/1250-922/1517) during the second half of the ninth/fifteenth century. The contextualisation and discussion of three letters render insight both into the (up to now unstudied) issues at play in Bahmani-Mamluk relations and into the nature of these Arabic texts.

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